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arXiv:1911.04342 · Physical Review A

Rydberg-positronium velocity and self-ionization studies in a 1T magnetic field and cryogenic environment

M. Antonello, Alexander S. Belov, G. Bonomi, Roberto Sennen Brusa, M. Caccia, A. Camper, R. Caravita, F. Castelli, D. Comparat, Giovanni Consolati, L. Di Noto, M. Doser, Mattia Fanì, R. Ferragut, J. Fesel, S. Gerber, A. Gligorova, L. T. Glöggler, F. Guatieri, S. Haider, Alexander Hinterberger, O. Khalidova, D. Krasnický, Vittorio Lagomarsino, C. Malbrunot, S. Mariazzi, V. Matveev, S. R. Müller, G. Nebbia, P. Nédélec, L. Nowak, Markus K. Oberthaler, Emmanuel Oswald, Davide Pagano, Luca Penasa, V. Petráček, F. Prelz, B. Rienäcker, Ole Myren Rohne, Alberto Rotondi, H. Sandaker, R. Santoro, G. Testera, Ingmari C. Tietje, T. Wolz, Christian Zimmer, Nicola Zurlo

Published Jul 2, 2020• 22 citations
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Abstract

We characterized the pulsed Rydberg-positronium production inside the Antimatter Experiment: Gravity, Interferometry, Spectroscopy ($\mathrm{AE}\overline{\text{g}}\mathrm{IS}$) apparatus in view of antihydrogen formation by means of a charge exchange reaction between cold antiprotons and slow Rydberg-positronium atoms. Velocity measurements on the positronium along two axes in a cryogenic environment ($\ensuremath{\approx}10\phantom{\rule{0.16em}{0ex}}\mathrm{K}$) and in $1\phantom{\rule{0.16em}{0ex}}\mathrm{T}$ magnetic field were performed. The velocimetry was done by microchannel-plate (MCP) imaging of a photoionized positronium previously excited to the $n=3$ state. One direction of velocity was measured via Doppler scan of this $n=3$ line, another direction perpendicular to the former by delaying the exciting laser pulses in a time-of-flight measurement. Self-ionization in the magnetic field due to the motional Stark effect was also quantified by using the same MCP-imaging technique for Rydberg positronium with an effective principal quantum number ${n}_{\mathrm{eff}}$ ranging between 14 and 22. We conclude with a discussion about the optimization of our experimental parameters for creating Rydberg positronium in preparation for an efficient pulsed production of antihydrogen.

