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arXiv:1911.10488 · Journal of Statistical Mechanics Theory and Experiment

Periodic thermodynamics of a two spin Rabi model

Heinz-Jürgen Schmidt

Published Apr 1, 2020• 6 citations
arXivHTMLPDF

Abstract

Abstract We consider two s = 1/2 spins with Heisenberg coupling and a monochromatic, circularly polarized magnetic field acting only onto one of the two spins. This system turns out to be analytically solvable. Also the statistical distribution of the work performed by the driving forces during one period can be obtained in closed form and the Jarzynski equation can be checked. The mean value of this work, viewed as a function of the physical parameters, exhibits features that can be related to some kind of Rabi oscillation. Moreover, when coupled to a heat bath the two spin system will approach a non-equilibrium steady state (NESS) that can be calculated in the golden rule approximation. The occupation probabilities of the NESS are shown not to be of Boltzmann type, with the exception of a single phase with infinite quasitemperature. The parameter space of the two spin Rabi model can be decomposed into eight phase domains such that the NESS probabilities possess discontinuous derivatives at the phase boundaries. The latter property is shown to hold also for more general periodically driven N -level systems.

DOI
10.1088/1742-5468/ab7812

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Abstract We consider two s = 1/2 spins with Heisenberg coupling and a monochromatic, circularly polarized magnetic field acting only onto one of the two spins. This system turns out to be analytically solvable. Also the statistical distribution of the work performed by the driving forces during one period can be obtained in closed form and the Jarzynski equation can be checked. The mean value of this work, viewed as a function of the physical parameters, exhibits features that can be related to some kind of Rabi oscillation. Moreover, when coupled to a heat bath the two spin system will approach a non-equilibrium steady state (NESS) that can be calculated in the golden rule approximation. The occupation probabilities of the NESS are shown not to be of Boltzmann type, with the exception of a single phase with infinite quasitemperature. The parameter space of the two spin Rabi model can be decomposed into eight phase domains such that the NESS probabilities possess discontinuous derivatives at the phase boundaries. The latter property is shown to hold also for more general periodically driven N -level systems.
We consider a spin s subjected to both a static and an orthogonally applied oscillating, circularly polarized magnetic field while being coupled to a heat bath and analytically determine the quasistationary distribution of its Floquet-state occupation probabilities for arbitrarily strong driving. This distribution is shown to be Boltzmannian with a quasitemperature which is different from the temperature of the bath and independent of the spin quantum number. We discover a remarkable formal analogy between the quasithermal magnetism of the nonequilibrium steady state of a driven ideal paramagnetic material and the usual thermal paramagnetism. Nonetheless, the response of such a material to the combined fields is predicted to show several unexpected features, even allowing one to turn a paramagnet into a diamagnet under strong driving. Thus, we argue that experimental measurements of this response may provide key paradigms for the emerging field of periodic thermodynamics.
Rabi oscillations and Floquet states are likely the most familiar concepts associated with a periodically time-varying Hamiltonian. Here, we present an exactly solvable model of a two-level system coupled to both a continuum and a classical field that varies sinusoidally with time, which sheds light on the relationship between the two problems. For a field of the rotating-wave-approximation form, results show that the dynamics of the two-level system can be mapped exactly onto that for a static field, if one shifts the energy separation between the two levels by an amount equal to ℏω, where ω is the frequency of the field and ℏ is Planck's constant. This correspondence allows one to view Rabi oscillations and Floquet states from the simpler perspective of their time-independent-problem equivalents. The comparison between the rigorous results and those from perturbation theory helps clarify some of the difficulties underlying textbook proofs of Fermi's golden rule, and the discussions on quantum decay and linear response theory.
We study the nonequilibrium dynamics of a periodically driven anisotropic Kondo impurity model. The periodic time dependence is introduced for a local magnetic field which couples to the impurity spin and also for an in-plane exchange interaction. We obtain the exact results on the time evolution for arbitrary periodic time dependence at the special point in the parameter space known as the Toulouse limit. We first consider a specific case where the local magnetic field is periodically switched on and off. When the driving period is much shorter than the inverse of the Kondo temperature, an intriguing oscillating behavior (resonance phenomenon) emerges in the time average of the impurity spin polarization with increasing the local magnetic field intensity. By taking the high-frequency limit of the external driving, we elucidate that the system recovers the translational invariance in time and can be described by a mixture of the zero-temperature and infinite-temperature properties. In certain cases, the system is governed by either zero-temperature or infinite-temperature properties and, therefore, can be properly described by the corresponding equilibrium state.
Driven many-body quantum systems where some parameter in the Hamiltonian is varied quasiperiodically in time may exhibit nonequilibrium steady states that are qualitatively different from their periodically driven counterparts. Here we consider a prototypical integrable spin system, the spin-1/21/21/2 transverse field Ising model in one dimension, in a pulsed magnetic field. The time dependence of the field is taken to be quasiperiodic by choosing the pulses to be of two types that alternate according to a Fibonacci sequence. We show that a steady state emerges after an exponentially long time when local properties (or equivalently, reduced density matrices of subsystems with size much smaller than the full system) are considered. We use the temporal evolution of certain coarse-grained quantities in momentum space to understand this nonequilibrium steady state in more detail and show that unlike the previously known cases, this steady state is neither described by a periodic generalized Gibbs ensemble nor by an infinite temperature ensemble. Finally, we study a toy problem with a single two-level system driven by a Fibonacci sequence; this problem shows how sensitive the nature of the final steady state is to the different parameters.
Rabi model result for Einstein's BBB coefficient: role of fundamental processes in nonequilibrium statistical mechanics
Starting from the Rabi Hamiltonian, which is useful in arriving at non-perturbative results within the rotating wave approximation, we have found Einstein's BBB coefficient to be time-dependent: B(t)∝∣J0(ωγt)∣B(t)\propto|J_0(\omega_\gamma t)|B(t)∝∣J0​(ωγ​t)∣ for a two-level system (atom or molecule) in thermal radiation field. Here ωγ\omega_\gammaωγ​ is the corresponding Rabi flopping (angular) frequency and J0J_0J0​ is the zeroth order Bessel function of the first kind. The resulting oscillations in the BBB coefficient---even for very small ωγ\omega_\gammaωγ​---drives the system away from thermodynamic equilibrium at any finite temperature contrary to Einstein's assumption. The time-dependent generalized BBB coefficient facilitates a path to go beyond Pauli's formalism of non-equilibrium statistical mechanics involving the quantum statistical Boltzmann (master) equation. In this context, we have obtained entropy production of the two-level system by revising Einstein's rate equations, while considering the AAA coefficient to be the original time-independent one and the BBB coefficient to be time-dependent.
The open quantum Rabi model describes a two-level system coupled to a harmonic oscillator. A Gaussian phase transition for the nonequilibrium steady states has been predicted when the bosonic mode is soft and subject to damping. We show that oscillator dephasing is a relevant perturbation, which leads to a non-Gaussian phase transition and an intriguing cascade of instabilities for kkk-th order bosonic operators, as well as a jump in the steady-state qubit polarization. For the soft-mode limit, the equations of motion form a closed hierarchy and spectral properties can be efficiently studied. To this purpose, we establish a fruitful connection to non-Hermitian Hamiltonians. The results for the phase diagram, stability boundaries, and relevant observables are based on mean-field analysis, exact diagonalization, perturbation theory, and Keldysh field theory.