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arXiv:1908.11442 · Journal of Physics B Atomic Molecular and Optical Physics

Coupling atoms to cavities using narrow linewidth optical transitions: applications to frequency metrology

Matthew A. Norcia

Published Sep 6, 2019• 3 citations
arXivHTMLPDF

Abstract

Abstract Narrow linewidth optical atomic transitions provide a valuable resource for frequency metrology, and form the basis of today's most precise and accurate clocks. Recent experiments have demonstrated that ensembles of atoms can be interfaced with the mode of an optical cavity using such transitions, and that atom-cavity interactions can dominate over decoherence processes even when the atomic transition that mediates the interactions is very weak. This scenario enables new opportunities for optical frequency metrology, including techniques for nondestructive readout and entanglement enhancement for optical lattice clocks, methods for cavity-enhanced laser frequency stabilization, and high-precision active optical frequency references based on superradiant emission. This tutorial provides a pedagogical description of the physics governing atom-cavity coupling with narrow linewidth optical transitions, and describes several examples of applications to optical frequency metrology.

DOI
10.1088/1361-6455/ab3930

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Abstract Narrow linewidth optical atomic transitions provide a valuable resource for frequency metrology, and form the basis of today's most precise and accurate clocks. Recent experiments have demonstrated that ensembles of atoms can be interfaced with the mode of an optical cavity using such transitions, and that atom-cavity interactions can dominate over decoherence processes even when the atomic transition that mediates the interactions is very weak. This scenario enables new opportunities for optical frequency metrology, including techniques for nondestructive readout and entanglement enhancement for optical lattice clocks, methods for cavity-enhanced laser frequency stabilization, and high-precision active optical frequency references based on superradiant emission. This tutorial provides a pedagogical description of the physics governing atom-cavity coupling with narrow linewidth optical transitions, and describes several examples of applications to optical frequency metrology.
In my thesis work, I have explored a variety of ways in which narrow linewidth optical transitions can be utilized to extend the capabilities of precision measurement and quantum science. These tools include non-destructive atom counting techniques that may enhance the performance of optical lattice clocks, a novel form of cavity enhanced atomic spectroscopy appropriate for laser frequency stabilization, a new form of laser cooling with reduced reliance on spontaneous emission, several methods for enhancing the sensitivity of proposed atomic gravitational wave detectors, a newly observed form of cavity-mediated spin-spin interactions, and a new class of laser based on optical superradiance from narrow and ultra-narrow linewidth transitions. As part of the superradiant laser project, we have demonstrated the most precise active absolute frequency reference realized to date, which still has great potential for improvement.\nMany of these tools involve coupling atoms to an optical cavity, a field known as cavity quantum electrodynamics, or cavity QED. In my thesis work, a key focus was the extension of cavity QED techniques into the new regime of coupling large ensembles of atoms to a cavity using narrow linewidth optical transitions (in contrast to the previously explored regimes of microwave-frequency transitions or broad-linewidth optical transitions). To this end, I constructed a new experiment to couple an ensemble of atoms to an optical cavity using two optical transitions in atomic strontium, one with a narrow 7.5 kHz linewidth, and another with an ultra-narrow 1 mHz linewidth. This new system has allowed us to access a unique new regime of cavity QED, and a wealth of interesting and useful applications.
Ultra stable frequency references such as the ones used in optical atomic clocks and for quantum metrology may be obtained by stabilizing a laser to an optical cavity that is stable over time. State-of-the-art frequency references are constructed in this way, but their stabilities are currently limited by thermally induced length fluctuations in the reference cavity. Several alternative approaches using the potential for frequency discriminating of highly forbidden narrow atomic transitions have been proposed in, e.g., [1] and [2]. In this proceeding we will present some of the ongoing experimental efforts derived from these proposals, to use cavity-enhanced interaction with atomic 88 Sr samples as a frequency reference for laser stabilization. Such systems can be realized using both passive and active approaches where either the atomic phase response is used as an error signal, or the narrow atomic transition itself is used as a source for a spectrally pure laser. Both approaches shows the promise of being able to compete with the current state of the art in stable lasers and have similar limitations on their ultimately achievable linewidths [1, 2].
