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arXiv:1907.08173 · Nature Communications

Kosterlitz-Thouless melting of magnetic order in the triangular quantum Ising material TmMgGaO4

Han Li, Yuan Da Liao, Bin-Bin Chen, Xu-Tao Zeng, Xian‐Lei Sheng, Yang Qi, Zi Yang Meng, Wei Li

Published Feb 28, 2020• 90 citations
arXivHTMLPDF

Abstract

Abstract Frustrated magnets hold the promise of material realizations of exotic phases of quantum matter, but direct comparisons of unbiased model calculations with experimental measurements remain very challenging. Here we design and implement a protocol of employing many-body computation methodologies for accurate model calculations—of both equilibrium and dynamical properties—for a frustrated rare-earth magnet TmMgGaO 4 (TMGO), which explains the corresponding experimental findings. Our results confirm TMGO is an ideal realization of triangular-lattice Ising model with an intrinsic transverse field. The magnetic order of TMGO is predicted to melt through two successive Kosterlitz–Thouless (KT) phase transitions, with a floating KT phase in between. The dynamical spectra calculated suggest remnant images of a vanishing magnetic stripe order that represent vortex–antivortex pairs, resembling rotons in a superfluid helium film. TMGO therefore constitutes a rare quantum magnet for realizing KT physics, and we further propose experimental detection of its intriguing properties.

DOI
10.1038/s41467-020-14907-8

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Abstract Frustrated magnets hold the promise of material realizations of exotic phases of quantum matter, but direct comparisons of unbiased model calculations with experimental measurements remain very challenging. Here we design and implement a protocol of employing many-body computation methodologies for accurate model calculations—of both equilibrium and dynamical properties—for a frustrated rare-earth magnet TmMgGaO 4 (TMGO), which explains the corresponding experimental findings. Our results confirm TMGO is an ideal realization of triangular-lattice Ising model with an intrinsic transverse field. The magnetic order of TMGO is predicted to melt through two successive Kosterlitz–Thouless (KT) phase transitions, with a floating KT phase in between. The dynamical spectra calculated suggest remnant images of a vanishing magnetic stripe order that represent vortex–antivortex pairs, resembling rotons in a superfluid helium film. TMGO therefore constitutes a rare quantum magnet for realizing KT physics, and we further propose experimental detection of its intriguing properties.
The Ghost of a Vanishing Stripe Order in the Triangular Quantum Ising Magnet TmMgGaO4_44​
Frustrated magnets host the promises of material realizations of new paradigm of quantum matter, while direct comparison of unbiased model calculations with experimental measurements is still very challenging. Here, we design and implement a protocol of employing many-body computation methodologies for accurate model calculation -- both equilibrium and dynamical properties -- of a frustrated rare-earth magnet TmMgGaO4_44​ (TMGO), which perfectly explains the corresponding experimental findings. Our results confirm TMGO is an ideal realization of triangular-lattice Ising model with an intrinsic transverse field. The magnetic order of TMGO is predicted to melt through two successive Kosterlitz-Thouless (KT) phase transitions, with a floating KT phase in between. The dynamical spectra calculated suggest remnant images of a vanishing magnetic stripe order that represent vortex-antivortex pairs, resembling rotons in a superfluid helium film. TMGO therefore constitutes a rare quantum magnet for realizing KT physics and we further propose experimental detections of its intriguing properties.
The rare-earth magnet TmMgGaO 4 is proposed to be an intrinsic quantum Ising magnet described by the antiferromagnetic transverse field Ising model (TFIM) on a triangular lattice, where the relevant degrees of freedom are the nondegenerate dipole-multipole doublets of the Tm 3+ ions and the transverse field has an intrinsic origin from the weak splitting of the doublet.We compare this special doublet of Tm 3+ with the dipole-octupole Kramers doublet.We study the proposed effective model for the Tm-based triangular lattice and consider the effects of external magnetic fields and finite temperatures.From the orthogonal operator approach, we show that the TFIM with the three-sublattice intertwined ordered state agrees with the experiments and further clarify the discrepancy in the numbers of the magnetic sublattices and the measured magnon branches.We make specific predictions for the evolution of the magnetic properties with the external magnetic field.Furthermore, we demonstrate that an emergent U(1) symmetry emerges in thermal melting of the underlying orders and at the criticality, and summarize the previously known signatures related to the finite-temperature Berezinskii-Kosterlitz-Thouless physics.We discuss the broad relevance of intrinsic quantum Ising magnets to many other systems, especially Tm-based materials.
A programmable quantum simulator using Rydberg-atom array provides a promising route to demystifying quantum many-body physics in strongly correlated systems. Motivated by the recent realization of various quantum magnetic phases on the frustrated Rydberg-atom array, we perform numerically exact quantum Monte Carlo simulations to investigate the exotic states of matter emerging in the model describing the Rydberg atom on a triangular lattice. Our state-of-the-art simulation unveils the $\sqrt{3}\ifmmode\times\else\texttimes\fi{}\sqrt{3}$ triangular antiferromagnetic order exists at 1/31/31/3 or 2/32/32/3-Rydberg filling, consistent with the observation in experiments. Remarkably, $\sqrt{3}\ifmmode\times\else\texttimes\fi{}\sqrt{3}$ long-range order arising from order-by-disorder mechanism emerges at 1/21/21/2 filling. At finite temperature, U(1)\mathrm{U}(1)U(1) symmetry is emergent at 1/21/21/2 filling and a Kosterlitz-Thouless phase transition occurs with increasing temperature. These intriguing phenomena are potentially detected in future Rydberg-atom experiments.
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Abstract We investigate the quantum dynamics of the antiferromagnetic transverse field Ising model on the triangular lattice through large-scale quantum Monte Carlo simulations and stochastic analytic continuation. This model effectively describes a series of triangular rare-earth compounds, for example, TmMgGaO 4 . At weak transverse field, we capture the excitations related to topological quantum strings, which exhibit continuum features described by XY chain along the strings and those in accord with ‘Luttinger string liquid’ in the perpendicular direction. The continuum features can be well understood from the perspective of topological strings. Furthermore, we identify the contribution of strings from the excitation spectrum. Our study provides characteristic features for the experimental search for string-related excitations and proposes a theoretical method to pinpoint topological excitations in the experimental spectra.
Abstract Phase transitions and thermodynamics properties of the frustrated antiferromagnetic XY (FAXY) model have been investigated near the two transition temperatures. We found that the Kosterlitz-Thouless (KT) transition corresponding to the rotational U(1) symmetry breaking and the Ising-like (I) transition corresponding to the reflection Z 2 symmetry breaking occur at two-separate transition temperatures, Tkt < TI . These temperatures lie close to each other, however in our results the separation is obvious. Our results show the order parameters as a function of temperature and we also estimate the critical exponents, β, α, γ, η and ν. The critical exponent ν indicates that the Ising-like transition is inconsistent with the Ising universality class.