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arXiv:1912.09447 · Physical review. B./Physical review. B

Dynamic process and Uhlmann process: Incompatibility and dynamic phase of mixed quantum states

Hao Guo, Xu-Yang Hou, Yan He, Chih-Chun Chien

Published Mar 16, 2020• 19 citations
arXivHTMLPDF

Abstract

While a pure quantum state may accumulate both the Berry phase and dynamic phase as it undergoes a cyclic path in the parameter space, the situation is more complicated when mixed quantum states are considered. From the Ulhmann bundle, a mixed quantum state can accumulate the Ulhmann phase if the parallel-transport condition is satisfied. However, we show that the Ulhmann process is in general not compatible with the evolution equation of the density matrix governed by the Hamiltonian. Thus a mixed quantum state usually accumulates a dynamic phase during its time evolution. We present the expression of the dynamic phase for mixed quantum states. In examples of one-dimensional two-band models and simple harmonic oscillator, the dynamic phase can take multiple discrete values in cyclic, quasistatic processes at infinitely high temperature due to the resonant points. However, the behavior differs if the energy spectrum is continuous without a band gap. Moreover, there is no natural analog of the dynamic phase in classical systems.

DOI
10.1103/physrevb.101.104310

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While a pure quantum state may accumulate both the Berry phase and dynamic phase as it undergoes a cyclic path in the parameter space, the situation is more complicated when mixed quantum states are considered. From the Ulhmann bundle, a mixed quantum state can accumulate the Ulhmann phase if the parallel-transport condition is satisfied. However, we show that the Ulhmann process is in general not compatible with the evolution equation of the density matrix governed by the Hamiltonian. Thus a mixed quantum state usually accumulates a dynamic phase during its time evolution. We present the expression of the dynamic phase for mixed quantum states. In examples of one-dimensional two-band models and simple harmonic oscillator, the dynamic phase can take multiple discrete values in cyclic, quasistatic processes at infinitely high temperature due to the resonant points. However, the behavior differs if the energy spectrum is continuous without a band gap. Moreover, there is no natural analog of the dynamic phase in classical systems.
Dynamic quantum phase transitions (DQPT) following quantum quenches exhibit singular behavior of the overlap between the initial and evolved states. Here we present a formalism to incorporate a geometric phase into quench dynamics of mixed quantum states, a process named the Uhlmann quench, based on the Uhlmann parallel transport. To overcome the incompatibility between the Uhlmann parallel-transport condition and Hamiltonian dynamics, we formulate the evolution of purification of the density matrix in a form which not only respects the dynamics according to the density matrix but also follows the Uhlmann parallel-transport condition to generate a geometric phase after a quantum quench. For cyclic processes exemplified by a spin-1/2 system, geometric DQPTs (GDQPTs) can emerge with both singular behavior in the dynamic analog of the free energy and jumps of the geometric phase. Moreover, the Uhlmann phase reflecting the holonomy is generated at the end of each cycle. The Uhlmann quench thus paves the way for investigating the interplay between quantum dynamics and geometric processes in mixed states.
Two geometric phases of mixed quantum states, known as the interferometric phase and Uhlmann phase, are generalizations of the Berry phase of pure states. After reviewing the two geometric phases and examining their parallel-transport conditions, we specify a class of cyclic processes that are compatible with both conditions and therefore accumulate both phases through their definitions, respectively. Those processes then facilitate a fair comparison between the two phases. We present exact solutions of two-level and three-level systems to contrast the two phases. While the interferometric phase exhibits finite-temperature transitions only in the three-level system but not the two-level system, the Uhlmann phase shows finite-temperature transitions in both cases. Thus, using the two geometric phases as finite-temperature topological indicators demonstrates the rich physics of topology of mixed states.