Superradiant lasers promise continuous, narrow-linewidth coherent emission at the bare atomic transition frequency, enabling frequency references of exceptional precision. Recent experiments have advanced the field, but achieving truly continuous operation remains technically challenging. Here we propose an alternative route to an active optical frequency reference with fewer emitters using all-to-all dipole-dipole interactions mediated by a nanophotonic waveguide. We show that selectively pumping only a sub-ensemble of emitters, rather than the full ensemble, substantially improves emission characteristics. The collective interactions with unpumped emitters provide narrowband frequency selection and establish an effective feedback mechanism analogous to the role of a macroscopic cavity. We find directional superradiant emission with strongly phase-synchronized emitter correlations and a narrow output spectrum close to the bare emitter resonance. Our results demonstrate a strong metrological gain from selective partial pumping of quantum emitters with the second-order intensity correlation g(2)(0)≃1g^{(2)}(0)\simeq 1g(2)(0)≃1, indicating reduced equal-time intensity fluctuations, and open a route to waveguide-based optical frequency references using small clock-atom ensembles for chip-scale precision metrology.
We will describe a next-generation active atomic frequency reference based on super-radiant pulses of laser light from the ultra-narrow, 1 mHz linewidth, optical clock transition in an ensemble of cold 87Sr atoms. Light is stimulated from the millihertz linewidth transition by confining an ensemble of laser cooled atoms inside of a high finesse optical cavity. Such a light source has been proposed as a next-generation active atomic frequency reference, with the potential to enable high-precision optical frequency references to be used outside laboratory environments. We achieve a remarkable short term fractional frequency stability, 6.7 × 1016 at 1 s of averaging, absolute accuracy, 2 Hz (4 × 1015 fractional frequency), and high insensitivity to changes in the cavity length that limits the performance of todays more stable lasers. We will also discuss current work on cavity-enhanced dispersive measurements to perform high resolution spectroscopy and atom counting.
Narrow-linewidth lasers with absolute frequency anchoring are essential for precision metrology, coherent sensing, and emerging quantum technologies beyond laboratory environments. Optical cavities and interferometers provide exceptional short-term spectral purity but lack intrinsic absolute frequency references. Atomic transitions, in contrast, provide stable frequency anchors but offer limited discrimination sensitivity. Recent hybrid approaches have demonstrated the combination of compact optical resonators with atomic references, yet achieving the Hz-level regime remains challenging. Here, we present a hybrid architecture that enables simultaneous realization of Hz-level linewidth and atomic-referenced frequency stability. An external-cavity diode laser is first stabilized to a fiber interferometer to achieve Hz-level spectral purity, while the interferometer is subsequently anchored to an 87Rb D2 transition via modulation transfer spectroscopy to suppress long-term drift and define the laser frequency relative to the atomic transition. This dual-stabilization scheme realizes a compact atomic-referenced laser with a 3.4-Hz linewidth (1-rad integrated-phase method), a minimum fractional frequency stability of 3.4x10-14 at 0.56 s, and 9x10-13 at 100 s. This architecture establishes a practical and scalable route toward compact and field-deployable atomic-referenced narrow-linewidth lasers for precision metrology and quantum technologies.
An ideal superradiant laser on an optical clock transition of noninteracting cold atoms is predicted to exhibit an extreme frequency stability and accuracy far below mHz-linewidth. In any concrete setup sufficiently many atoms have to be confined and pumped within a finite cavity mode volume. Using a magic wavelength lattice minimizes light shifts and allows for almost uniform coupling to the cavity mode. Nevertheless, the atoms are subject to dipole-dipole interaction and collective spontaneous decay which compromises the ultimate frequency stability. In the high density limit the Dicke superradiant linewidth enhancement will broaden the laser line and nearest neighbor couplings will induce shifts and fluctuations of the laser frequency. We estimate the magnitude and scaling of these effects by direct numerical simulations of few atom systems for different geometries and densities. For Strontium in a regularly filled magic wavelength configuration atomic interactions induce small laser frequency shifts only and collective spontaneous emission weakly broadens the laser. These interactions generally enhance the laser sensitivity to cavity length fluctuations but for optimally chosen operating conditions can lead to an improved synchronization of the atomic dipoles.