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arXiv:1608.02785 · Physical Review A

Cross section for Rydberg antihydrogen production via charge exchange between Rydberg positroniums and antiprotons in a magnetic field

D. Krasnický, R. Caravita, C. Canali, G. Testera

Published Aug 30, 2016• 43 citations
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Abstract

The antihydrogen formation by charge exchange between cold antiprotons and Rydberg positronium ${\text{P}}_{s}^{*}$ is studied by using the classical trajectory Monte Carlo method. In the absence of external magnetic field the cross section scaled by the fourth power of the ${\text{P}}_{s}^{*}$ principal quantum number ${n}_{{\text{P}}_{s}}$ shows a universal behavior as a function of the ratio ${k}_{v}$ between the velocity of the ${\text{P}}_{s}$ center of mass and that of the positron in the classical circular orbit. At low velocity, below about ${k}_{v}\ensuremath{\simeq}0.2--0.3$, we show for Rydberg positronium that the cross section increases as $1/{k}_{v}^{2}$ or, in an equivalent way, as $1/{E}_{{\text{P}}_{s}}^{\text{cm}}$ with ${E}_{{\text{P}}_{s}}^{\text{cm}}$ being the ${\text{P}}_{s}^{*}$ center-of-mass energy. In this regime the distribution of the principal quantum number of the antihydrogen state is narrow and it shows a peak at about $\sqrt{2}{n}_{{\text{P}}_{s}}$ while at higher ${k}_{v}$ values a broad distribution of antihydrogen states is produced. The study of the collision process in the presence of moderate magnetic field (0.5--2 T) shows that there is an experimentally interesting region of ${k}_{v}$ with the cross section slightly higher than that in the absence of field. However the presence of a magnetic field changes significantly the cross section behavior as a function of ${k}_{v}$, especially at low velocities, where reductions of the cross sections and deviations from the $1/{k}_{v}^{2}$ ($1/{E}_{{\text{P}}_{s}}^{\text{cm}}$) are observed. Our calculations show a dependance of the cross section upon the angle between the magnetic field and the flight direction of the incoming ${\text{P}}_{s}^{*}$.

