As in between liquid and crystal phases lies a nematic liquid crystal, which breaks rotation with preservation of translation symmetry, there is a nematic superfluid phase bridging a superfluid and a supersolid. The nematic order also emerges in interacting electrons and has been found to largely intertwine with multiorbital correlation in high-temperature superconductivity, where Ising nematicity arises from a four-fold rotation symmetry C_{4} broken down to C_{2}. Here, we report an observation of a three-state (Z_{3}) quantum nematic order, dubbed "Potts-nematicity", in a system of cold atoms loaded in an excited band of a hexagonal optical lattice described by an sp^{2}-orbital hybridized model. This Potts-nematic quantum state spontaneously breaks a three-fold rotation symmetry of the lattice, qualitatively distinct from the Ising nematicity. Our field theory analysis shows that the Potts-nematic order is stabilized by intricate renormalization effects enabled by strong interorbital mixing present in the hexagonal lattice. This discovery paves a way to investigate quantum vestigial orders in multiorbital atomic superfluids.
As in between liquid and crystal phases lies a nematic liquid crystal, which breaks rotation with preservation of translation symmetry, there is a nematic superfluid phase bridging a superfluid and a supersolid. The nematic order also emerges in interacting electrons and has been found to largely intertwine with multiorbital correlation in high-temperature superconductivity, where Ising nematicity arises from a four-fold rotation symmetry C_{4} broken down to C_{2}. Here, we report an observation of a three-state (Z_{3}) quantum nematic order, dubbed "Potts-nematicity", in a system of cold atoms loaded in an excited band of a hexagonal optical lattice described by an sp^{2}-orbital hybridized model. This Potts-nematic quantum state spontaneously breaks a three-fold rotation symmetry of the lattice, qualitatively distinct from the Ising nematicity. Our field theory analysis shows that the Potts-nematic order is stabilized by intricate renormalization effects enabled by strong interorbital mixing present in the hexagonal lattice. This discovery paves a way to investigate quantum vestigial orders in multiorbital atomic superfluids.
Electronic liquid crystals are ubiquitous in strongly correlated matter, and often seen in multiorbital materials exhibiting non-Fermi-liquid transport. The authors propose here and analyze a three-orbital Sachdev-Ye-Kitaev model that hosts a uniform solution corresponding to a \ensuremath{\mathbb{Z}}3 Potts nematic. In the atomic limit, this model displays an orbital-selective non-Fermi liquid down to T=0. On the triangular and cubic lattice, this evolves into a nematic with highly anisotropic transport, reminiscent of dynamical mean field theory studies of multiorbital Hubbard models.
"This thesis is devoted to the investigation of the quantum liquid crystal phases in strongly correlated electronic systems. Such phases are characterized by their partially broken spatial symmetries and are observed in various strongly correlated systems as being summarized in Chapter 1. In quantum liquid crystal phases formed by fermions, behaviors beyond Landau's theory of the Fermi liquids appear naturally, signed by the absence of well-defined quasiparticle excitations. Although quantum liquid crystal phases often involve strong-coupling physics, the associated symmetry analysis can often be carried out also in a relatively weak coupling regime and this is the main approach taken in this thesis. Two different quantum liquid crystal phases, the nematic state and the smectic state, are studied in Chapters 2 and 3 respectively, by investigating various instabilities of a Landau Fermi liquid. A nematic phase is a state that breaks the rotational symmetry spontaneously but preserves the translational symmetries. It can be reached by the Pomeranchuk instability of a Landau Fermi liquid. The Pomeranchuk instability in the charge (spin-singlet) sector of a Fermi liquid was studied previously within a random phase approximation and by a high-dimensional bosonization method. In Chapter 2, we concentrate on the Pomeranchuk instability in the spin-triplet sector, and two different classes of ordered phases are discovered, dubbed the a and ,8-phases by analogy to the superfluid 3He-A and B-phases. The Fermi surfaces in the a-phases exhibit spontaneous anisotropic distortions, while in the ,8-phases the Fermi surfaces remain circular or spherical with topologically non-trivial spin configurations in momentum space. The behaviors of the low energy bosonic excitations are studied both in the order phases (a and .B) and at the quantum critical point separating the ordered phases from the Fermi liquid phase. In Chapter 3, the smectic phase and the quantum phase transition between a metallic nematic state and a metallic smectic phase are investigated using the random phase approximation, by considering the formation of a unidirectional charge density wave in an electronic nematic state. The associated quantum critical point is investigated within the Hertz-Millis approach. Non-Fermi liquid behaviors are discovered both at the quantum phase transition and in the smectic ordered phase. The theory we studied here provides a simple description for the so-called ""fluctuating stripe"" phase in cuprates. Similar to its classical counterpart, the phase transition between the nematic and smectic phases are described by a ""gauge-like"" theory as required by the rotational invariance in close analogy with the McMillan-deGennes theory of the smectic-nematic phase transition in classical liquid crystals. However, unlike the classical McMillandeGennes theory, in which the coupling between the ""gauge-like"" nematic fluctuations and the ""matter-like"" smectic fields is relevant, in the sense of renormalization group, this coupling is irrelevant at the quantum phase transition. This property enables the study of low energy fluctuations and the fate of fermions near this quantum critical point. In Chapter 4, quantum liquid crystal phases with a broken time-reversal symmetry are investigated. We start by studying the general scenario of timereversal symmetry breaking phases in the absence of magnetic ordering in systems with long-lived low-energy fermionic quasiparticle excitations in two dimensions. Using a Berry phase approach, we classified possible time-reversal symmetry breaking phases by the accompanying spatial symmetry breaking patterns. Two of the simplest situations are referred to as the type I state, which breaks simultaneously the space-inversion symmetry and the time-reversal symmetry, and the type I I state, in which the chiral symmetry is broken in addition to the breaking of the time-reversal symmetry. Although the starting point is general and has little relation with the quantum liquid crystal phases, both type I and type II states defined above are realized by (generalized) Pomeranchuk instabilities. In fact , a type I I state is usually a nematic state which also breaks the time-reversal symmetry. Interestingly, the type II states also shows spontaneously generated Hall effect even in the absence of a magnetic field, which is known as the spontaneous anomalous Hall effect. In Chapter 5, we investigate the stability of a quadratic band-crossing point in two-dimensional fermionic systems that provide an explicit example, within well controlled approximations, for the nematic ordering discussed in Chapter 2 and spontaneous anomalous Hall effect discussed in Chapter 4. At the non-interacting level, we show that a quadratic band-crossing point exists and is topologically stable when the Berry flux of this crossing point is ±27r and the point symmetry group at this point has either fourfold or sixfold rotational symmetries. Strikingly, we find that this would-be topologically stable quadratic band-crossing is marginally unstable against short-range interactions: a quadratic band-crossing point in two dimensions is unstable against shortrange repulsion, no matter how weak! Four ordered phases are found in this system, the quantum anomalous Hall state, the quantum spin Hall phase, the nematic phase, and the nematic-spin-nematic phase."