DOI
10.1103/physreva.102.013101

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We characterized the pulsed Rydberg-positronium production inside the Antimatter Experiment: Gravity, Interferometry, Spectroscopy (AEg‾IS\mathrm{AE}\overline{\text{g}}\mathrm{IS}AEg​IS) apparatus in view of antihydrogen formation by means of a charge exchange reaction between cold antiprotons and slow Rydberg-positronium atoms. Velocity measurements on the positronium along two axes in a cryogenic environment (\ensuremath≈10K\ensuremath{\approx}10\phantom{\rule{0.16em}{0ex}}\mathrm{K}\ensuremath≈10K) and in 1T1\phantom{\rule{0.16em}{0ex}}\mathrm{T}1T magnetic field were performed. The velocimetry was done by microchannel-plate (MCP) imaging of a photoionized positronium previously excited to the n=3n=3n=3 state. One direction of velocity was measured via Doppler scan of this n=3n=3n=3 line, another direction perpendicular to the former by delaying the exciting laser pulses in a time-of-flight measurement. Self-ionization in the magnetic field due to the motional Stark effect was also quantified by using the same MCP-imaging technique for Rydberg positronium with an effective principal quantum number neff{n}_{\mathrm{eff}}neff​ ranging between 14 and 22. We conclude with a discussion about the optimization of our experimental parameters for creating Rydberg positronium in preparation for an efficient pulsed production of antihydrogen.
This work reports on experiments in which antihydrogen atoms have been produced in cryogenic Penning traps from antiproton and positron plasmas by two different methods and on experiments that have been carried out subsequently in order to investigate the antihydrogen atoms. By the first method antihydrogen atoms have been formed during the process of positron cooling of antiprotons in so called nested Penning traps and detected via a field ionization method. A linear dependence of the number of detected antihydrogen atoms on the number of positrons has been found. A measurement of the state distribution has revealed that the antihydrogen atoms are formed in highly excited states. This suggests along with the high production rate that the antihydrogen atoms are formed by three-body recombination processes and subsequent collisional deexcitations. However current theory cannot yet account for the measured state distribution. Typical radii of the detected antihydrogen atoms lie in the range between 0.4 µm and 0.15 µm. The deepest bound antihydrogen atoms have radii below 0.1 µm. Antihydrogen atoms with that size have chaotic positron orbits so that for the first time antihydrogen atoms have been detected that cannot be described by the GCA-model. The kinetic energy of the weakest bound antihydrogen atoms has been measured to about 200 meV, which corresponds to an antihydrogen velocity of approximately 6200 m/s. A simple model suggests that these atoms are formed from only one deexcitation collision and methods that might lead to a decrease of the antihydrogen velocity are presented. By the second method antihydrogen atoms have been synthesized in charge-exchange processes. Lasers are used to produce a Rydberg cesium beam within the cryogenic Penning trap that collides with trapped positrons so that Rydberg positronium atoms are formed via charge-exchange reactions. Due to their charge neutrality the Rydberg positronium atoms are free to leave the positron trapping region. The Rydberg positronium atoms that collide with nearby stored antiprotons form antihydrogen atoms in charge-exchange reactions. So far, 14 +/- 4 antihydrogen atoms have been detected background-free via a field-ionization method. The antihydrogen atoms produced via the two-step charge-exchange mechanism are expected to have a temperature of 4.2 K, the temperature of the antiprotons from which they are formed. A method is proposed by which the antihydrogen temperature can be determined with an accuracy of better than 1 K from a measurement of the time delay between antihydrogen annihilation events and the laser pulse that initiates the antihydrogen production via the production of Rydberg cesium atoms. First experiments have been carried out during the last days of the 2004 beam time, but the number of detected antihydrogen annihilations has been too low for a determination of the antihydrogen temperature. Trapped antiprotons have been directly exposed to laser light delivered by a Titanium:Sapphire laser in order to investigate if the laser light causes any loss on the trapped antiprotons. Experiments have shown that no extra loss occurs for laser powers of less than 590 mW. This is an important result against the background of the future plan to confine antihydrogen atoms in a combined Penning-Ioffe trap and then to carry out laser spectroscopy on these atoms, since it reveals that laser light does not cause an increase of the pressure in the trapping region to the extend that annihilations with the background gas become noticeable. The ATRAP Collaboration plans to precisely investigate antihydrogen atoms. The ultimate goal is to test the CPT-theorem by a high precision measurement of the 1S-2S transition of antihydrogen and a comparison with the precisely known value of the corresponding transition in hydrogen. This thesis presents the achievement of the first step towards this challenging goal: the production of cold antihydrogen itself.
