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arXiv:1907.09888 · Physical Review A

Idealized Einstein-Podolsky-Rosen states from non–phase-matched parametric down-conversion

Cameron Okoth, E. V. Kovlakov, Florian Bönsel, Andrea Cavanna, Stanislav S. Straupe, S. P. Kulik, Maria V. Chekhova

Published Jan 14, 2020• 30 citations
arXivHTMLPDF

Abstract

The most common source of entangled photons is spontaneous parametric down-conversion (SPDC). The degree of energy and momentum entanglement in SPDC is determined by the nonlinear interaction volume. By reducing the length of a highly nonlinear material, we relax the longitudinal phase-matching condition and reach record levels of transverse momentum entanglement. The degree of entanglement is estimated using both correlation measurements and stimulated emission tomography in wave-vector space. The high entanglement of the state in wave-vector space can be used to massively increase the quantum information capacity of photons, but more interestingly the equivalent state measured in position space is correlated over distances far less than the photon wavelength. This property promises to improve the resolution of many quantum imaging techniques beyond the current state of the art.

DOI
10.1103/physreva.101.011801

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The most common source of entangled photons is spontaneous parametric down-conversion (SPDC). The degree of energy and momentum entanglement in SPDC is determined by the nonlinear interaction volume. By reducing the length of a highly nonlinear material, we relax the longitudinal phase-matching condition and reach record levels of transverse momentum entanglement. The degree of entanglement is estimated using both correlation measurements and stimulated emission tomography in wave-vector space. The high entanglement of the state in wave-vector space can be used to massively increase the quantum information capacity of photons, but more interestingly the equivalent state measured in position space is correlated over distances far less than the photon wavelength. This property promises to improve the resolution of many quantum imaging techniques beyond the current state of the art.
The successful employment of high-dimensional quantum correlations and its integration in telecommunication infrastructures is vital in cutting-edge quantum technologies for increasing robustness and key generation rate. Position-momentum Einstein-Podolsky-Rosen (EPR) entanglement of photon pairs are a promising resource of such high-dimensional quantum correlations. Here, we experimentally certify EPR correlations of photon pairs generated by spontaneous parametric down-conversion (SPDC) in a nonlinear crystal with type-0 phase-matching at telecom wavelength for the first time. To experimentally observe EPR entanglement, we perform scanning measurements in the near- and far-field planes of the signal and idler modes. We certify EPR correlations with high statistical significance of up to 45 standard deviations. Furthermore, we determine the entanglement of formation of our source to be greater than one, which gives evidence for the the high-dimensional entanglement between the photons. Operating at telecom wavelengths around 1550 nm, our source is compatible with today's deployed telecommunication infrastructure, thus paving the way for integrating sources of high-dimensional entanglement into quantum-communication infrastructures.
Abstract The successful employment of high-dimensional quantum correlations and its integration in telecommunication infrastructures is vital in cutting-edge quantum technologies for increasing robustness and key generation rate. Position-momentum Einstein-Podolsky-Rosen (EPR) entanglement of photon pairs are a promising resource of such high-dimensional quantum correlations. Here, we experimentally certify EPR correlations of photon pairs generated by spontaneous parametric down-conversion (SPDC) in a nonlinear crystal with type-0 phase-matching at telecommunication wavelength for the first time. To experimentally observe EPR entanglement, we perform scanning measurements in the near- and far-field planes of the signal and idler modes. We certify EPR correlations with high statistical significance of up to 45 standard deviations. Furthermore, we determine the entanglement of formation of our source to be greater than one, indicating a dimensionality of greater than 2. Operating at telecommunication wavelengths around 1550 nm, our source is compatible with today’s deployed telecommunication infrastructure, thus paving the way for integrating sources of high-dimensional entanglement into quantum-communication infrastructures.
The generation of entangled photon pairs through spontaneous parametric down conversion (SPDC) is widely used and considered one of the key entanglement generation techniques in quantum optics. The quality of the entanglement produced depends significantly on the physical properties of the nonlinear crystal employed in the SPDC process. In this study, we investigate the influence of the crystal parameters such as phase matching configurations on the degree of entanglement. Our results demonstrate the importance of crystal selection for achieving highly entangled photon sources, which are essential for applications in quantum communication and quantum information.
