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arXiv:2010.01750 · npj Quantum Materials

Quantum dynamics of topological strings in a frustrated Ising antiferromagnet

Zheng Zhou, Changle Liu, Zheng Yan, Yan Chen, Xue‐Feng Zhang

Published Jun 8, 2022• 26 citations
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Abstract

Abstract We investigate the quantum dynamics of the antiferromagnetic transverse field Ising model on the triangular lattice through large-scale quantum Monte Carlo simulations and stochastic analytic continuation. This model effectively describes a series of triangular rare-earth compounds, for example, TmMgGaO 4 . At weak transverse field, we capture the excitations related to topological quantum strings, which exhibit continuum features described by XY chain along the strings and those in accord with ‘Luttinger string liquid’ in the perpendicular direction. The continuum features can be well understood from the perspective of topological strings. Furthermore, we identify the contribution of strings from the excitation spectrum. Our study provides characteristic features for the experimental search for string-related excitations and proposes a theoretical method to pinpoint topological excitations in the experimental spectra.

DOI
10.1038/s41535-022-00465-3

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Abstract We investigate the quantum dynamics of the antiferromagnetic transverse field Ising model on the triangular lattice through large-scale quantum Monte Carlo simulations and stochastic analytic continuation. This model effectively describes a series of triangular rare-earth compounds, for example, TmMgGaO 4 . At weak transverse field, we capture the excitations related to topological quantum strings, which exhibit continuum features described by XY chain along the strings and those in accord with ‘Luttinger string liquid’ in the perpendicular direction. The continuum features can be well understood from the perspective of topological strings. Furthermore, we identify the contribution of strings from the excitation spectrum. Our study provides characteristic features for the experimental search for string-related excitations and proposes a theoretical method to pinpoint topological excitations in the experimental spectra.
Incommensurability plays a critical role in many strongly correlated systems. In some cases, the origin of such exotic order can be theoretically understood in the framework of 1d line-like topological excitations known as “quantum strings”. Here we study an extended transverse field Ising model on a triangular lattice. Using large-scale quantum Monte Carlo simulations, we find that the spatial anisotropy can stabilize an incommensurate phase out of the commensurate clock order. Our results for the structure factor and the string density exhibit a linear relationship between incommensurate ordering wave vector and the density of quantum strings, which is reminiscent of hole density in under-doped cuprate superconductors. When introducing the next-nearest-neighbor interaction, we observe a quantum tricritical point out of the incommensurate phase. After carefully analyzing the ground state energies within different string topological sectors, we conclude that this tricriticality is non-trivially caused by effective long-range inter-string interactions with two competing terms following different decaying behaviors.
We report on a systematic study of two-dimensional, periodic, frustrated Ising models with quantum dynamics introduced via a transverse magnetic field. The systems studied are the triangular and kagom\'e lattice antiferromagnets, fully frustrated models on the square and hexagonal (honeycomb) lattices, a planar analog of the pyrochlore antiferromagnet, a pentagonal lattice antiferromagnet, as well as two quasi-one-dimensional lattices that have considerable pedagogical value. All of these exhibit a macroscopic degeneracy at T=0T=0T=0 in the absence of the transverse field, which enters as a singular perturbation. We analyze these systems with a combination of a variational method at weak fields, a perturbative Landau-Ginzburg-Wilson approach from large fields, as well as quantum Monte Carlo simulations utilizing a cluster algorithm. Our results include instances of quantum order arising from classical criticality (triangular lattice) or classical disorder (pentagonal and probably hexagonal) as well as notable instances of quantum disorder arising from classical disorder (kagom\'e). We also discuss the effect of finite temperature, as well as the interplay between longitudinal and transverse fields---in the kagom\'e problem the latter gives rise to a nontrivial phase diagram with bond-ordered and bond-critical phases in addition to the disordered phase. We also note connections to quantum-dimer models and thereby to the physics of Heisenberg antiferromagnets in short-ranged resonating valence-bond phases that have been invoked in discussions of high-temperature superconductivity.
Geometric frustration in two-dimensional Ising models allows for a wealth of exotic universal behavior, both Ising and non-Ising, in the presence of quantum fluctuations. In particular, the triangular antiferromagnet and Villain model in a transverse field can be understood through distinct XY pseudospins, but have qualitatively similar phase diagrams including a quantum phase transition in the (2+1)-dimensional XY universality class. While the quantum dynamics of modestly-sized systems can be simulated classically using tensor-based methods, these methods become infeasible for larger lattices. Here we perform both classical and quantum simulations of these dynamics, where our quantum simulator is a superconducting quantum annealer. Our observations on the triangular lattice suggest that the dominant quench dynamics are not described by the quantum Kibble-Zurek scaling of the quantum phase transition, but rather a faster coarsening dynamics in an effective two-dimensional XY model in the ordered phase. Similarly, on the Villain model, the scaling exponent does not match the Kibble-Zurek expectation. These results demonstrate the ability of quantum annealers to perform coherent quantum dynamics simulations that are hard to classically scale beyond small systems, and open the avenue to predictive simulations of the dynamics of Ising magnetic materials on quantum simulators.
The Ghost of a Vanishing Stripe Order in the Triangular Quantum Ising Magnet TmMgGaO4_44​
Frustrated magnets host the promises of material realizations of new paradigm of quantum matter, while direct comparison of unbiased model calculations with experimental measurements is still very challenging. Here, we design and implement a protocol of employing many-body computation methodologies for accurate model calculation -- both equilibrium and dynamical properties -- of a frustrated rare-earth magnet TmMgGaO4_44​ (TMGO), which perfectly explains the corresponding experimental findings. Our results confirm TMGO is an ideal realization of triangular-lattice Ising model with an intrinsic transverse field. The magnetic order of TMGO is predicted to melt through two successive Kosterlitz-Thouless (KT) phase transitions, with a floating KT phase in between. The dynamical spectra calculated suggest remnant images of a vanishing magnetic stripe order that represent vortex-antivortex pairs, resembling rotons in a superfluid helium film. TMGO therefore constitutes a rare quantum magnet for realizing KT physics and we further propose experimental detections of its intriguing properties.
Working within the stochastic series expansion framework, we introduce and characterize a plaquette-based quantum cluster algorithm for quantum Monte Carlo simulations of transverse field Ising models with frustrated Ising exchange interactions. As a demonstration of the capabilities of this algorithm, we show that a relatively small ferromagnetic next-nearest-neighbor coupling drives the transverse field Ising antiferromagnet on the triangular lattice from an antiferromagnetic three-sublattice ordered state at low temperature to a ferrimagnetic three-sublattice ordered state.
Motivated by recent experiments with a Penning ion trap quantum simulator, we perform numerically exact Stochastic Series Expansion quantum Monte Carlo simulations of long-range transverse-field Ising models on a triangular lattice for different decay powers $\ensuremath{\alpha}$ of the interactions. The phase boundary for the ferromagnet is obtained as a function of $\ensuremath{\alpha}$. For antiferromagnetic interactions, there is strong indication that the transverse field stabilizes a clock ordered phase with sublattice magnetization $(M,\ensuremath{-}\frac{M}{2},\ensuremath{-}\frac{M}{2})$ with unsaturated M<1M<1M<1 in a process known as ``order by disorder'' similar to the nearest-neighbor antiferromagnet on the triangular lattice. Connecting the known limiting cases of nearest-neighbor and infinite-range interactions, a semiquantitative phase diagram is obtained. Magnetization curves for the ferromagnet for experimentally relevant system sizes and with open boundary conditions are presented.