The Uhlmann phase extends geometric phases to mixed quantum states via a parallel-transport condition on purification amplitudes, yet its direct implementation under standard Hamiltonian dynamics is obstructed by the non-Hermitian nature of the purification. We establish that for any smooth one-dimensional closed loop of full-rank qubit density matrices, there exists a four-level Hermitian parent Hamiltonian whose doubly degenerate ground-state subspace carries a Wilczek--Zee connection exactly equal to the Uhlmann connection. Consequently, the Uhlmann holonomy is faithfully reproduced by adiabatic evolution in the enlarged system. We further prove that this auxiliary-field construction is obstructed in generic two-dimensional parameter spaces by a Frobenius integrability condition, which we derive explicitly. The one-dimensional Uhlmann phase is thus placed on the same footing as the non-Abelian Berry phase, offering a purely Hermitian, Hamiltonian-based route to simulating mixed-state geometric phases. Numerical integration of the adiabatic dynamics confirms the exact correspondence and validates the convergence to the Uhlmann holonomy in the large-gap limit.
The Loschmidt amplitude of the purified states of mixed-state density matrices is shown to have zeros when the system undergoes a quasistatic, quench, or Uhlmann process. While the Loschmidt-amplitude zero of a quench process corresponds to a dynamical quantum phase transition (DQPT) accompanied by the diverging dynamical free energy, the Loschmidt-amplitude zero of the Uhlmann process corresponds to a topological phase transition (TQPT) accompanied by a jump of the Uhlmann phase. Although the density matrix remains intact in a quasistatic process, the Loschmidt amplitude can have zeros not associated with a phase transition. We present examples of two-level and three-level systems exhibiting finite- or infinite-temperature DQPTs and finite-temperature TQPTs associated with the Loschmidt-amplitude zeros. Moreover, the dynamical phase or geometrical phase of mixed states can be extracted from the Loschmidt amplitude. Those phases may become quantized or exhibit discontinuity at the Loschmidt-amplitude zeros. A spinor representation of the purified states of a general two-level system is presented to offer more insights into the change of purification in different processes. The quasistatic process, for example, is shown to cause a rotation of the spinor.
The Berry phase arises naturally from the adiabatic dynamics of a pure quantum state, whereas the Uhlmann phase is usually formulated kinematically for a prescribed path of mixed states. For a qubit subject to a uniformly gapped conical drive, we obtain the Uhlmann connection and holonomy in closed form for the equilibrium Gibbs cycle. We then solve the corresponding Lindblad equation exactly in the rotating frame and show that its steady state forms a nonequilibrium limit cycle that lags the instantaneous Gibbs cycle. As the driving becomes slow, the Uhlmann phase approaches the equilibrium Uhlmann phase, which cooling then reduces to the Berry phase: in the joint adiabatic and low-temperature limit, the dynamical Uhlmann phase therefore converges to the Berry phase. This grounds the Uhlmann--Berry correspondence in the physical dynamics of an open system. We also characterize the finite-driving corrections, together with the discontinuous πππ jump that the Uhlmann phase undergoes on the equatorial cycle as the temperature is varied. Finally, we examine an isolated transversal gap closing, where this zero-temperature correspondence can break down: the pure-state path becomes open, its closure is ambiguous, and gap-opening regularizations close it along a geodesic set by the direction of the bias field, splitting the Berry phase into a one-parameter family of values. The Gibbs path instead closes smoothly through the maximally mixed state, so the Uhlmann holonomy requires no regularization and remains unique and continuous at every finite temperature. In the low-temperature limit the Uhlmann phase selects a single member of the Berry family---the geodesic closure in the osculating plane, fixed by the velocity and acceleration of the driving field. The Uhlmann--Berry correspondence of the gapped regime thus survives the gap closing as a geodesic selection rule.
Pure-state manifestations of geometric phase are well established and have found applications across essentially all branches of physics, yet their generalization to mixed-state regimes remains largely unexplored experimentally. The Uhlmann geometric phase offers a natural extension of pure-state paradigms and can exhibit a topological character. However, observation of this invariant is impeded by the incompatibility between Uhlmann parallel transport and Hamiltonian dynamics, as well as the difficulty of preparing topologically nontrivial mixed states. To address this challenge, we report an experimentally accessible protocol for directly measuring the mixed-state topological invariant. By engineering controlled nonunitary dynamics in a photonic quantum walk, we prepare topologically nontrivial mixed states from a trivial initial state. Furthermore, by machine-learning the full density matrix in momentum space, we directly extract the quantized geometric phase of the nontrivial mixed states. These results highlight a geometric phase framework that naturally extends to open quantum systems both in and out of thermal equilibrium.