Spontaneous parametric down-conversion (SPDC) is one of the most important sources of entangled photons in quantum optics and underpins a wide range of applications in quantum communication, quantum imaging, quantum sensing, and photonic quantum information processing. In this nonlinear optical process, a pump photon is converted into a pair of lower-energy photons that exhibit strong correlations in multiple degrees of freedom. While the generation of photon pairs is governed by energy and momentum conservation, the resulting biphoton state possesses a rich spatial structure whose properties are determined by the interplay among the pump field, the nonlinear medium, and subsequent propagation. This thesis investigates the spatial properties of entangled photon pairs generated through SPDC, focusing on the evolution of their correlations in the near field and on the behavior of orbital-angular-momentum (OAM) entangled states under tight focusing conditions. A common theme throughout this work is the examination of physical effects that emerge when the full biphoton wavefunction is retained rather than reduced through the simplifying approximations often employed in theoretical treatments. The principal contribution of this thesis concerns the near-field propagation of SPDC photon pairs. The spatial correlations of SPDC-generated photons are commonly analyzed within the thin-crystal approximation, where the biphoton wavefunction is assumed to factorize into independent functions of the sum and difference coordinates. We demonstrate that birefringence-induced transverse walk-off breaks this factorization and introduces an intrinsic coupling between these coordinates. More importantly, this coupling survives free-space propagation and remains observable even for crystals that nominally satisfy the thin-crystal condition. As a result, the joint spatial correlations develop a characteristic tapering near the crystal image plane that cannot be captured by conventional factorized models. Numerical simulations and experimental measurements are found to be in excellent agreement, revealing a previously overlooked feature of SPDC and providing a more complete description of photon-pair generation and propagation in birefringent nonlinear media. The second part of the thesis explores the propagation of OAM-entangled photon pairs beyond the paraxial regime. While OAM correlations are typically studied under weak-focusing conditions, many emerging quantum technologies require structured quantum states to be manipulated in highly confined optical systems. We show that tight focusing modifies the OAM correlation spectrum, leading to a broadening of the accessible mode distribution. This broadening exhibits distinct transverse and longitudinal characteristics and arises from the emergence of nonparaxial field components absent in conventional scalar descriptions. These results provide new insight into the behavior of structured quantum light in strongly focused optical fields and establish a framework for understanding OAM entanglement beyond the paraxial approximation. Together, the results presented in this thesis reveal previously unexplored aspects of the structure and propagation of entangled photon pairs. By moving beyond widely used approximations, this work uncovers physical effects that influence the generation, evolution, and measurement of spatially entangled states, with implications for quantum imaging, high-dimensional quantum communication, and the broader development of structured-light-based quantum technologies.
Miniaturization of nonlinear optical elements is one of the major trends of modern photonics. In particular, in the ‘flatoptics’ geometry, the sample is ultrathin along the light propagation direction. For nonlinear optical effects in such samples, phase matching is satisfied automatically, which allows for the use of materials with giant nonlinear susceptibilities. The tiny thickness reduces the efficiency but it can be compensated for by using geometric and material resonances. Recently also spontaneous parametric down-conversion (SPDC), leading to the generation of entangled photons, has been implemented in ultrasmall sources: subwavelength layers, metasurfaces, even nanoantennas. The lifted constraint of phase matching gives to SPDC even more freedom than to classical frequency conversion effects. The reason is that SPDC, as a spontaneous effect, is stimulated by quantum vacuum fluctuations, which populate all modes uniformly. SPDC in ultrathin samples demonstrates very broad spectral and angular width, extremely high degrees of continuous-variable entanglement, tunable polarization entanglement, and orders of magnitude enhancement of photon pair production rate due to the geometric resonances of dielectric metasurfaces.