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arXiv:1910.05459 · Physical Review Letters

Large Momentum Transfer Clock Atom Interferometry on the 689 nm Intercombination Line of Strontium

Jan Rudolph, Thomas F. Wilkason, Megan K. T. Nantel, Hunter Swan, Connor M. Holland, Yijun Jiang, Benjamin E. Garber, Samuel P. Carman, Jason M. Hogan

Published Feb 28, 2020• 126 citations
arXivHTMLPDF

Abstract

We report the first realization of large momentum transfer (LMT) clock atom interferometry. Using single-photon interactions on the strontium ^{1}S_{0}-^{3}P_{1} transition, we demonstrate Mach-Zehnder interferometers with state-of-the-art momentum separation of up to 141 ℏk and gradiometers of up to 81 ℏk. Moreover, we circumvent excited state decay limitations and extend the gradiometer duration to 50 times the excited state lifetime. Because of the broad velocity acceptance of the interferometry pulses, all experiments are performed with laser-cooled atoms at a temperature of 3 μK. This work has applications in high-precision inertial sensing and paves the way for LMT-enhanced clock atom interferometry on even narrower transitions, a key ingredient in proposals for gravitational wave detection and dark matter searches.

DOI
10.1103/physrevlett.124.083604

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We report the first realization of large momentum transfer (LMT) clock atom interferometry. Using single-photon interactions on the strontium ^{1}S_{0}-^{3}P_{1} transition, we demonstrate Mach-Zehnder interferometers with state-of-the-art momentum separation of up to 141 ℏk and gradiometers of up to 81 ℏk. Moreover, we circumvent excited state decay limitations and extend the gradiometer duration to 50 times the excited state lifetime. Because of the broad velocity acceptance of the interferometry pulses, all experiments are performed with laser-cooled atoms at a temperature of 3 μK. This work has applications in high-precision inertial sensing and paves the way for LMT-enhanced clock atom interferometry on even narrower transitions, a key ingredient in proposals for gravitational wave detection and dark matter searches.
Strontium clock atom interferometry is a promising new technology, with multiple experiments under development around the world to explore its potential for dark matter and gravitational wave detection. In these detectors, large momentum transfer using sequences of many laser pulses is necessary, and thus high-fidelity pulses are important since small errors become magnified. Quantum optimal control (QOC) is a framework for developing control pulse waveforms that achieve high fidelity and are robust against experimental imperfections. Resonant single-photon transitions using the narrow clock transition of strontium involve significantly different quantum dynamics than more established atom interferometry methods based on far-detuned two-photon Raman or Bragg transitions, which leads to new opportunities and challenges when applying QOC. Here, we study in simulation QOC pulses for strontium clock interferometry and demonstrate their advantage over basic square pulses (primitive pulses) and composite pulses in terms of robustness against multiple noise channels. This could improve the scale of large momentum transfer in Sr clock interferometers, paving the way to achieving these scientific goals.
We report on the realization of a matter-wave interferometer based on single-photon interaction on the ultranarrow optical clock transition of strontium atoms. We experimentally demonstrate its operation as a gravimeter and as a gravity gradiometer. No reduction of interferometric contrast was observed for a total interferometer time up to ∼10 ms, limited by geometric constraints of the apparatus. Single-photon interferometers represent a new class of high-precision sensors that could be used for the detection of gravitational waves in so far unexplored frequency ranges and to enlighten the boundary between quantum mechanics and general relativity.
Atom interferometry is a maturing quantum technology which provides one of the most precise approaches to explore fundamental physics, e.g. to search for dark matter, and one day to observe gravitational waves in the frequency range from 10 mHz - 10 Hz. Standard atom interferometers use Bragg or Raman two-photon transitions for the coherent manipulation of matter waves. In a Michelson configuration for atom-aided gravitational waves detection, two orthogonal arms are built to reject laser noise, in the same way as optical interferometers. Atom interferometers utilizing an optical clock transition for coherent manipulation are less affected by the technical noise of the laser, and as a result that single baseline detectors become feasible.At LP2N, we are building a vertical gravity-gradiometer based on atom interferometry using strontium atoms probed on such a clock transition. The final experimental setup will implement a 6-meter tall atomic fountain to realize gradiometry with two or more separated atomic clouds.In my dissertation, I present the realization of the experimental setup in all its sub-systems, and the first experiments with atoms at millikelvin temperature obtained with the first cooling stage with blue light. The laser system for the second red cooling phase and for the coherent manipulation is ready; meanwhile, we realized a dual-frequency Zeeman slower that improves the atomic flux by a factor of six. We also present a study of an original scheme to achieve pulsed and fast light-atom interaction in a narrow-linewidth cavity by exploiting the Stark shift as a high bandwidth switch; this technique could open to the use of narrow-linewidth cavities – and notably their high power buildup - in several contexts, like atom interferometry and quantum information.
