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arXiv:1905.02379 · Physical Review Research

Determination of universal critical exponents using Lee-Yang theory

Aydin Deger, Christian Flindt

Published Sep 4, 2019• 41 citations
arXivHTMLPDF

Abstract

This article presents a pathway from measurements of partition function zeros to the determination of critical points and universal critical exponents of continuous phase transitions. The method is illustrated in ferromagnetism, but can be applied to other physical systems.
DOI
10.1103/physrevresearch.1.023004

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Yang-Lee edge singularities are the branch point of free energy on the complex plane of physical parameters and have been shown to be the simplest universality class of phase transitions.However, Yang-Lee edge singularities have not been regarded as experimentally observable since they occur at complex physical parameters which are unphysical.A recent discovery regarding the relation between partition functions and probe spin coherence makes it experimentally feasible to access the complex plane of physical parameters.However, how to extract the critical point and the critical exponent of Yang-Lee edge singularities in many-body systems, which occurs only at the thermodynamic limit, has still been elusive.Here we show that the quantum coherence of a probe spin coupled to finite-size Ising-type spin systems presents universal scaling behavior near the Yang-Lee edge singularity.The finite-size scaling behavior of the quantum coherence of the probe spin predicts that one can extract the critical point and the critical exponent of the Yang-Lee edge singularity of an Ising-type spin system in the thermodynamic limit from the spin coherence measurement of the probe spin coupled to finite-size Ising-type spin systems.This finding provides a practical approach to studying the nature of Yang-Lee edge singularities of many-body systems.In 1952, Yang and Lee [1, 2] initiated the examination of phase transitions by studying the partition function zeros, termed Lee-Yang zeros, on the complex plane of a magnetic field h (or fugacity z for fluids).They found that for a system above its critical temperature T c , the partition function must be nonzero throughout some neighborhood of the real axis of the magnetic field within a gap determined by two edges at  ( ) h T YL .Therefore the free energy is an analytic function of the real magnetic field.On the other hand, below the critical temperature T c , the Lee-Yang zeros will come arbitrarily to the real axis as the thermodynamic limit is taken, destroying the analyticity of the free energy in h for those real fields at which the Lee-Yang zeros accumulate.Kortman and Griffiths [3] pointed out that the edges of Lee-Yang zeros of a many-body system in the thermodynamic limit are singularity points, termed Yang-Lee edge singularities [4].Fisher [4] proposed that the Yang-Lee edge singularity could be considered as a new second order phase transition point with associated critical exponents.Renormalization group analyses [4] show that the Yang-Lee edge singularity is associated with an j i 3 theory and the crossover dimensionality of the Yang-Lee edge singularity is d c = 6.Later, the investigation of the Yang-Lee edge singularity has been extended to many other models, such as the classical nvector model [5], the quantum Heisenberg model [5], the spherical model [6], the quantum one-dimensional (1D) transverse Ising model [7], the hierarchical model [8], branched polymers [9], the directed-site animalsenumeration problem [10], Ising models on fractal lattices [11], Ising systems with correlated disorder [12], fluid models with repulsive-core interactions [13], the antiferromagnetic Ising model [14] etc.A comprehensive review of the study of Yang-Lee edge singularities can be found in [15, 16].Recently, Kibble-Zurek scaling was shown to appear at the Yang-Lee edge singularity [17], which supports that the Yang-Lee edge singularity is similar to conventional second order phase transitions.Yang-Lee edge singularity occurs in the ferromagnetic Ising models above its critical temperatures in a purely imaginary magnetic field  h i (figure 1).For  > ( ) h h T YL , the partition function acquires zeros, which becomes dense on the line with > ( ) Ih h T YL .The density of Lee-Yang zeros  ( ) g T h , in the thermodynamic limit behaves as  ~ -s ( ) | ( )| g T h h h T , YL when   ( ) h h T YL from above, with σ being the universal critical

