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arXiv:1911.10481 · Journal of Physics A Mathematical and Theoretical

Lindblad approximation and spin relaxation in quantum electrodynamics

Laurent Amour, Jean Nourrigat

Published Apr 28, 2020• 4 citations
arXivHTMLPDF

Abstract

Abstract This article is concerned with the time evolution of spin observables for generalized spin boson models. This applies in particular to a model of nuclear magnetic resonance, namely a 1 2 -spin particle in a constant external magnetic field and in interaction with the quantized electromagnetic field (photons). We derive a Lindblad (or GKLS) type approximation of the spin dynamics initially in a photon vacuum state together with a precise control of the error coming from this approximation. The error term is bounded by g 2 where g is the coupling constant of the spin–photon interaction. The point here is the uniformity in time t > 0 of this error control.

DOI
10.1088/1751-8121/ab8e04

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Abstract This article is concerned with the time evolution of spin observables for generalized spin boson models. This applies in particular to a model of nuclear magnetic resonance, namely a 1 2 -spin particle in a constant external magnetic field and in interaction with the quantized electromagnetic field (photons). We derive a Lindblad (or GKLS) type approximation of the spin dynamics initially in a photon vacuum state together with a precise control of the error coming from this approximation. The error term is bounded by g 2 where g is the coupling constant of the spin–photon interaction. The point here is the uniformity in time t > 0 of this error control.
We are interested in this paper with the connection between the dynamics of a model related to Nuclear Magnetic Resonance (NMR) in Quantum Field Theory (QFT) with its classical counterpart known as the Maxwell-Bloch equations. The model in QFT is a model of Quantum Electrodynamics (QED) considering fixed spins interacting with the quantized electromagnetic field in an external constant magnetic field. This model is close to the common spin-boson model. The classical model goes back to F. Bloch [15] in 1946. Our goal is not only to study the derivation of the Maxwell-Bloch equations but to also establish a semiclassical asymptotic expansion of arbitrary high orders with control of the error terms of this standard nonlinear classical motion equations. This provides therefore quantum corrections of any order in powers of the semiclassical parameter of the Bloch equations. Besides, the asymptotic expansion for the photon number is also analyzed and a law describing the photon number time evolution is written down involving the radiation field polarization. Since the quantum photon state Hilbert space (radiation field) is infinite dimensional we are thus concerned in this article with the issue of semiclassical calculus in an infinite dimensional setting. In this regard, we are studying standard notions as Wick and anti-Wick quantizations, heat operator, Beals characterization theorem and compositions of symbols in the infinite dimensional context which can have their own interest.
In this article, we are interested in a spin model including the quantized electromagnetic field (photons). With this model of quantum electrodynamics (QED) related to nuclear magnetic resonance (NMR) we give explicit quantum radiative corrections of the time evolution for the spin observables, for the electric and magnetic fields observables and for the photon number observable. As a by-product, this underlines that Bloch equations are the semiclassical limit of the model in QED considered here. In addition, transition probabilities for the same model are investigated.
In this article, we consider fixed spin-1/2 particles interacting through the quantized electromagnetic field in a constant magnetic field. We give approximate evolutions of coherent states. This uses spins-photon classical Hamiltonian mechanics. These approximations enable to derive that the approximate average fields and spins follow Maxwell-Bloch equations with a current density coming from spins. In addition, we obain a law concerning the evolution of the approximate average number of photons. Next, we provide stationary points of the spins-photon Hamiltonian when the spin particles belong to an orthogonal plane to the constant magnetic field. This allows for the construction of quasimodes with spins colinear to the constant magnetic field. Finally, a quasimode with an arbitrary high accuracy is built up and its first order radiative correction is computed.
The coherent quantum dynamics of a single bosonic spin variable, subject to a constraint derived from the quantum spherical model of a ferromagnet, and coupled to an external heat bath, is studied through the Lindblad equation for the reduced density matrix. Closed systems of equations of motion for several quantum observables are derived and solved exactly. The relationship to the single-mode Dicke model from quantum optics is discussed. The analysis of the interplay of the quantum fluctuation and the dissipation and their influence on the relaxation of the time-dependent magnetisation leads to the distinction of qualitatively different regimes of weak and strong quantum couplings. Considering the model's behaviour in an external field as a simple mean-field approximation of the dynamics of a quantum spherical ferromagnet, the magnetic phase diagram appears to be re-entrant and presents a quantum analogue of well-established classical examples of fluctuation-induced order.
We investigate the controllability of quantum systems in two different settings: the standard "closed" setting, in which a quantum system is seen as isolated and the control problem is formulated on the Schrödinger equation; the open setting that describes a quantum system in interaction with a larger one, of which just qualitative parameters are known, by means of the Lindblad equation on states. In the context of closed systems we focus our attention to an interesting class of models, namely the spin-boson models. The latter describe the interaction between a 2-level quantum system and finitely many distinguished modes of a bosonic field. We discuss two prototypical examples, the Rabi model and the Jaynes-Cummings model, which despite their age are still very popular in several fields of quantum physics. Notably, in the context of cavity Quantum Electro Dynamics (C-QED) they provide an approximate yet accurate description of the dynamics of a 2-level atom in a resonant microwave cavity, as in recent experiments of S. Haroche. We investigate the controllability properties of these models, analyzing two different types of control operators acting on the bosonic part, corresponding -in the application to cavity QED- to an external electric and magnetic field, respectively. We review some recent results and prove the approximate controllability of the Jaynes-Cummings model with these controls. This result is based on a spectral analysis exploiting the non-resonances of the spectrum. As far as the relation between the Rabi and the Jaynes-Cummings Hamiltonians concerns, we treat the so called rotating wave approximation in a rigorous framework. We formulate the problem as an adiabatic limit in which the detuning frequency and the interaction strength parameter goes to zero, known as the weak-coupling regime. We prove that, under certain hypothesis on the ratio between the detuning and the coupling, the Jaynes-Cumming and the Rabi dynamics exhibit the same behaviour, more precisely the evolution operators they generate are close in norm. In the framework of open quantum systems we investigate the controllability of the Lindblad equation. We consider a control acting adiabatically on the internal part of the system, which we see as a degree of freedom that can be used to contrast the action of the environment. The adiabatic action of the control is chosen to produce a robust transition. We prove, in the prototype case of a two-level system, that the system approach a set of equilibrium points determined by the environment, i.e. the parameters that specify the Lindblad operator. On that set the system can be adiabatically steered choosing a suitable control. The analysis is based on the application of geometrical singular perturbation methods.
Controllable, partially isolated few-level systems in semiconductors have recently gained multidisciplinary attention due to their widespread nanoscale sensing and quantum technology applications. Quantitative simulation of the dynamics and related applications of such systems is a challenging theoretical task that requires faithful description not only of the few-level systems but also their local environments. Here, we develop a method that can describe relevant relaxation processes induced by a dilute bath of nuclear and electron spins. The method utilizes an extended Lindblad equation in the framework of cluster approximation of a central spin system. We demonstrate that the proposed method can accurately describe T1{\mathrm{T}}_{1}T1​ time of an exemplary solid-state point-defect qubit system, in particular, the nitrogen-vacancy (NV) center in diamond, at various magnetic fields and strain.