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arXiv:1904.00016 · Physical Review Letters

Photon Pair Condensation by Engineered Dissipation

Ze-Pei Cian, Guanyu Zhu, Su-Kuan Chu, Alireza Seif, Wade DeGottardi, Liang Jiang, Mohammad Hafezi

Published Aug 6, 2019• 14 citations
arXivHTMLPDF

Abstract

Dissipation can usually induce detrimental decoherence in a quantum system. However, engineered dissipation can be used to prepare and stabilize coherent quantum many-body states. Here, we show that, by engineering dissipators containing photon pair operators, one can stabilize an exotic dark state, which is a condensate of photon pairs with a phase-nematic order. In this system, the usual superfluid order parameter, i.e., single-photon correlation, is absent, while the photon pair correlation exhibits long-range order. Although the dark state is not unique due to multiple parity sectors, we devise an additional type of dissipators to stabilize the dark state in a particular parity sector via a diffusive annihilation process which obeys Glauber dynamics in an Ising model. Furthermore, we propose an implementation of these photon pair dissipators in circuit-QED architecture.

DOI
10.1103/physrevlett.123.063602

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Dissipation can usually induce detrimental decoherence in a quantum system. However, engineered dissipation can be used to prepare and stabilize coherent quantum many-body states. Here, we show that, by engineering dissipators containing photon pair operators, one can stabilize an exotic dark state, which is a condensate of photon pairs with a phase-nematic order. In this system, the usual superfluid order parameter, i.e., single-photon correlation, is absent, while the photon pair correlation exhibits long-range order. Although the dark state is not unique due to multiple parity sectors, we devise an additional type of dissipators to stabilize the dark state in a particular parity sector via a diffusive annihilation process which obeys Glauber dynamics in an Ising model. Furthermore, we propose an implementation of these photon pair dissipators in circuit-QED architecture.
Understanding the mechanism through which an open quantum system exchanges information with an environment is central to the creation and stabilization of quantum states. This theme has been explored recently, with attention mostly focused on system control or environment engineering. Here, we bring these ideas together to describe the many-body dynamics of an extended atomic array coupled to a squeezed vacuum. We show that fluctuations can drive the array into a pure dark state decoupled from the environment. The dark state is obtained for an even number of atoms and consists of maximally entangled atomic pairs, or dimers, that mimic the behavior of the squeezed field. Each pair displays reduced fluctuations in one polarization quadrature and amplified in another. This dissipation-induced stabilization relies on an efficient transfer of correlations between pairs of photons and atoms. It uncovers the mechanism through which squeezed light causes an atomic array to self-organize and illustrates the increasing importance of spatial correlations in modern quantum technologies where many-body effects play a central role.
Modern quantum platforms such as superconducting circuits offer exciting opportunities for the experimental exploration of driven-dissipative many-body systems in unconventional regimes. One such regime arises in bosonic systems, where driving and dissipation can nowadays be engineered through pairs of excitations, rather than through conventional single-excitation or linear processes. These platforms also enable collective rather than local pair loss, so that excitations emitted into the environment originate from a coherent superposition of lattice sites rather than any specific site. In this work, we analyze the superfluid phases accessible to bosonic arrays subject to these novel mechanisms, which are more characteristic of quantum optics, and show that they lead to remarkable spatiotemporal properties beyond the traditional scope of pattern formation in either condensed-matter systems or nonlinear optics alone. In particular, we show that, even in the presence of residual local loss, the system is stabilized into an exotic state in which bosons condense along the modes of a closed manifold in Fourier space. A weak bias drive controls the population distribution across these modes, providing access to a wealth of patterns: from periodic and quasiperiodic structures with tunable spatial wavelengths to condensates that uniformly populate the closed Fourier manifold. Furthermore, when residual local linear dissipation is balanced by pumping, new constants of motion emerge that can force the superfluid to oscillate in time, through a mechanism analogous to that underlying recently discovered superfluid time crystals. Finally, we propose a specific experimental implementation for exploring this rich and unusual spatiotemporal superfluid behavior.