The antihydrogen formation by charge exchange between cold antiprotons and Rydberg positronium Ps∗{\text{P}}_{s}^{*}Ps∗​ is studied by using the classical trajectory Monte Carlo method. In the absence of external magnetic field the cross section scaled by the fourth power of the Ps∗{\text{P}}_{s}^{*}Ps∗​ principal quantum number nPs{n}_{{\text{P}}_{s}}nPs​​ shows a universal behavior as a function of the ratio kv{k}_{v}kv​ between the velocity of the Ps{\text{P}}_{s}Ps​ center of mass and that of the positron in the classical circular orbit. At low velocity, below about ${k}_{v}\ensuremath{\simeq}0.2--0.3$, we show for Rydberg positronium that the cross section increases as 1/kv21/{k}_{v}^{2}1/kv2​ or, in an equivalent way, as 1/EPscm1/{E}_{{\text{P}}_{s}}^{\text{cm}}1/EPs​cm​ with EPscm{E}_{{\text{P}}_{s}}^{\text{cm}}EPs​cm​ being the Ps∗{\text{P}}_{s}^{*}Ps∗​ center-of-mass energy. In this regime the distribution of the principal quantum number of the antihydrogen state is narrow and it shows a peak at about 2nPs\sqrt{2}{n}_{{\text{P}}_{s}}2​nPs​​ while at higher kv{k}_{v}kv​ values a broad distribution of antihydrogen states is produced. The study of the collision process in the presence of moderate magnetic field (0.5--2 T) shows that there is an experimentally interesting region of kv{k}_{v}kv​ with the cross section slightly higher than that in the absence of field. However the presence of a magnetic field changes significantly the cross section behavior as a function of kv{k}_{v}kv​, especially at low velocities, where reductions of the cross sections and deviations from the 1/kv21/{k}_{v}^{2}1/kv2​ (1/EPscm1/{E}_{{\text{P}}_{s}}^{\text{cm}}1/EPs​cm​) are observed. Our calculations show a dependance of the cross section upon the angle between the magnetic field and the flight direction of the incoming Ps∗{\text{P}}_{s}^{*}Ps∗​.
Antihydrogen production by charge exchange reaction between positronium (Ps) atoms and antiprotons requires an efficient excitation of Ps atoms up to high-nnn levels (Rydberg levels). In this study it is assumed that a Ps cloud is produced within a relatively strong uniform magnetic field (1T)(1\phantom{\rule{0.3em}{0ex}}\mathrm{T})(1T) and with a relatively high temperature (100K)(100\phantom{\rule{0.3em}{0ex}}\mathrm{K})(100K). Consequently, the structure of energy levels are deeply modified by Zeeman and motional Stark effects. A two-step laser light excitation, the first one from ground to n=3n=3n=3 and the second from this level to a Rydberg level, is proposed and the physics of the problem is discussed. We derive a simple formula giving the absorption probability with substantially incoherent laser pulses. A 30% population deposition in high-nnn states can be reached with feasible lasers suitably tailored in power and spectral bandwidth.
Cold antihydrogen atoms are a powerful tool to probe the validity of fundamental physics laws, and it's clear that colder atoms, generally speaking, allow an increased level of precision. After the first production of cold antihydrogen (Hˉ\bar{H}Hˉ) in 2002, experimental efforts have progressed continuously (trapping, beam formation, spectroscopy), with competitive results already achieved by adapting to cold antiatoms techniques previously well developed for ordinary atoms. Unfortunately, the number of Hˉ\bar{H}Hˉ atoms that can be produced in dedicated experiments is many orders of magnitude smaller than available hydrogen atoms, which are at hand in large amount, so the development of novel techniques that allow the production of Hˉ\bar{H}Hˉ with well defined conditions (and possibly control its formation time and energy levels) is essential to improve the sensitivity of the methods applied by the different experiments. We present here the first experimental results concerning the production of Hˉ\bar{H}Hˉ in a pulsed mode where the time when 90\% of the atoms are produced is known with an uncertainty of around 250~ns. The pulsed Hˉ\bar{H}Hˉ source is generated by the charge-exchange reaction between Rydberg positronium atoms (PsPsPs) and trapped antiprotons (pˉ\bar{p}pˉ​), cooled and manipulated in an electromagnetic trap: pˉ+Ps∗→Hˉ∗+e− \bar{ p}+Ps^* \rightarrow \bar{H}^* + e^- pˉ​+Ps∗→Hˉ∗+e− where Rydberg positronium atoms, in turn, are produced through the implantation of a pulsed positron beam into a mesoporous silica target, and are excited by two subsequent laser pulses, the first to n=3n=3n=3, the second to the needed Rydberg level (n≃17n \simeq 17n≃17). The pulsed production allows the control of the antihydrogen temperature, and facilitates the tunability of the Rydberg states, their de-excitation by pulsed lasers and the manipulation through electric field gradients. In fact, the production of pulsed antihydrogen is a major milestone in the AEgIS experiment to perform direct measurements of the validity of the Weak Equivalence Principle for antimatter.
The production of long-lived Rydberg positronium (Ps) and correction for Doppler shifts in the excitation laser frequencies are crucial elements of proposed measurements of the gravitational freefall of antimatter and for precision measurements of the optical spectrum of Ps. Using a two-step optical transition via 2P2P2P levels, we have prepared Ps atoms in Rydberg states up to the term limit. The spectra are corrected for the first-order Doppler shift using measured velocities, and the Balmer transitions are resolved for $15\ensuremath{\le}n\ensuremath{\le}31$. The excitation signal amplitude begins to decrease for n>50n>50n>50, consistent with the onset of motional electric field ionization in the 3.5-mT magnetic field at the Ps formation target.
Abstract Antihydrogen atoms with K or sub-K temperature are a powerful tool to precisely probe the validity of fundamental physics laws and the design of highly sensitive experiments needs antihydrogen with controllable and well defined conditions. We present here experimental results on the production of antihydrogen in a pulsed mode in which the time when 90% of the atoms are produced is known with an uncertainty of ~250 ns. The pulsed source is generated by the charge-exchange reaction between Rydberg positronium atoms—produced via the injection of a pulsed positron beam into a nanochanneled Si target, and excited by laser pulses—and antiprotons, trapped, cooled and manipulated in electromagnetic traps. The pulsed production enables the control of the antihydrogen temperature, the tunability of the Rydberg states, their de-excitation by pulsed lasers and the manipulation through electric field gradients. The production of pulsed antihydrogen is a major landmark in the AE gˉ\bar{g}gˉ​ ḡ IS experiment to perform direct measurements of the validity of the Weak Equivalence Principle for antimatter.