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arXiv:2510.05561 · Physical Review A

General dark-state theory for arbitrary multilevel quantum systems

Xuan Zhao, Le-Man Kuang, Jie‐Qiao Liao

Published Dec 23, 2025• 3 citations
arXivHTMLPDF

Abstract

The dark-state effect, caused by destructive quantum interference, is an important physical effect in atomic physics and quantum optics. It not only deepens the understanding of light-atom interactions, but also has wide applications in quantum physics and quantum information. Therefore, how to efficiently and conveniently determine the number and form of the dark states in multilevel quantum systems with complex transitions is an important and interesting topic in this field. In this work, we present a general theory for determining the dark states in multilevel quantum systems with any coupling configuration using the arrowhead-matrix method. To confirm the dark states in a multilevel system, we first define the upper- and lower-state subspaces, and then diagonalize the Hamiltonians restricted within the two subspaces to obtain the dressed upper and lower states. By further expressing the transitions between the dressed upper and lower states, we can map the multilevel system to a bipartite-graph network, in which the nodes and links are acted by the dressed states and transitions, respectively. Based on the coupling configurations of the network, we can determine the lower dark states with respect to the upper-state subspace. As examples, we analyze the dark states in three-, four-, and five-level quantum systems, for all possible configurations through the classification of the numbers of upper and lower states. Furthermore, we extend the framework to multilevel quantum systems and discuss the existence of dark states in some typical configurations. We also recover the results of the dark-state polaritons in driven three-level systems with the arrowhead-matrix method. Our theory paves the way for manipulating and utilizing the dark states of multilevel quantum systems in atomic physics and quantum optics.

DOI
10.1103/k7vj-b3jy

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The dark-state effect, caused by destructive quantum interference, is an important physical effect in atomic physics and quantum optics. It not only deepens the understanding of light-atom interactions, but also has wide applications in quantum physics and quantum information. Therefore, how to efficiently and conveniently determine the number and form of the dark states in multilevel quantum systems with complex transitions is an important and interesting topic in this field. In this work, we present a general theory for determining the dark states in multilevel quantum systems with any coupling configuration using the arrowhead-matrix method. To confirm the dark states in a multilevel system, we first define the upper- and lower-state subspaces, and then diagonalize the Hamiltonians restricted within the two subspaces to obtain the dressed upper and lower states. By further expressing the transitions between the dressed upper and lower states, we can map the multilevel system to a bipartite-graph network, in which the nodes and links are acted by the dressed states and transitions, respectively. Based on the coupling configurations of the network, we can determine the lower dark states with respect to the upper-state subspace. As examples, we analyze the dark states in three-, four-, and five-level quantum systems, for all possible configurations through the classification of the numbers of upper and lower states. Furthermore, we extend the framework to multilevel quantum systems and discuss the existence of dark states in some typical configurations. We also recover the results of the dark-state polaritons in driven three-level systems with the arrowhead-matrix method. Our theory paves the way for manipulating and utilizing the dark states of multilevel quantum systems in atomic physics and quantum optics.
The dark-state effect, caused by destructive interference, not only is an important fundamental research topic in atomic physics and quantum optics, but also has wide potential application in quantum physics and quantum information science. Using the arrowhead-matrix method, here we study the dark-state effect in a coupled cavity-Rydberg-atom system, in which NNN Rydberg atoms with the dipole-dipole interactions are coupled to a single-mode cavity field. We obtain the numbers and form of the dark states in certain excitation-number subspaces for the two-, three-, and four-atom cases, as well as in the single-excitation subspace for a general NNN-atom case. We also suggest to characterize the dark states by inspecting the populations of some specific quantum states, which can be detected in experiments. Furthermore, we analyze the dark-state effect in a realistic case, where both the atomic dipole-dipole interaction strengths and the atom-cavity-field coupling strengths depend on the position of the atoms. Our findings pave the way for studying dark-state physics and applications in the cavity-Rydberg-atom platform.
Fock-state lattices (FSLs) are becoming an emerging research hotspot in quantum physics, not only because the FSLs provide a new perspective for studying atom-field interactions, but also because they build a connection between quantum optics and condensed matter physics. Because of the multiple transition paths in the lattices, an inherent quantum interference effect exists in these systems, and hence finding new quantum-coherent phenomena and exploiting their applications become a significant and desired task in this field. In this work, we study the dark-state effect in the FSLs generated by the multimode Jaynes-Cummings (JC) models. By considering the FSLs in certain excitation-number subspaces, we study the dark states with respect to the states associated with the atomic excited state using the arrowhead-matrix method. We find that dark-state subspaces exist with dimensions determined by the number of orthogonal dark states. When the dimension is greater than one, the forms of these dark-state bases are not unique. Further, we obtain the number and form of the orthogonal dark states in the two-, three-, and four-mode JC models. In addition, we find that for a general N -mode JC model, there are C N + n − 2 N − 2 orthogonal dark states in the n -excitation subspace. We also build the relationship between the dark states and dark modes. Our work paves the way for exploring quantum optical effects and quantum information processing based on the FSLs.
We propose and prove two theorems for determining the number of dark modes in linear two-component quantum networks composed of two types of bosonic modes. This is achieved by diagonalizing the two sub-networks of the same type of modes, mapping the networks to either a standard or a thick arrowhead matrix, and analyzing the linear dependence and independence between the column vectors associated with degenerate normal modes in the coupling matrix. We confirm the two theorems by checking the simultaneous ground-state cooling of the mechanical modes in linearized optomechanical networks. These results also work for linear fermionic networks and other networks described by quadratic coupled-mode Hamiltonian. The present method can be extended to study the dark-state effect in driven atom systems and to construct large decoherence-free subspaces for processing quantum information. This work will initiate the studies on dynamical, transport, and statistical properties of linear networks with decoupled subspaces.
Optical dark resonance in systems with arbitrary multilevels and multiphotons is studied theoretically. When the system configuration is treelike (the term of graph theory), all the coherence terms in the system can be categorized into several groups on dark resonance. It is proved for generic system configurations with arbitrary multilevels that the resonance conditions can be obtained successively by setting the determinant of the submatrix of the Hamiltonian with respect to each group to zero. We calculate, as one of the practical examples, all the conditions of dark resonance of potassium atoms with two laser fields and one rf field mixing one excited state and eight ground states in the hyperfine structure. Although the system configuration is very complicated, the condition is easily obtained in an analytic form and verified by the result of a numerical simulation. Furthermore, our theory can reveal the fine structure of dark lines with power broadening in the observed light-induced-fluorescence spectra and numerical calculations. In addition, the dark lines with the complicated splitting pattern observed in experiments can be assigned to the relevant level configuration and transitions by the present theory. \textcopyright{} 1996 The American Physical Society.
We analyze electromagnetically induced transparency and light storage in an ensemble of atoms with multiple excited levels (multi-$\ensuremath{\Lambda}$ configuration) which are coupled to one of the ground states by quantized signal fields and to the other one via classical control fields. We present a basis transformation of atomic and optical states which reduces the analysis of the system to that of electromagnetically induced transparency in a regular three-level configuration. We demonstrate the existence of dark state polaritons and propose a protocol to transfer quantum information from one optical mode to another by an adiabatic control of the control fields.