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arXiv:1905.00033 · Physical review. B./Physical review. B

Ferromagnetism and spin-valley liquid states in moiré correlated insulators

Xiao-Chuan Wu, Anna Keselman, Chao‐Ming Jian, Kelly Ann Pawlak, Cenke Xu

Published Jul 22, 2019• 32 citations
arXivHTMLPDF

Abstract

Motivated by the recent observation of evidence of ferromagnetism in correlated insulating states in systems with moir\'e superlattices, we study a two-orbital quantum antiferromagnetic model on the triangular lattice, where the two orbitals physically correspond to the two valleys of the original graphene sheet. For simplicity this model has a $\mathrm{SU}{(2)}^{s}\ensuremath{\bigotimes}\mathrm{SU}{(2)}^{v}$ symmetry, where the two $\mathrm{SU}(2)$ symmetries correspond to the rotation within the spin and valley spaces, respectively. Through analytical argument, Schwinger boson analysis, and also density matrix renormalization group simulation, we find that even though all the couplings in the Hamiltonian are antiferromagnetic, there is still a region in the phase diagram with fully polarized ferromagnetic order. We argue that a Zeeman field can drive a metal-insulator transition in our picture, as was observed experimentally. We also construct spin liquids and topological ordered phases at various limits of this model. Then after doping this model with extra charge carriers, the system most likely becomes a spin-triplet/valley-singlet $d+id$ topological superconductor, as was predicted previously.

DOI
10.1103/physrevb.100.024421

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Abstract The observation of strongly correlated states in moiré systems has renewed the conceptual interest in magnetic systems with higher SU(4) spin symmetry, e.g., to describe Mott insulators where the local moments are coupled spin–valley degrees of freedom. Here, we discuss a numerical renormalization group scheme to explore the formation of spin–valley ordered and unconventional spin–valley liquid states at zero temperature based on a pseudo-fermion representation. Our generalization of the conventional pseudo-fermion functional renormalization group approach for su{{\mathfrak {s}}}{{\mathfrak {u}}}su s u (2) spins is capable of treating diagonal and off-diagonal couplings of generic spin–valley exchange Hamiltonians in the self-conjugate representation of the su{{\mathfrak {s}}}{{\mathfrak {u}}}su s u (4) algebra. To achieve proper numerical efficiency, we derive a number of symmetry constraints on the flow equations that significantly limit the number of ordinary differential equations to be solved. As an example system, we investigate a diagonal SU(2) spin_{\text {spin}}spin​ spin ⊗\otimes ⊗ ⊗ U(1) valley_{\text {valley}}valley​ valley model on the triangular lattice which exhibits a rich phase diagram of spin and valley ordered phases. Graphic Abstract
Recent advances in moiré engineering motivate the study of lattice models of strongly-correlated electrons subjected to substantial orbital magnetic flux. We analyze the triangular lattice Hofstadter-Hubbard model at one-quarter flux quantum per plaquette and a density of one electron per site, where a chiral spin liquid phase may exist between weak-coupling integer quantum Hall and strong-coupling 120∘^\circ∘ antiferromagnetic phases. We use matrix product state methods and analytical arguments to investigate this model compactified to cylinders of finite circumference. We uncover a glide particle-hole symmetry operation which, we argue, is spontaneously broken at the quantum Hall to spin liquid transition on odd-circumference cylinders. We numerically verify the spontaneous symmetry breaking and further demonstrate that this transition is associated with algebraic long-range correlations of various spin-singlet, charge-neutral operators. For even-circumference cylinders, the transition becomes a crossover associated with a large correlation length that grows substantially with circumference. Our findings suggest that in the two-dimensional limit, the transition to a chiral spin liquid phase is continuous and features critical fluctuations of the current.
Twisted transition metal dichalcogenides offer an exceptionally tunable moiré platform for studying correlation physics beyond conventional condensed matter systems. In particular, the intriguing interplay between the displacement field and the twist angle remains to be fully resolved. In this paper, we use large-scale density matrix renormalization group simulations to study the minimal moiré Hubbard model on a triangular lattice at half-filling, where the displacement field effect is captured by a spin-dependent staggered flux. We find that the displacement field significantly enriches the triangular Hubbard phase diagram in several qualitative ways. It rapidly destabilizes the chiral spin liquid phase beyond a narrow weak-field regime, induces pronounced chiral correlations in the strong-coupling 120∘120^\circ120∘-antiferromagnetic phase, and stabilizes incommensurate spin-density wave phases at weaker coupling. We further find signatures of a continuous transition between the chiral spin liquid and chiral antiferromagnetic phases at a finite displacement field, potentially driven by spinon condensation. Our results uncover rich displacement-field-driven many-body physics and provide useful guidance for future experiments in moiré superlattice systems.
Moiré systems provide a rich platform for studies of strong correlation physics. Recent experiments on heterobilayer transition metal dichalcogenide Moiré systems are exciting in that they manifest a relatively simple model system of an extended Hubbard model on a triangular lattice. Inspired by the prospect of the hetero-transition metal dichalcogenide Moiré system's potential as a solid-state-based quantum simulator, we explore the extended Hubbard model on the triangular lattice using the density matrix renormalization group. Specifically, we explore the two-dimensional phase space spanned by the key tuning parameters in the extended Hubbard model, namely, the kinetic energy strength and the further-range Coulomb interaction strengths. We find competition between Fermi fluid, chiral spin liquid, spin density wave, and charge order. In particular, our finding of the optimal further-range interaction for the chiral correlation presents a tantalizing possibility.
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