Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1904.06233 · Physical Review Letters

Recovering the Homogeneous Absorption of Inhomogeneous Media

Ohr Lahad, Ran Finkelstein, Omri Davidson, Ohad Michel, Eilon Poem, Ofer Firstenberg

Published Oct 25, 2019• 19 citations
arXivHTMLPDF

Abstract

The resonant absorption of light by an ensemble of absorbers decreases when the resonance is inhomogeneously broadened. Recovering the lost absorption cross section is of great importance for various applications of light-matter interactions, particularly in quantum optics, but no recovery mechanism has yet been identified and successfully demonstrated. Here, we formulate the limit set by the inhomogeneity on the absorption, and present a mechanism able to circumvent this limit and fully recover the homogeneous absorption of the ensemble. We experimentally study this mechanism using two different level schemes in atomic vapors and demonstrate up to fivefold enhancement of the absorption above the inhomogeneous limit. Our scheme relies on light shifts induced by auxiliary fields and is thus applicable to various physical systems and inhomogeneity mechanisms.

DOI
10.1103/physrevlett.123.173203

Related papers

Quantum Memory for Light

Jean-Louis Le Gouët

We ouline two strategies for storage and recovery of quantum light in an ensemble of atoms. This series of lectures has been devised as an elementary introduction. Hence discussion is essentially confined to a semi-classical picture. We first consider electromagnetically induced transparency (EIT) and stopped light. The roles of homogeneous and inhomogeneous broadening are examined. We propose both time- and frequency-domain descriptions. Then we discuss the total recall of a signal after capture by an absorbing material. Rephasing processes are briefly reviewed. We refer to various recent experimental works, especially those conducted in solid state media. The course is intended to be self contained and includes reminders on some quantum physics elements such as the density operator and the Bloch vector.

•Nov 13, 2007•0 citations

Fully Tunable Photonic Structures In Homogeneous Absorbing Media.

M. Artoni, Giuseppe Carlo La Rocca

Resonantly absorbing media supporting electromagnetically induced transparency may give rise to specific periodic patterns where a light probe is found to experience a fully developed photonic band-gap yet with negligible absorption everywhere. Accurate and efficient coherent optical control of the gap can be accomplished while the remarkable experimental simplicity of the control scheme would ease quantum nonlinear optics applications.

The Rochester Conferences on Coherence and Quantum Optics and the Quantum Information and Measurement meeting•Jan 1, 2007•0 citations

Enhancing electromagnetically-induced transparency in a multilevel broadened medium

Michael S. Scherman, O. S. Mishina, Pietro Lombardi +2 more

Electromagnetically-induced transparency has become an important tool to control the optical properties of dense media. However, in a broad class of systems, the interplay between inhomogeneous broadening and the existence of several excited levels may lead to a vanishing transparency. Here, by identifying the underlying physical mechanisms resulting in this effect, we show that transparency can be strongly enhanced. We thereby demonstrate a 5-fold enhancement in a room-temperature vapor of alkali-metal atoms via a specific shaping of the atomic velocity distribution.

arXiv:1106.0988•Optics Express•Feb 7, 2012•22 citations

Two-Photon Absorption

Isabel Pérez–Arjona, Germán J. de Valcárcel, Eugenio Roldán

Two-photon absorption is theoretically analyzed within the semiclassical formalism of radiation-matter interaction. We consider an ensemble of inhomogeneously broadened three-level atoms subjected to the action of two counterpropagating fields of the same frequency. By concentrating in the limit of large detuning in one-photon transitions, we solve perturbatively the Bloch equations in a non-usual way. In this way we derive an analytical expression for the width of the two-photon resonance that makes evident sub-Doppler two--photon spectroscopy. We also derive an analytical expression for the Stark shift of the two-photon resonance.

arXiv:quant-ph/0402155•Feb 20, 2004•0 citations

Photon storage in Λ -type optically dense atomic media. III. Effects of inhomogeneous broadening

Alexey Vyacheslavovich Gorshkov, Axel André, Mikhail D. Lukin +1 more

In a recent paper [Gorshkov et al., Phys. Rev. Lett. 98, 123601 (2007)] and in the two preceding papers [Gorshkov et al., this issue, Phys. Rev. A 76, 033804 (2006); 76, 033805 (2006)], we used a universal physical picture to optimize and demonstrate equivalence between a wide range of techniques for storage and retrieval of photon wave packets in homogeneously broadened $\ensuremath{\Lambda}$-type atomic media, including the adiabatic reduction of the photon group velocity, pulse-propagation control via off-resonant Raman techniques, and photon-echo-based techniques. In the present paper, we generalize this treatment to include inhomogeneous broadening. In particular, we consider the case of Doppler-broadened atoms and assume that there is a negligible difference between the Doppler shifts of the two optical transitions. In this situation, we show that, at high enough optical depth, all atoms contribute coherently to the storage process as if the medium were homogeneously broadened. We also discuss the effects of inhomogeneous broadening in solid state samples. In this context, we discuss the advantages and limitations of reversing the inhomogeneous broadening during the storage time, as well as suggest a way for achieving high efficiencies with a nonreversible inhomogeneous profile.