DOI
10.1103/physreva.94.022714

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An efficient method for production of cold antihydrogen $(\mathrm{H}\ifmmode\bar\else\textasciimacron\fi{})$ is proposed. Alkali-metal atoms laser excited to a Rydberg state are charge exchanged with cold trapped positrons, producing Rydberg states of positronium. In a second Rydberg-state charge exchange, the positronium atoms give up their Rydberg positrons to cold trapped antiprotons, producing Rydberg states of $\mathrm{H}\ifmmode\bar\else\textasciimacron\fi{}$. These $\mathrm{H}\ifmmode\bar\else\textasciimacron\fi{}$ atoms soon decay down to the ground state, and, because they are cold, could be trapped in a magnetic trap. The efficiency of the process results from the extremely large cross sections for Rydberg charge exchange. Classical trajectory Monte Carlo calculations indicate an $\mathrm{H}\ifmmode\bar\else\textasciimacron\fi{}$ instantaneous production rate of 106/{}^{6}/6/s.
The aim of this work is to investigate the dynamics of collisions between ions and Rydberg atoms by using the Classical Trajectory Monte Carlo (CTMC) method. The study is started by collisions with oriented elliptical Rydberg atom, is then continued to collisions involving hydrogen Rydberg target in an external magnetic field in the l-mixing regime, and later arrives at antihydrogen formation in an external magnetic field where Rydberg positronium is taken as target.\nThe CTMC method has been applied in the study. For different targets, the CTMC method had to be adjusted and reconstructed to properly create the initial target state for the quasi-separable one-body initial system (hydrogen target) and the two-body initial system (positronium target). Charge exchange and ionization cross sections are calculated under special consideration of different initial target states.\nThe velocity matching phenomenon and Thomas capture which appears in the upstream-downstream asymmetry are found in ion-oriented elliptical Rydberg atom collisions, reflecting the important roles of the initial electron spatial and momentum distributions. By increasing the projectile charge, the distortion of the initial states caused by the strong perturbation of approaching projectile induces pronounced changes in the momentum distribution.\nIn the collisions involving hydrogen Rydberg atoms in a magnetic field, a cross section reduction in case of an increasing magnetic field is found for multiply charged projectiles. The structure effect due to the influence of the magnetic field on the initial state distribution results in different capture cross sections for two characterized, kmax and kmin, states. The velocity matching phenomenon as well as the effect of multiply charged projectile ion are observed in the collisions.\nFurthermore, antihydrogen formation in a magnetic field has been studied. Rydberg positroniums are assumed to be the target atoms, colliding with antiprotons. The initial target positronium state is carefully constructed by means of a newly introduced conserved operator, the pseudomomentum K. Similar properties as in the previous hydrogen target atom case were investigated. It is found that the existence of the magnetic field changes the spatial distribution of positronium to irregular motion. By increasing the magnetic field, it induces a decrease of the resulting capture cross sections (i.e. the antihydrogen formation). Thomas capture which happens in the collision plane in the field-free case is foiled. A smaller positronium binding energy and a larger geometrical extension of the target positronium atom yield a larger capture cross section.
This work reports on experiments in which antihydrogen atoms have been produced in cryogenic Penning traps from antiproton and positron plasmas by two different methods and on experiments that have been carried out subsequently in order to investigate the antihydrogen atoms. By the first method antihydrogen atoms have been formed during the process of positron cooling of antiprotons in so called nested Penning traps and detected via a field ionization method. A linear dependence of the number of detected antihydrogen atoms on the number of positrons has been found. A measurement of the state distribution has revealed that the antihydrogen atoms are formed in highly excited states. This suggests along with the high production rate that the antihydrogen atoms are formed by three-body recombination processes and subsequent collisional deexcitations. However current theory cannot yet account for the measured state distribution. Typical radii of the detected antihydrogen atoms lie in the range between 0.4 µm and 0.15 µm. The deepest bound antihydrogen atoms have radii below 0.1 µm. Antihydrogen atoms with that size have chaotic positron orbits so that for the first time antihydrogen atoms have been detected that cannot be described by the GCA-model. The kinetic energy of the weakest bound antihydrogen atoms has been measured to about 200 meV, which corresponds to an antihydrogen velocity of approximately 6200 m/s. A simple model suggests that these atoms are formed from only one deexcitation collision and methods that might lead to a decrease of the antihydrogen velocity are presented. By the second method antihydrogen atoms have been synthesized in charge-exchange processes. Lasers are used to produce a Rydberg cesium beam within the cryogenic Penning trap that collides with trapped positrons so that Rydberg positronium atoms are formed via charge-exchange reactions. Due to their charge neutrality the Rydberg positronium atoms are free to leave the positron trapping region. The Rydberg positronium atoms that collide with nearby stored antiprotons form antihydrogen atoms in charge-exchange reactions. So far, 14 +/- 4 antihydrogen atoms have been detected background-free via a field-ionization method. The antihydrogen atoms produced via the two-step charge-exchange mechanism are expected to have a temperature of 4.2 K, the temperature of the antiprotons from which they are formed. A method is proposed by which the antihydrogen temperature can be determined with an accuracy of better than 1 K from a measurement of the time delay between antihydrogen annihilation events and the laser pulse that initiates the antihydrogen production via the production of Rydberg cesium atoms. First experiments have been carried out during the last days of the 2004 beam time, but the number of detected antihydrogen annihilations has been too low for a determination of the antihydrogen temperature. Trapped antiprotons have been directly exposed to laser light delivered by a Titanium:Sapphire laser in order to investigate if the laser light causes any loss on the trapped antiprotons. Experiments have shown that no extra loss occurs for laser powers of less than 590 mW. This is an important result against the background of the future plan to confine antihydrogen atoms in a combined Penning-Ioffe trap and then to carry out laser spectroscopy on these atoms, since it reveals that laser light does not cause an increase of the pressure in the trapping region to the extend that annihilations with the background gas become noticeable. The ATRAP Collaboration plans to precisely investigate antihydrogen atoms. The ultimate goal is to test the CPT-theorem by a high precision measurement of the 1S-2S transition of antihydrogen and a comparison with the precisely known value of the corresponding transition in hydrogen. This thesis presents the achievement of the first step towards this challenging goal: the production of cold antihydrogen itself.
Abstract We compare classical and quantum predictions of the cross section for anti-hydrogen formation by charge exchange between Rydberg positronium and antiprotons as a function of the positronium energy. We show that these two highly different approaches furnish the same scaling law with the principal quantum number of positronium n Ps and numerical values in agreement within some tens of percent for n Ps ≥ 3 and down to very low collision energy of tens of μ eV. We discuss these results in the context of a recently claimed hypothesis of quantum suppression of the reaction driven by supposedly different scaling law of classical and quantum predictions. Finally we underline how the basic agreement between classical and quantum results enforces the reliability of the classical calculations that, presently, are the only ones able to obtain the cross section for positronium initially in high Rydberg states and in the presence of external electric and magnetic fields.
We characterized the pulsed Rydberg-positronium production inside the Antimatter Experiment: Gravity, Interferometry, Spectroscopy (AEg‾IS\mathrm{AE}\overline{\text{g}}\mathrm{IS}AEg​IS) apparatus in view of antihydrogen formation by means of a charge exchange reaction between cold antiprotons and slow Rydberg-positronium atoms. Velocity measurements on the positronium along two axes in a cryogenic environment ($\ensuremath{\approx}10\phantom{\rule{0.16em}{0ex}}\mathrm{K}$) and in 1T1\phantom{\rule{0.16em}{0ex}}\mathrm{T}1T magnetic field were performed. The velocimetry was done by microchannel-plate (MCP) imaging of a photoionized positronium previously excited to the n=3n=3n=3 state. One direction of velocity was measured via Doppler scan of this n=3n=3n=3 line, another direction perpendicular to the former by delaying the exciting laser pulses in a time-of-flight measurement. Self-ionization in the magnetic field due to the motional Stark effect was also quantified by using the same MCP-imaging technique for Rydberg positronium with an effective principal quantum number neff{n}_{\mathrm{eff}}neff​ ranging between 14 and 22. We conclude with a discussion about the optimization of our experimental parameters for creating Rydberg positronium in preparation for an efficient pulsed production of antihydrogen.