Non-Gaussian quantum states have been deterministically prepared and autonomously stabilized in single-and two-mode circuit quantum electrodynamics architectures via engineered dissipation.However, it is currently unknown how to scale up this technique to multimode non-Gaussian systems.Here, we upgrade dissipation engineering to collective (normal) modes of nonlinear resonator arrays and show how to stabilize multimode Schrödinger cat states.These states are multiphoton and multimode quantum superpositions of coherent states in a single normal mode delocalized over an arbitrary number of cavities.We consider tailored dissipative coupling between resonators that are parametrically driven and feature an on-site nonlinearity, which is either a Kerr-type nonlinearity or an engineered two-photon loss.For both types of nonlinearity, we find the same exact closed-form solutions for the two-dimensional steady-state manifold spanned by superpositions of multimode Schrödinger cat states.We further show that, in the Zeno limit of strong dissipative coupling, the even-parity multimode cat state can be deterministically prepared from the vacuum.Remarkably, engineered two-photon loss gives rise to a fast relaxation toward the steady state, protecting the state preparation against decoherence due to intrinsic single-photon losses and imperfections in tailored dissipative coupling, which sets in at longer times.The relaxation time is independent of system size making the state preparation scalable.Multimode cat states are naturally endowed with a noise bias that increases exponentially with system size and can thus be exploited for enhanced robust encoding of quantum information.
The photon blockade is a key quantum-nonlinear effect in which the admission of a second photon to a resonator is inhibited, enabling on-demand single-photon emission. Its practical use is limited by the weak intrinsic nonlinearity of most optical platforms. We address this limitation in a coupled-cavity architecture by engineering two-photon dissipation as a control resource rather than a detrimental loss. Within a quantum-master-equation framework, we model single-photon loss, engineered two-photon decay, and pure dephasing, and analyze their joint impact on the steady-state statistics of the driven cavities. We track the zero-delay correlation, photon populations, and detuning/drive dependences under distinct driving schemes (both cavities driven vs. single-cavity drive with. The results show that adding two-photon dissipation (i) suppresses multiphoton occupation and strengthens antibunching, (ii) broadens the operating window in detuning and drive amplitude, and (iii) improves robustness against moderate dephasing and device imperfections. A mechanism analysis attributes these gains to interference between coherent second-order processes and dissipative selection that stabilizes the odd-photon manifold. The study yields design guidelines for realizing stable, cavity-based single-photon sources using dissipation engineering.
Three-level atomic systems coupled to light have the capacity to host dark states. We study a system of V-shaped three-level atoms coherently coupled to the two quadratures of a dissipative cavity. The interplay between the atomic level structure and dissipation makes the phase diagram of the open system drastically different from the closed one. In particular, it leads to the stabilization of a continuous family of dark and nearly dark excited many-body states with inverted atomic populations as the steady states. The multistability of these states can be probed via their distinct fluctuations and excitation spectra, as well as the system's Liouvillian dynamics which are highly sensitive to ramp protocols. Our model can be implemented experimentally by encoding the two higher-energy modes in orthogonal density-modulated states in a bosonic quantum gas. This implementation offers prospects for potential applications like the realization of quantum optical random walks and microscopy with subwavelength spatial resolution.
Modern experimental platforms such as superconducting circuit arrays call for the exploration of bosonic tight-binding models in unconventional situations with no counterpart in real materials. Here we investigate one such situation in which excitations are driven and damped by pairs, leading to pattern formation and exotic bosonic states emerging from a nonequilibrium quantum many-body system. Focusing on a two-dimensional driven-dissipative Bose-Hubbard model, we find that its steady states are characterized by the condensation of bosons around momenta lying on a "Bose surface," a bosonic analog of the Fermi surface in solid-state systems. The interplay between instabilities generated by the driving, the nonlinear dissipative mode coupling, and the underlying lattice effect allows the system to equilibrate into an exotic superfluid state of bosons condensed on a closed ring in momentum space instead of discrete points. Such an unconventional state with a spatially uniform density distribution goes beyond the traditional scope of pattern formation and thus has no counterpart in the classical literature. In addition, it is a state connected to several open problems in modern condensed-matter physics. Here we provide the means to stabilize it, opening the way to its experimental study. Moreover, we also provide a concrete experimental implementation of our model in currently available superconducting circuit arrays. We also investigate the relaxation spectrum around the condensate, which shows a characteristic purely diffusive behavior.