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arXiv:1908.06107 · Bulletin of the American Physical Society

Dielectric breakdown of strongly correlated insulators in one dimension: Universal formula from non-Hermitian sine-Gordon theory

Kazuaki Takasan, Masaya Nakagawa, Norio Kawakami

Published Aug 16, 2019• 2 citations
arXivHTMLPDF

Abstract

Application of a strong electric field to insulators induces a finite current. This phenomenon is called dielectric breakdown and is known as a fundamental nonequilibrium and nonlinear transport phenomenon in solids. Here, we study the dielectric breakdown of generic strongly correlated insulators in one dimension. Combining bosonization techniques with a quantum tunneling theory, we develop an effective field-theoretical description of dielectric breakdown using a non-Hermitian sine-Gordon theory. Then, we derive an analytic formula for the threshold field, which is a many-body generalization of the Landau-Zener formula. Importantly, we point out that the threshold field contains a previously overlooked factor originating from the charges of elementary excitations, which should be significant when a system has fractionalized excitations. We apply our results to integrable lattice models and confirm that our formula is valid in a broad range including the weak coupling regime, indicating its wide potential applicability. Our results unveil universal aspects of nonlinear and nonequilibrium transport phenomena in various strongly correlated insulators.

DOI
10.48550/arxiv.1908.06107

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Application of a strong electric field to insulators induces a finite current. This phenomenon is called dielectric breakdown and is known as a fundamental nonequilibrium and nonlinear transport phenomenon in solids. Here, we study the dielectric breakdown of generic strongly correlated insulators in one dimension. Combining bosonization techniques with a quantum tunneling theory, we develop an effective field-theoretical description of dielectric breakdown using a non-Hermitian sine-Gordon theory. Then, we derive an analytic formula for the threshold field, which is a many-body generalization of the Landau-Zener formula. Importantly, we point out that the threshold field contains a previously overlooked factor originating from the charges of elementary excitations, which should be significant when a system has fractionalized excitations. We apply our results to integrable lattice models and confirm that our formula is valid in a broad range including the weak coupling regime, indicating its wide potential applicability. Our results unveil universal aspects of nonlinear and nonequilibrium transport phenomena in various strongly correlated insulators.
The nonadiabatic quantum tunneling picture, which may be called the many-body Schwinger-Landau-Zener mechanism, for the dielectric breakdown of Mott insulators in strong electric fields is studied in the one-dimensional Hubbard model. The tunneling probability is calculated by a method due to Dykhne-Davis-Pechukas with an analytical continuation of the Bethe-ansatz solution for excited states to a non-Hermitian case. A remarkable agreement with the time-dependent density-matrix renormalization-group result is obtained.
We investigate the dielectric breakdown of mesoscopic Mott insulators, a phenomenon where a strong electric field destabilizes the insulating state, resulting in a transition to a metallic phase. Using the Landau-Zener formalism, which models the excitation of a two-level system, we derive a theoretical expression for the threshold value of the field. To validate our predictions, we present an efficient protocol for estimating the charge gap and threshold field via non-equilibrium current oscillations, overcoming the computational limitations of exact diagonalization. Our simulations demonstrate the accuracy of our theoretical formula for systems with small gaps. Moreover, our findings are directly testable in ultracold atomic experiments with ring geometries and artificial gauge fields, as our method uses measurable quantities and relies on already available technologies. This work aims to bridge the gap between theoretical models and experimentally realizable protocols, providing tools to explore non-equilibrium mesoscopic phenomena in strongly correlated quantum systems.
Time-dependent nonequilibrium properties of a strongly correlated electron system driven by large electric fields is obtained by means of solving the time-dependent Schrödinger equation for the many-body wave function numerically in one dimension. While the insulator-to-metal transition depends on the electric field and the interaction, the metallization is found to be described in terms of a universal Landau-Zener quantum tunneling among the many-body levels. These processes induce current oscillation for small systems, while giving rise to finite resistivity through dissipation for larger systems/on longer time scales.
Correlated systems are a wide class of materials in which the strong electron-electron repulsion is the origin of very fascinating and unusual properties, among which metal-to-insulator transitions and high temperature superconductivity are the most striking examples. In the recent years, the fast development of non-adiabatic probing techniques opened new interesting perspectives for the investigation of such materials in non-equilibrium conditions. In this thesis, we discuss the theoretical description of few relevant cases which represent different examples of non-equilibrium phenomena in correlated materials. In particular, we will focus on the dynamics following a sudden excitation and the coupling to an external driving field. As a first example we consider the dynamics across a phase transition, namely we explore the possibility of driving a phase transition as the result of a sudden excitation, as e.g. the coupling with a short light pulse. We consider systems showing different equilibrium phases and study the conditions under which the off-equilibrium dynamics may lead to non-trivial dynamical phase transitions. A different case is represented by the dynamics induced by a driving electric field. This problem is particularly relevant for the possible applications of correlated materials in electronic devices. Here we consider the paradigmatic case of a correlated material coupled to external sources which impose a finite bias across the system. We analyze the formation and the properties of the non-equilibrium stationary states in which a finite current flows through the system. This allows us to study the non-linear response properties of a correlated system. In this context, a particularly relevant aspect is the problem of the dielectric breakdown of a Mott insulator, namely the formation of conducting states in the Mott insulating phase. In this thesis we explore different mechanisms leading to such possibility. First we discuss a quantum tunneling mechanism of carriers driven across the insulating gap by the effect of strong electric-fields. Eventually, we discuss the possibility of a resistive transition from an insulating to a metallic state induced by the application of an external electric-field.
Charge creation via quantum tunneling, i.e. dielectric breakdown, is one of the most fundamental and significant phenomena arising from strong light(field)-matter coupling. In this work, we conduct a systematic numerical analysis of quantum tunneling in one-dimensional Mott insulators described by the extended (UUU-VVV) Hubbard model. We discuss the applicability of the analytical formula for doublon-holon (DH) pair production, previously derived for the one-dimensional Hubbard model, which highlights the relationship between the tunneling threshold, the charge gap, and the correlation length. We test the formulas ability to predict both DH pair production and energy increase rate. Using tensor-network-based approaches, we demonstrate that the formula provides accurate predictions in the absence of excitonic states facilitated by the nearest-neighbor interaction VVV. However, when excitonic states emerge, the formula more accurately describes the rate of energy increase than the DH pair creation rate and in both cases gets improved by incorporating the exciton energy as the effective gap.
The nonlinear transport properties of the Mott insulator are discussed with focus on the many-body Landau-Zener mechanism. After reviewing basic concepts such as the non-adiabatic geometric phase and the Schwinger mechanism, we study the decay of the insulating groundstate in strong electric fields using the time-dependent density matrix renormalization group. A short comment on the proposed mapping to the quantum walk model is added before discussing the relevance of the theory to experimental results. This article is a draft of a book chapter of the book entitled "Quantum and Semi-classical Percolation & Breakdown" (Lecture Note in Physics, Springer-Verlag), to appear 2008.