arXiv:quant-ph/0612084•Physical Review A•Sep 7, 2007•76 citations

Nonlinear saturated absorption in resonant media: Level-degeneracy-induced polarization effects

Govind Prasad Agrawal

The effect of level degeneracy on saturated absorption in a resonant medium is considered using a simple but realistic three-level system to model $J=1\ensuremath{\rightarrow}J=0$ atomic transition. Assuming homogeneous broadening and exact resonance, an analytic nonperturbative expression for the medium susceptibility is obtained and used to study propagation of an arbitrarily polarized optical field. Optical saturation affects considerably Zeeman-coherence-induced circular dichroism. The analysis may find application in high-resolution spectroscopy and other branches of nonlinear optics.

Physical Review A•Feb 1, 1984•13 citations
The resonant absorption of light by an ensemble of absorbers decreases when the resonance is inhomogeneously broadened. Recovering the lost absorption cross section is of great importance for various applications of light-matter interactions, particularly in quantum optics, but no recovery mechanism has yet been identified and successfully demonstrated. Here, we formulate the limit set by the inhomogeneity on the absorption, and present a mechanism able to circumvent this limit and fully recover the homogeneous absorption of the ensemble. We experimentally study this mechanism using two different level schemes in atomic vapors and demonstrate up to fivefold enhancement of the absorption above the inhomogeneous limit. Our scheme relies on light shifts induced by auxiliary fields and is thus applicable to various physical systems and inhomogeneity mechanisms.
We ouline two strategies for storage and recovery of quantum light in an ensemble of atoms. This series of lectures has been devised as an elementary introduction. Hence discussion is essentially confined to a semi-classical picture. We first consider electromagnetically induced transparency (EIT) and stopped light. The roles of homogeneous and inhomogeneous broadening are examined. We propose both time- and frequency-domain descriptions. Then we discuss the total recall of a signal after capture by an absorbing material. Rephasing processes are briefly reviewed. We refer to various recent experimental works, especially those conducted in solid state media. The course is intended to be self contained and includes reminders on some quantum physics elements such as the density operator and the Bloch vector.
Electromagnetically-induced transparency has become an important tool to control the optical properties of dense media. However, in a broad class of systems, the interplay between inhomogeneous broadening and the existence of several excited levels may lead to a vanishing transparency. Here, by identifying the underlying physical mechanisms resulting in this effect, we show that transparency can be strongly enhanced. We thereby demonstrate a 5-fold enhancement in a room-temperature vapor of alkali-metal atoms via a specific shaping of the atomic velocity distribution.
Two-photon absorption is theoretically analyzed within the semiclassical formalism of radiation-matter interaction. We consider an ensemble of inhomogeneously broadened three-level atoms subjected to the action of two counterpropagating fields of the same frequency. By concentrating in the limit of large detuning in one-photon transitions, we solve perturbatively the Bloch equations in a non-usual way. In this way we derive an analytical expression for the width of the two-photon resonance that makes evident sub-Doppler two--photon spectroscopy. We also derive an analytical expression for the Stark shift of the two-photon resonance.
In a recent paper [Gorshkov et al., Phys. Rev. Lett. 98, 123601 (2007)] and in the two preceding papers [Gorshkov et al., this issue, Phys. Rev. A 76, 033804 (2006); 76, 033805 (2006)], we used a universal physical picture to optimize and demonstrate equivalence between a wide range of techniques for storage and retrieval of photon wave packets in homogeneously broadened $\ensuremath{\Lambda}$-type atomic media, including the adiabatic reduction of the photon group velocity, pulse-propagation control via off-resonant Raman techniques, and photon-echo-based techniques. In the present paper, we generalize this treatment to include inhomogeneous broadening. In particular, we consider the case of Doppler-broadened atoms and assume that there is a negligible difference between the Doppler shifts of the two optical transitions. In this situation, we show that, at high enough optical depth, all atoms contribute coherently to the storage process as if the medium were homogeneously broadened. We also discuss the effects of inhomogeneous broadening in solid state samples. In this context, we discuss the advantages and limitations of reversing the inhomogeneous broadening during the storage time, as well as suggest a way for achieving high efficiencies with a nonreversible inhomogeneous profile.
The effect of level degeneracy on saturated absorption in a resonant medium is considered using a simple but realistic three-level system to model $J=1\ensuremath{\rightarrow}J=0$ atomic transition. Assuming homogeneous broadening and exact resonance, an analytic nonperturbative expression for the medium susceptibility is obtained and used to study propagation of an arbitrarily polarized optical field. Optical saturation affects considerably Zeeman-coherence-induced circular dichroism. The analysis may find application in high-resolution spectroscopy and other branches of nonlinear optics.