Broadband quadrature-squeezed vacuum and nonclassical photon number correlations from a nanophotonic device
Varun Vaidya, B. Morrison, L. G. Helt, R. Shahrokshahi, D. H. Mahler, M. J. Collins, K. Tan, J. Lavoie, A. Repingon, M. Menotti, N. Quesada, R. C. Pooser, A. E. Lita, T. Gerrits, S. W. Nam, Z. Vernon
as high as 1.95(1). Multiphoton events of over 10 photons are directly detected with rates exceeding any previous quantum optical demonstration using integrated nanophotonics. These results will have an enabling impact on scaling continuous variable quantum technology.
Squeezed light are optical beams with variance below the Shot Noise Level. They are a key resource for quantum technologies based on photons, they can be used to achieve better precision measurements, improve security in quantum key distribution channels and as a fundamental resource for quantum computation. To date, the majority of experiments based on squeezed light have been based on non-linear crystals and discrete optical components, as the integration of quadrature squeezed states of light in a nanofabrication-friendly material is a challenging technological task. Here we measure 0.45 dB of GHz-broad quadrature squeezing produced by a ring resonator integrated on a Silicon Nitride photonic chip that we fabricated with CMOS compatible steps. The result corrected for the off-chip losses is estimated to be 1 dB below the Shot Noise Level. We identify and verify that the current results are limited by excess noise produced in the chip, and propose ways to reduce it. Calculations suggest that an improvement in the optical properties of the chip achievable with existing technology can develop scalable quantum technologies based on light.
Abstract Growing interest in quantum computing for practical applications has led to a surge in the availability of programmable machines for executing quantum algorithms1, 2. Present-day photonic quantum computers3–7 have been limited either to non-deterministic operation, low photon numbers and rates, or fixed random gate sequences. Here we introduce a full-stack hardware−software system for executing many-photon quantum circuit operations using integrated nanophotonics: a programmable chip, operating at room temperature and interfaced with a fully automated control system. The system enables remote users to execute quantum algorithms that require up to eight modes of strongly squeezed vacuum initialized as two-mode squeezed states in single temporal modes, a fully general and programmable four-mode interferometer, and photon number-resolving readout on all outputs. Detection of multi-photon events with photon numbers and rates exceeding any previous programmable quantum optical demonstration is made possible by strong squeezing and high sampling rates. We verify the non-classicality of the device output, and use the platform to carry out proof-of-principle demonstrations of three quantum algorithms: Gaussian boson sampling, molecular vibronic spectra and graph similarity8. These demonstrations validate the platform as a launchpad for scaling photonic technologies for quantum information processing.
Photonics offers the potential for large-scale, room-temperature, and ultrafast quantum operations. Multiplexing pulses of light allows for high throughput speeds and dense encoding, with tens of thousands of optical modes being present in a time as short as a microsecond. However, the measurement speed of electronic devices such as photodetectors is currently one bottleneck in such time-multiplexed scalability, because many quantum optical protocols rely on measurement, including state preparation, feed-forward, and feedback. Furthermore, characterization of quantum states and modes is essential for their effective use. Using nanophotonic optical parametric amplifiers (OPAs) presents one way to circumvent the measurement limitations of current quantum photonic schemes. Their large amplification bandwidth, enabled by dispersion engineering on nanophotonic integrated platforms, allows information encoded in femtosecond-scale, THz-bandwidth, multimode quantum optical states to be accessed with nonlinear optical interactions. In this work, we show how ultra-broadband integrated nanophotonic OPAs can be used to measure ultrafast and multimode quantum states of light. First, we explore the single-photon detection capabilities of OPAs, showing that current OPAs operating in the Gaussian regime are capable of 250 MHz photon count rates with 26% efficiency and a 2% dark count probability. We also show how non-Gaussian operation through pump depletion, with performance that approaches state-of-the-art photon detectors in terms of efficiency and dark count rate while retaining ultrafast operation, can become experimentally possible with a higher nonlinear coupling rate and lower loss. Next, we use nanophotonic OPAs to both generate and characterize multimode ultrafast squeezed vacuum. We use the photocurrent distribution of amplified squeezed vacuum to recover 2.41 dB of squeezing in one mode of a 154-fs multimode squeezed pulse and reconstruct its Wigner distribution. Finally, we investigate the capabilities of broadband nanophotonic OPAs to determine the temporal mode structure and quadrature variances of ultra-broadband temporally multimode quantum states by adapting frequency-resolved optical gating to the quantum regime. We numerically show the successful full characterization of a multimode squeezed state, even in the presence of noise. Together, these results establish OPAs as a valuable measurement device for measuring ultrafast quantum pulses and learning the structure of multimode quantum states, and they provide one building block towards a framework for scalable continuous-variable quantum photonics in which state generation, manipulation, and characterization occur within the same nanophotonic platform.
Optical quantum information science plays a central role in the development of advanced photonic technologies, with applications ranging from quantum imaging and communication to continuous-variable (CV) quantum computing. The efficient realization of these technologies depends not only on the generation of nonclassical states of light but also on their proper detection. Optical parametric amplification (OPA) has long been known as both a fundamental nonlinear process for generating nonclassical light and as a method to boost detection efficiency through pre-amplification. Recently, OPA has been revisited as a tool for all-optical quadrature detection, offering a powerful alternative to conventional homodyne detection by enabling broadband, loss-tolerant squeezing measurements across various optical platforms. In this thesis, I establish optical parametric amplification as a versatile tool for the detection of CV quantum states through all-optical quadrature detection. I extend squeezing detection to high-dimensional scenarios by exploiting the intrinsic multimode nature of OPA, thereby enabling, for the first time to the best of my knowledge, the real-time monitoring of multimode squeezed light, a long-standing challenge in quantum optics. This approach further permits the simultaneous monitoring of multiple CV Einstein–Podolsky–Rosen (EPR) mode pairs, providing a framework for scalable detection of multimode entanglement, namely optical cluster states, which constitute essential resources for CV quantum computing. Furthermore, I demonstrate OPA as a platform for loss-tolerant and broadband quantum state tomography, applying it to both Gaussian and non-Gaussian states. This paves the way for the scalable tomography of multimode quantum states. Finally, I show that OPA enables the certification of the non-Gaussian and nonclassical character of quantum states without the need for photon-number-resolving detectors, relying instead on post-amplification intensity statistics. In particular, I amplify a single photon sufficiently strongly that its non-Gaussian character becomes accessible through conventional intensity detectors. Altogether, this work establishes optical parametric amplification as a powerful and scalable platform for high-dimensional continuous-variable optical quantum technologies.