We present the first experimental demonstration of quantum enhanced detection at x-ray wavelengths.We show that x-ray pairs that are generated by spontaneous down-conversion can be used for the generation of heralded x-ray photons and directly measure the sub-Poissonian statistics of the single photons by using photon number resolving detectors.We utilize the properties of the strong time-energy correlations of the down-converted photons to demonstrate the ability to improve the visibility and the signal-to-noise ratio of an image with a small number of photons in an environment with a noise level that is higher than the signal by many orders of magnitude.A long-term goal of this work is to demonstrate x-ray photon entanglement.However, given the technical challenges, which are much greater than in the visible regime, we take a first step in demonstrating nonclassical (sub-Poisson) photon correlations.In our work, we demonstrate a new protocol for the measurement of quantum effects with x rays using advantages such as background-free measurements that the x-ray regime offers for experiments aiming at testing fundamental concepts in quantum optics.
We present the first experimental demonstration of quantum enhanced detection at x-ray wavelengths.We show that x-ray pairs that are generated by spontaneous down-conversion can be used for the generation of heralded x-ray photons and directly measure the sub-Poissonian statistics of the single photons by using photon number resolving detectors.We utilize the properties of the strong time-energy correlations of the down-converted photons to demonstrate the ability to improve the visibility and the signal-to-noise ratio of an image with a small number of photons in an environment with a noise level that is higher than the signal by many orders of magnitude.A long-term goal of this work is to demonstrate x-ray photon entanglement.However, given the technical challenges, which are much greater than in the visible regime, we take a first step in demonstrating nonclassical (sub-Poisson) photon correlations.In our work, we demonstrate a new protocol for the measurement of quantum effects with x rays using advantages such as background-free measurements that the x-ray regime offers for experiments aiming at testing fundamental concepts in quantum optics.
Understanding and harnessing X-ray quantum effects could open new, to our knowledge, frontiers in imaging and quantum optics. In this study, we measured the process of X-ray parametric down-conversion, where a single high-energy X-ray photon splits into two lower-energy photons. Using the SACLA X-ray free electron laser in Japan at 9.83 keV, we found clear evidence that pairs of photons were produced along the energy-angle relationship that conserved both energy and momentum, as predicted for down-conversion, and consistent with quantum entanglement of X-ray photons. By matching specific photon pairs for energy and momentum conservation, we observe a signal rate of 1250 pairs per hour, confirming that correlated photon pairs can be generated and observed in the absence of explicit time correlations. Our results show that with further refinement, the number of entangled photons produced per laser pulse could increase by an order of magnitude. This paves the way for demonstrating quantum-enhanced X-ray imaging, and confirmation of X-ray photon entanglement.
Quantum imaging leverages correlations between pairs of photons and has the potential to obtain image information beyond what classical sources provide. Extending this approach to the X-ray regime has been limited by low photon-pair generation rates and the lack of suitable detectors. Here, we demonstrate X-ray coincidence imaging using spontaneous parametric down-conversion (SPDC) and a pixelated area detector with time- and energy-resolved capabilities. This configuration enables simultaneous detection of correlated X-ray photon pairs and coincidence-based imaging of test objects, including a biological specimen. The increased coincidence rate and spatially resolved detection establish a basis for future quantum-enhanced and low-dose X-ray imaging.
Quantum imaging encompasses a broad range of methods that exploit the quantum properties of light to capture information about an object. One such approach involves using a two-photon quantum state, where only one photon interacts with the object being imaged while its entangled partner carries spatial or temporal information. To implement this technique, it is necessary to generate specific quantum states of light and detect photons at the single-photon level. While this method has been successfully demonstrated in the visible electromagnetic spectrum, extending it to X-rays has faced significant challenges due to the difficulties in producing a sufficient rate of X-ray photon pairs and detecting them with adequate resolution. Here, we demonstrate record high rates of correlated X-ray photon pairs produced via a spontaneous parametric down-conversion process and we employ these photons to perform quantum correlation imaging of several objects, including a biological sample (E. cardamomum seedpod). Notably, we report an unprecedented detection rate of about 6,300 pairs per hour and the observation of energy anti-correlation for the X-ray photon pairs. We also present a detailed analysis of the properties of the down-converted X-ray photons, as well as a comprehensive study of the correlation imaging formation, including a study of distortions and corrections. These results mark a substantial advancement in X-ray quantum imaging, expanding the possibilities of X-ray quantum optical technologies, and illustrating the pathway towards enhancing biological imaging with reduced radiation doses.
We investigate the use of correlated photon pair sources for the improved quantum-level detection of a target in the presence of a noise background. Photon pairs are generated by spontaneous four-wave mixing, one photon from each pair (the herald) is measured locally while the other (the signal) is sent to illuminate the target. Following diffuse reflection from the target, the signal photons are detected by a receiver and nonclassical timing correlations between the signal and herald are measured in the presence of a configurable background noise source. Quantum correlations from the photon pair source can be used to provide an enhanced signal-to-noise ratio when compared to a classical light source of the same intensity.
Spontaneous parametric down-conversion is a vital method for generating correlated photon pairs in the visible and near-infrared spectral regions; however, its extension to X-ray frequencies has faced substantial barriers. Here, we present an advancement in correlated X-ray pair generation and detection by employing a two-dimensional pixelated detector to obtain the first direct image of the pair distribution. Our study explores and directly visualizes the down-conversion process, revealing the characteristic ring structure of coincident photon pairs and demonstrating robust spatial correlations. A significant finding is the observation of energy anti-correlation, achieved at an unprecedented rate of approximately 4,100 pairs/hour, far exceeding previous reports in the literature. We believe these results represent a significant leap in X-ray quantum imaging, unlocking the potential for enhanced imaging of biological materials with reduced doses and broadening the applicability of X-ray quantum optical technologies.
Abstract In this review we present the potentialities and the achievements of the use of non-classical photon-number correlations in twin-beam states for many applications, ranging from imaging to metrology. Photon-number correlations in the quantum regime are easily produced and are rather robust against unavoidable experimental losses, and noise in some cases, if compared to the entanglement, where losing one photon can completely compromise the state and its exploitable advantages. Here, we will focus on quantum enhanced protocols in which only phase-insensitive intensity measurements (photon-number counting) are performed, which allow probing the transmission/absorption properties of a system, leading, for example, to innovative target detection schemes in a strong background. In this framework, one of the advantages is that the sources experimentally available emit a wide number of pair-wise correlated modes, which can be intercepted and exploited separately, for example by many pixels of a camera, providing a parallelism, essential in several applications, such as wide-field sub-shot-noise imaging and quantum enhanced ghost imaging. Finally, non-classical correlation enables new possibilities in quantum radiometry, e.g. the possibility of absolute calibration of a spatial resolving detector from the on-off single-photon regime to the linear regime in the same setup.