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By an extension of the Yang-Lee picture of phase transitions to the case of two complex variables, we have been able to study the properties of a ferromagnetic system in the vicinity of the critical point. A linear approximation is used, which yields a satisfactory result close to that point. Especially, we see how a critical point and a phase boundary can arise from statistical mechanical laws. It is shown that scaling laws are generally valid, although there may be special cases when they are not.
Renormalization group theory is a powerful and intriguing technique with a wide range of applications. One of the main successes of renormalization group theory is the description of continuous phase transitions and the development of scaling theory. Most courses on phase transitions focus on scaling and critical exponents, while less attention is paid to universality, renormalization group flow, and the existence of a unique fixed point, which are the ultimate reasons why scaling theory is so effective in describing continuous phase transitions. We use a combination of Monte Carlo simulations and real space renormalization group theory to determine the renormalization group flow and to show the existence of a universal fixed point in the context of the ferromagnetic Ising model.
The collective behavior of large numbers of interacting particles may give rise to a phase transition. A continuing challenge is to identify the underlying principles of this phenomenon emerging in many important systems in nature and characterize the critical behavior of interacting many-body systems. In this thesis, we present a theoretical and methodological framework for predicting the phase properties of a macroscopic system based on the behavior of just a few of its constituents. To this end, we devise a direct pathway from the detection of partition function zeros by measuring or simulating fluctuating observables in systems of finite size to the characterization of criticality and large deviation statistics in interacting many-body systems. Our approach combines ideas and concepts from the finite-size scaling analysis with the Lee-Yang formalism and theories of high cumulants and large deviations, and it can be applied in a wide range of critical systems from physics, chemistry, and biology, both in theory and experiment. The thesis consists of four publications. In publications I and II, we report a novel method that makes it possible to extract the partition function zeros in interacting many-body systems of finite size solely from the fluctuations of thermodynamic observables without any prior knowledge of the partition function. To illustrate the feasibility of our approach, we use the Fisher zeros and their relation to the energy fluctuations as a tool for probing criticality in Ising models in two and three dimensions. In particular, we suggest an alternative way of extracting the universal critical exponents from measured fluctuations in finite-size systems away from the phase transition. In publications III and IV, we develop a scaling analysis of the partition function zeros to investigate the criticality in higher dimensions where the hyperscaling breaks down. We also show that even if the system does not exhibit a sharp phase transition, the partition function zeros carry important information about the large-deviation statistics of the system and its symmetry properties. To this end, we determine the rare magnetization fluctuations from the asymptotic behavior of the Lee-Yang zeros, i.e., from the Yang-Lee edge singularities. This finding may constitute a profound connection between Lee-Yang theory and large-deviation statistics.
Yang-Lee edge singularities are the branch point of free energy on the complex plane of physical parameters and have been shown to be the simplest universality class of phase transitions.However, Yang-Lee edge singularities have not been regarded as experimentally observable since they occur at complex physical parameters which are unphysical.A recent discovery regarding the relation between partition functions and probe spin coherence makes it experimentally feasible to access the complex plane of physical parameters.However, how to extract the critical point and the critical exponent of Yang-Lee edge singularities in many-body systems, which occurs only at the thermodynamic limit, has still been elusive.Here we show that the quantum coherence of a probe spin coupled to finite-size Ising-type spin systems presents universal scaling behavior near the Yang-Lee edge singularity.The finite-size scaling behavior of the quantum coherence of the probe spin predicts that one can extract the critical point and the critical exponent of the Yang-Lee edge singularity of an Ising-type spin system in the thermodynamic limit from the spin coherence measurement of the probe spin coupled to finite-size Ising-type spin systems.This finding provides a practical approach to studying the nature of Yang-Lee edge singularities of many-body systems.In 1952, Yang and Lee [1, 2] initiated the examination of phase transitions by studying the partition function zeros, termed Lee-Yang zeros, on the complex plane of a magnetic field h (or fugacity z for fluids).They found that for a system above its critical temperature T c , the partition function must be nonzero throughout some neighborhood of the real axis of the magnetic field within a gap determined by two edges at  ( ) h T YL .Therefore the free energy is an analytic function of the real magnetic field.On the other hand, below the critical temperature T c , the Lee-Yang zeros will come arbitrarily to the real axis as the thermodynamic limit is taken, destroying the analyticity of the free energy in h for those real fields at which the Lee-Yang zeros accumulate.Kortman and Griffiths [3] pointed out that the edges of Lee-Yang zeros of a many-body system in the thermodynamic limit are singularity points, termed Yang-Lee edge singularities [4].Fisher [4] proposed that the Yang-Lee edge singularity could be considered as a new second order phase transition point with associated critical exponents.Renormalization group analyses [4] show that the Yang-Lee edge singularity is associated with an j i 3 theory and the crossover dimensionality of the Yang-Lee edge singularity is d c = 6.Later, the investigation of the Yang-Lee edge singularity has been extended to many other models, such as the classical nvector model [5], the quantum Heisenberg model [5], the spherical model [6], the quantum one-dimensional (1D) transverse Ising model [7], the hierarchical model [8], branched polymers [9], the directed-site animalsenumeration problem [10], Ising models on fractal lattices [11], Ising systems with correlated disorder [12], fluid models with repulsive-core interactions [13], the antiferromagnetic Ising model [14] etc.A comprehensive review of the study of Yang-Lee edge singularities can be found in [15, 16].Recently, Kibble-Zurek scaling was shown to appear at the Yang-Lee edge singularity [17], which supports that the Yang-Lee edge singularity is similar to conventional second order phase transitions.Yang-Lee edge singularity occurs in the ferromagnetic Ising models above its critical temperatures in a purely imaginary magnetic field  h i (figure 1).For  > ( ) h h T YL , the partition function acquires zeros, which becomes dense on the line with > ( ) Ih h T YL .The density of Lee-Yang zeros  ( ) g T h , in the thermodynamic limit behaves as  ~ -s ( ) | ( )| g T h h h T , YL when   ( ) h h T YL from above, with σ being the universal critical