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arXiv:1907.05541 · Physical Review Letters

Dark States of Multilevel Fermionic Atoms in Doubly Filled Optical Lattices

Asier Piñeiro Orioli, Ana María Rey

Published Nov 26, 2019• 30 citations
arXivHTMLPDF

Abstract

We propose to use fermionic atoms with degenerate ground and excited internal levels (F_{g}→F_{e}), loaded into the motional ground state of an optical lattice with two atoms per lattice site, to realize dark states with no radiative decay. The physical mechanism behind the dark states is an interplay of Pauli blocking and multilevel dipolar interactions. The dark states are independent of lattice geometry, can support an extensive number of excitations, and can be coherently prepared using a Raman scheme taking advantage of the quantum Zeno effect. These attributes make them appealing for atomic clocks, quantum memories, and quantum information on decoherence free subspaces.

DOI
10.1103/physrevlett.123.223601

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We propose to use fermionic atoms with degenerate ground and excited internal levels (F_{g}→F_{e}), loaded into the motional ground state of an optical lattice with two atoms per lattice site, to realize dark states with no radiative decay. The physical mechanism behind the dark states is an interplay of Pauli blocking and multilevel dipolar interactions. The dark states are independent of lattice geometry, can support an extensive number of excitations, and can be coherently prepared using a Raman scheme taking advantage of the quantum Zeno effect. These attributes make them appealing for atomic clocks, quantum memories, and quantum information on decoherence free subspaces.
Fock-state lattices (FSLs) are becoming an emerging research hotspot in quantum physics, not only because the FSLs provide a new perspective for studying atom-field interactions, but also because they build a connection between quantum optics and condensed matter physics. Because of the multiple transition paths in the lattices, an inherent quantum interference effect exists in these systems, and hence finding new quantum-coherent phenomena and exploiting their applications become a significant and desired task in this field. In this work, we study the dark-state effect in the FSLs generated by the multimode Jaynes-Cummings (JC) models. By considering the FSLs in certain excitation-number subspaces, we study the dark states with respect to the states associated with the atomic excited state using the arrowhead-matrix method. We find that dark-state subspaces exist with dimensions determined by the number of orthogonal dark states. When the dimension is greater than one, the forms of these dark-state bases are not unique. Further, we obtain the number and form of the orthogonal dark states in the two-, three-, and four-mode JC models. In addition, we find that for a general N -mode JC model, there are C N + n − 2 N − 2 orthogonal dark states in the n -excitation subspace. We also build the relationship between the dark states and dark modes. Our work paves the way for exploring quantum optical effects and quantum information processing based on the FSLs.
The dark-state effect, caused by destructive quantum interference, is an important physical effect in atomic physics and quantum optics. It not only deepens the understanding of light-atom interactions, but also has wide applications in quantum physics and quantum information. Therefore, how to efficiently and conveniently determine the number and form of the dark states in multilevel quantum systems with complex transitions is an important and interesting topic in this field. In this work, we present a general theory for determining the dark states in multilevel quantum systems with any coupling configuration using the arrowhead-matrix method. To confirm the dark states in a multilevel system, we first define the upper- and lower-state subspaces, and then diagonalize the Hamiltonians restricted within the two subspaces to obtain the dressed upper and lower states. By further expressing the transitions between the dressed upper and lower states, we can map the multilevel system to a bipartite-graph network, in which the nodes and links are acted by the dressed states and transitions, respectively. Based on the coupling configurations of the network, we can determine the lower dark states with respect to the upper-state subspace. As examples, we analyze the dark states in three-, four-, and five-level quantum systems, for all possible configurations through the classification of the numbers of upper and lower states. Furthermore, we extend the framework to multilevel quantum systems and discuss the existence of dark states in some typical configurations. We also recover the results of the dark-state polaritons in driven three-level systems with the arrowhead-matrix method. Our theory paves the way for manipulating and utilizing the dark states of multilevel quantum systems in atomic physics and quantum optics.
We study electronic excitations of a degenerate gas of atoms trapped in pairs in an optical lattice. Local dipole-dipole interactions produce a long-lived antisymmetric and a short-lived symmetric superposition of individual atomic excitations as the lowest internal on-site excitations. Due to the much larger dipole moment the symmetric states couple efficiently to neighbouring lattice sites and can be well represented by Frenkel excitons, while the antisymmetric dark states stay localized. Within a cavity only symmetric states couple to cavity photons inducing long-range interactions to form polaritons. We calculate their dispersion curves as well as cavity transmission and reflection spectra to observe them. For a lattice with aspherical sites bright and dark states get mixed and their relative excitation energies depend on photon polarizations.
We examine dark quantum superposition states of weakly bound Rb2 Feshbach molecules and tightly bound triplet Rb2 molecules in the rovibrational ground state, created by subjecting a pure sample of Feshbach molecules in an optical lattice to a bichromatic Raman laser field. We analyze, both experimentally and theoretically, the creation and dynamics of these dark states. Coherent wavepacket oscillations of deeply bound molecules in lattice sites, as previously observed by Lang et al. (Phys. Rev. Lett., 2008, 101, 133005), are suppressed due to laser-induced phase locking of molecular levels. This can be understood as the appearance of a novel multilevel dark state. In addition, the experimental methods developed help to determine important properties of our coupled atom/ laser system.
Spontaneous emission by an excited fermionic atom can be suppressed due to the Pauli exclusion principle if the relevant final states after the decay are already occupied by identical atoms in the ground state. Here we discuss a setup where a single atom is prepared in the first excited state on a single site of an optical lattice under conditions of very tight trapping. We investigate these phenomena in the context of two experimental realizations: (1) with alkali-metal atoms, where the decay rate of the excited state is large, and (2) with alkaline-earth-metal-like atoms, where the decay rate from metastable states can be tuned in experiments. This phenomenon has potential applications towards reservoir engineering and dissipative many-body state preparation in an optical lattice.
Coherent dark states in atoms, created by simultaneous interaction of two coherent light fields with a 3-level system, are of prime importance in quantum state manipulation. They are used extensively in quantum sensing and quantum information applications to build atomic clocks, magnetometers, atomic interferometers and more. Here we study the formation and decay of coherent dark-states in an ensemble of laser-cooled free-falling atoms. We measure the optical-pumping rate into the dark-state in the σ+−σ−σ^+-σ^-σ+−σ− polarization configuration. We find that the pumping rate is linear with the optical field intensity, but about an order-of-magnitude slower than the rate predicted by the commonly used, but simplistic, three-level analytic formula. Using a numerical model we demonstrate that this discrepancy is due to the multi-level Zeeman manifold. Taking into account the slower pumping rate we explain quantitatively the relation between the light-shift and the duration of pumping into dark-state in Ramsey spectroscopy. We also measure the decay of the dark-state coherence and find that in our apparatus it is dominated by the mechanical motion of the atoms out of the probing region, while the atomic decoherence is negligible.