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arXiv:2512.24857

Measuring Mixed-State Topological Invariant in Open Photonic Quantum Walk

Qin-Qin Wang, Xiao-Ye Xu, Yong-Jian Han, Chuan-Feng Li, Guang-Can Guo

quant-phphysics.opticsSubmitted Dec 31, 2025• Announced Jan 1, 2026• 0 citations
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Abstract

Pure-state manifestations of geometric phase are well established and have found applications across essentially all branches of physics, yet their generalization to mixed-state regimes remains largely unexplored experimentally. The Uhlmann geometric phase offers a natural extension of pure-state paradigms and can exhibit a topological character. However, observation of this invariant is impeded by the incompatibility between Uhlmann parallel transport and Hamiltonian dynamics, as well as the difficulty of preparing topologically nontrivial mixed states. To address this challenge, we report an experimentally accessible protocol for directly measuring the mixed-state topological invariant. By engineering controlled nonunitary dynamics in a photonic quantum walk, we prepare topologically nontrivial mixed states from a trivial initial state. Furthermore, by machine-learning the full density matrix in momentum space, we directly extract the quantized geometric phase of the nontrivial mixed states. These results highlight a geometric phase framework that naturally extends to open quantum systems both in and out of thermal equilibrium.

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6 pages, 3 figures

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Pure-state manifestations of geometric phase are well established and have found applications across essentially all branches of physics, yet their generalization to mixed-state regimes remains largely unexplored experimentally. The Uhlmann geometric phase offers a natural extension of pure-state paradigms and can exhibit a topological character. However, observation of this invariant is impeded by the incompatibility between Uhlmann parallel transport and Hamiltonian dynamics, as well as the difficulty of preparing topologically nontrivial mixed states. To address this challenge, we report an experimentally accessible protocol for directly measuring the mixed-state topological invariant. By engineering controlled nonunitary dynamics in a photonic quantum walk, we prepare topologically nontrivial mixed states from a trivial initial state. Furthermore, by machine-learning the full density matrix in momentum space, we directly extract the quantized geometric phase of the nontrivial mixed states. These results highlight a geometric phase framework that naturally extends to open quantum systems both in and out of thermal equilibrium.
Geometrical phases have been applied in virtually every major branch of physics and they play an important role in topology and knot theory in mathematics and quantum computation. However, most of the early works focus on pure quantum states which are very unrealistic and almost never occur in practice. The two existed definitions -Uhlmann's and Sjöqvist's- would result in different values for the geometric phase in general. The definition of geometric phase in mixed state scenario is still an open question. Here we present a unified framework for both approaches within one and the same formalism based on simple interferometry. We then present experimental results which confirm both approaches to mixed state geometric phase and clearly demonstrate that their unification is possible. Our experiments are furthermore the first such to measure Uhlmann's mixed state geometric phase and show in addition that it is different to the Sjöqvist's phase.
Geometric phases play a fundamental role in understanding the geometric structure of quantum states, yet extending the Uhlmann phase to non-Hermitian systems poses significant challenges due to parameter-dependent inner product structures. In this work, we develop a comprehensive theory of the Uhlmann phase for quasi-Hermitian systems, where the physical Hilbert space metric varies with external parameters. By constructing a generalized purification that respects the quasi-Hermitian inner product, we derive the corresponding parallel transport condition and Uhlmann connection. Our analysis reveals that the parameter-dependent metric modifies the Uhlmann connection and leads to a finite-temperature distribution of Uhlmann-phase regions that differs from the standard Hermitian case. Applying this formalism to solvable two-level models, we uncover tunable finite-temperature Uhlmann-phase diagrams, where the parameter-dependent metric shifts and deforms the zeros of the Uhlmann amplitude, thereby reshaping the temperature intervals in which nontrivial Uhlmann phases occur. Furthermore, by extending established interferometric protocols originally developed for Hermitian systems, the geometric amplitude can be recast as a measurable Loschmidt amplitude between purified states, providing a practical and experimentally accessible pathway to investigate quasi-Hermitian mixed-state geometric phases and their finite-temperature transitions. This work establishes a unified framework for understanding mixed-state geometric phases in quasi-Hermitian quantum systems and, through its natural relation to the mixed-state quantum geometric tensor, opens new avenues for exploring local geometry in quasi-Hermitian thermal states.
Meaningful topological invariants for mixed quantum states are challenging to identify as there is no unique way to define them, and most choices do not directly relate to physical observables. Here, we propose a simple pragmatic approach to construct topological invariants of mixed states while preserving a connection to physical observables, by continuously deforming known topological invariants for pure (ground) states. Our approach relies on expectation values of many-body operators, with no reference to single-particle (e.g., Bloch) wavefunctions. To illustrate it, we examine extensions to mixed states of U(1)U(1)U(1) geometric (Berry) phases and their corresponding topological invariant (winding or Chern number). We discuss measurement schemes, and provide a detailed construction of invariants for thermal or more general mixed states of quantum systems with (at least) U(1)U(1)U(1) charge-conservation symmetry, such as quantum Hall insulators.
I will introduce the Uhlmann geometric phase as a tool to characterise density matrices of 1D and 2D topological insulators and superconductors. We achieve this goal by constructing new topological invariants called Topological Uhlmann numbers. Since this phase is formulated for general mixed quantum states, it provides a way to extend topological properties to finite temperature situations. New effects appear such as the existence of critical temperatures, novel thermal-topological transitions in models with high Chern numbers, breakdown of the usual bulk-edge correspondence, … Moreover, as the Uhlmann phase is an observable itself, we analyse potential measurement schemes that could be applicable to current experimental setups like cold atoms in optical lattices.
Two geometric phases of mixed quantum states, known as the interferometric phase and Uhlmann phase, are generalizations of the Berry phase of pure states. After reviewing the two geometric phases and examining their parallel-transport conditions, we specify a class of cyclic processes that are compatible with both conditions and therefore accumulate both phases through their definitions, respectively. Those processes then facilitate a fair comparison between the two phases. We present exact solutions of two-level and three-level systems to contrast the two phases. While the interferometric phase exhibits finite-temperature transitions only in the three-level system but not the two-level system, the Uhlmann phase shows finite-temperature transitions in both cases. Thus, using the two geometric phases as finite-temperature topological indicators demonstrates the rich physics of topology of mixed states.
The Berry phase is a geometric phase of a pure state when the system is adiabatically transported along a loop in its parameter space. The concept of geometric phase has been generalized to mixed states by the so-called Uhlmann phase. However, the Uhlmann phase is constructed from the Uhlmann connection that possesses a well-defined global section. This property implies that the Uhlmann connection is topologically trivial and, as a consequence, the corresponding Chern character vanishes. We propose a modified Chern character whose integral gives the thermal Uhlmann Chern number, which is related to the winding number of the mapping defined by the Hamiltonian. Therefore, the thermal Uhlmann Chern number reflects the topological properties of the underlying Hamiltonian of a mixed state. By including the temperature dependence in the volume integral, we also introduce the nontopological thermal Uhlmann Chern number, which varies with temperature but is not quantized at finite temperatures. We illustrate the applications to a two-band model and a degenerate four-band model.