The problem of interacting bosons in frustrated lattices is an intricate one due to the absence of a unique minimum in the single-particle dispersion where macroscopic number of bosons can condense. Here, we consider a family of tight-binding models with macroscopically degenerate lowest energy bands, separated from other bands by a gap. We predict the formation of exotic states that spontaneously break rotational symmetry at relatively low filling. These states belong to three nematic phases: Wigner crystal, supersolid, and superfluid. The Wigner crystal phase is established exactly at low filling. Supersolid and superfluid phases, at larger filling, are obtained by making use of a projection onto the flat band, construction of an appropriate Wannier basis, and subsequent mean-field treatment. The nematic superfluid that we predict is uniform in real space but has an anisotropic momentum distribution, providing a novel scenario for Bose condensation with an additional nematic order. Our findings open up a promising direction of studying microscopic quantum liquid crystalline phases of bosons.
Orbital selective order and Z3 Potts nematicity from a non-Fermi liquid
Motivated by systems where a high temperature non-Fermi liquid gives way to low temperature Z3 Potts nematic order, we studied a three-orbital Sachdev-Ye-Kitaev (SYK) model in the large-N limit. In the single-site limit, this model exhibits a spontaneous orbital-selective transition which preserves average particle-hole symmetry, with two orbitals becoming insulators while the third orbital remains a non-Fermi liquid down to zero temperature. We extend this study to lattice models of three-orbital SYK dots, exploring uniform symmetry broken states on the triangular and cubic lattices. At high temperature, these lattice models exhibit an isotropic non-Fermi liquid metal phase. On the three-dimensional (3D) cubic lattice, the low temperature uniform Z3 nematic state corresponds to an orbital selective layered state which preserves particle-hole symmetry at small hopping and spontaneously breaks the particle-hole symmetry at large hopping. Over a wide range of temperature, the transport in this layered state shows metallic in-plane resistivity but insulating out-of-plane resistivity. On the 2D triangular lattice, the low temperature state with uniform orbital order is also a correlated Z3 nematic with orbital-selective transport but it remains metallic in both principal directions. We discuss a Landau theory with Z3 clock terms which captures salient features of the phase diagram and nematic order in all these models. We also present results on the approximate wavevector dependent orbital susceptibility of the isotropic non-Fermi liquid states.
Frustration in quantum spin systems promote a variety of novel quantum phases. An important example is the frustrated spin-1 model on the square lattice with the nearest-neighbor bilinear (J1) and biquadratic (K1) interactions. We provide strong evidence for a nematic spin liquid phase in a range of K1/J1 near the SU(3)-symmetric point (J1=K1), based on the linear flavor-wave theory and extensive density matrix renormalization group calculation. This phase displays no spin dipolar or quadrupolar order, preserves translational symmetry but spontaneously breaks C4 lattice rotational symmetry, and possesses fluctuations peaked at the wave vector $(\ensuremath{\pi},2\ensuremath{\pi}/3)$. The spin excitation gap drops rapidly with system size and appears to be gapless, and the nematic order is attributed to the dominant $(\ensuremath{\pi},2\ensuremath{\pi}/3)$ fluctuations. Our results provide a novel mechanism for electronic nematic order and, more generally, open up a new avenue to explore frustration-induced exotic ground states.
Strong interaction between fermions may lead to a novel quantum ground state where the rotational symmetry is spontaneously broken while the translational symmetry is still preserved. Such a 'nematic' Fermi liquid has a spontaneously deformed Fermi surface and supports a gapless Goldstone mode associated with the broken rotational symmetry. We consider a nematic Fermi liquid of fermions carrying two internal quantum numbers that, for example, may represent the layer degree of freedom of a bilayer system. It is found that the effective interaction mediated by a collective mode gives rise to a pairing instability of the underlying fermions under certain conditions, leading to the conclusion that the nematic order could be useful for superconductivity.