Abstract Large-scale atom interferometers promise unrivaled strain sensitivity to mid-band gravitational waves, and will probe a new parameter space in the search for ultra-light scalar dark matter. These proposals require gradiometry with kilometer-scale baselines, a momentum separation above 104ℏk between interferometer arms, and optical transitions to long-lived clock states to reach the target sensitivities. Prohibitively high optical power and wavefront flatness requirements have thus far limited the maximum achievable momentum splitting. Here we propose a scheme for optical cavity enhanced atom interferometry, using circulating, spatially resolved pulses, and intracavity frequency modulation to meet these requirements. We present parameters for the realization of 20 kW circulating pulses in a 1 km interferometer enabling 104ℏk splitting on the 698 nm clock transition in 87Sr. This scheme addresses the presently insurmountable laser power requirements and is feasible in the context of a kilometer-scale atom interferometer facility.
The utilization of light-pulse atom interferometry presents a valuable technique that has found application in both fundamental scientific inquiries, such as investigating constants such as measurements of fine structure constant α and gravitational constant G, and practical endeavors including acceleration sensing and rotation measurements. This thesis delves into our implementation of a dual atom interferometer design involving the clock transition 1S0 → 3P0 in strontium, concurrently conducting the interferometric sequence on atoms in both ground and excited states. To facilitate the dual atom interferometer’s operation, we have firstly established a compact experimental setup with a transversely loaded bi-dimensional magneto-optical-trap (2D-MOT) to create a high flux source of cold strontium atoms. Introducing a novel cross-polarized bi-color atomic beam slower, we simultaneously addresses two excited Zeeman substates of the transition 1S0 → 1P1 in strontium-88, significantly enhancing the number of atoms prepared in the 461 nm MOT by around 10-fold. Following the 461 nm MOT, the atomic ensemble undergoes cooling in a 689 nm MOT, achieving atomic temperatures below 1 µK. We also install a network of eight magnetic field probes arranged around the cold atomic sample, enabling precise three-axis active control of magnetic fields down to the milligauss level. With the atoms confined in a 2D lattice at the magic-wavelength of 813.427 nm after the initial preparation phase, we conduct the magnetically-induced clock transition to create a statistical mixture state of ground and excited states. After a velocity selection stage, implementing a Mach-Zehnder interferometer with Bragg pulses operating at the magic-wavelength along the vertical axis, we conduct tests of the weak equivalence principle (WEP). The Eötvös ratio we found in our system stood at (1.8 ± 3.1) × 10−4, mainly limited by the finite temperature of the atomic cloud constraining the interrogation time. Furthermore, the dual atom interferometer scheme enables the measurement of state-dependent force and eventually polarizability difference via the phase shift between the atoms in different states, and we experimentally demonstrate this by introducing an additional light field gradient.
Atom interferometry on optical clock transitions is being pursued for numerous long-baseline experiments both terrestrially and for future space missions. Crucial to meeting these experiments' required sensitivities is the implementation of large momentum transfer ($>101010^3\hbar k$). Here we show that to sequentially apply such a large momentum via πππ pulses places stringent requirements on the frequency noise of the interferometry laser, finding that the linewidth is required to be considerably lower than has previously been suggested. This is due to imperfect pulse fidelity in the presence of noise and is apparent even for an atom at rest interacting with resonant light, making this a fundamental constraint on operational fidelity for a given laser and pulse sequence. Within this framework, we further present and analyse two high-power, frequency-stabilised laser sources designed to perform interferometry on the 1^11S0_00​ - 3^33P0_00​ clock transitions of cadmium and strontium, respectively operating at 332 nm and 698 nm.