Understanding the mechanism through which an open quantum system exchanges information with an environment is central to the creation and stabilization of quantum states. This theme has been explored recently, with attention mostly focused on system control or environment engineering. Here, we bring these ideas together to describe the many-body dynamics of an extended atomic array coupled to a squeezed vacuum. We show that fluctuations can drive the array into a pure dark state decoupled from the environment. The dark state is obtained for an even number of atoms and consists of maximally entangled atomic pairs, or dimers, that mimic the behavior of the squeezed field. Each pair displays reduced fluctuations in one polarization quadrature and amplified in another. This dissipation-induced stabilization relies on an efficient transfer of correlations between pairs of photons and atoms. It uncovers the mechanism through which squeezed light causes an atomic array to self-organize and illustrates the increasing importance of spatial correlations in modern quantum technologies where many-body effects play a central role.
Understanding the mechanism through which an open quantum system exchanges information with an environment is central to the creation and stabilization of quantum states. This theme has been explored recently, with attention mostly focused on system control or environment engineering. Here, we bring these ideas together to describe the many-body dynamics of an extended atomic array coupled to a squeezed vacuum. We show that fluctuations can drive the array into a pure dark state decoupled from the environment. The dark state is obtained for an even number of atoms and consists of maximally entangled atomic pairs, or dimers, that mimic the behavior of the squeezed field. Each pair displays reduced fluctuations in one polarization quadrature and amplified in another. This dissipation-induced stabilization relies on an efficient transfer of correlations between pairs of photons and atoms. It uncovers the mechanism through which squeezed light causes an atomic array to self-organize and illustrates the increasing importance of spatial correlations in modern quantum technologies where many-body effects play a central role.
We show how the directional collective response of atomic arrays to light can be exploited for the dissipative generation of entangled atomic states, relevant for, e.g., quantum metrology. We consider an atomic array illuminated by a paraxial beam of a squeezed-vacuum field and demonstrate that quantum-squeezing correlations are dissipatively transferred to the array atoms, resulting in an atomic spin-squeezed steady state. We find that the entanglement transfer efficiency and hence the degree of spin squeezing are determined by the resonant optical reflectivity of the array. Considering realistic cases of finite-size array and illuminating beam, we find how the spin-squeezing strength scales with system parameters, such as the number of layers in the array and its spatial overlap with the beam. We discuss applications in atomic clocks in both optical and microwave domains.
The interaction between light and matter has captivated physicists for centuries, from early studies of vision and refraction in ancient Greece to the development of quantum mechanics and quantum electrodynamics in the past century. While the response of a single quantum emitter to light is well understood, the radiative properties of an ensemble of closely spaced emitters are far more intricate. Coupling to a shared electromagnetic environment induces coherent and dissipative interactions between emitters, giving rise to a collective response that cannot be captured by treating them independently. In the regime of few excitations, the system hosts delocalized subradiant states, that is, coherent superpositions that are largely decoupled from the electromagnetic field and thus decay at suppressed rates. While this weak coupling makes subradiant states attractive for quantum technologies, it also renders them difficult to manipulate. At higher excitation densities, the intrinsic nonlinearity of emitters and the exponential growth of the Hilbert space make theoretical and numerical descriptions of the system and its dynamics increasingly challenging. This thesis explores two fundamental questions: How can subradiant and dark states be selectively accessed and harnessed for practical applications in quantum technologies? And how can interacting ensembles of quantum emitters be efficiently simulated to uncover their many-body physics? The first part of the thesis develops protocols for controlling and addressing dark states in free-space and waveguide-coupled atomic arrays, demonstrating their utility in quantum storage and the deterministic generation of entangled photonic states. Incorporating atomic motion, we further show that collective subradiant states can enhance cooling in dense atomic arrays, offering new avenues for controlling motional dynamics. In the second part, we introduce cumulant expansions of the equations of motion as a powerful tool to analytically and numerically investigate collective decay in the many-body regime. We first examine the collective decay of fully excited atomic arrays in free space, characterizing the onset and scaling of the superradiant burst across different geometries. In collaboration with experiments on ultracold erbium atoms in optical lattices, we provide the first direct observations of many-body collective effects in free-space ordered arrays, including early-time superradiant bursts, late-time subradiant tails, and the emergence of atomic correlations throughout the dynamics. Finally, we theoretically and numerically explore the transient formation of multi-excitation subradiant states, and demonstrate how the existence of multiple dissipation channels suppresses steady-state superradiance in extended arrays.
Three-level atomic systems coupled to light have the capacity to host dark states. We study a system of V-shaped three-level atoms coherently coupled to the two quadratures of a dissipative cavity. The interplay between the atomic level structure and dissipation makes the phase diagram of the open system drastically different from the closed one. In particular, it leads to the stabilization of a continuous family of dark and nearly dark excited many-body states with inverted atomic populations as the steady states. The multistability of these states can be probed via their distinct fluctuations and excitation spectra, as well as the system's Liouvillian dynamics which are highly sensitive to ramp protocols. Our model can be implemented experimentally by encoding the two higher-energy modes in orthogonal density-modulated states in a bosonic quantum gas. This implementation offers prospects for potential applications like the realization of quantum optical random walks and microscopy with subwavelength spatial resolution.
Abstract Quantum technologies critically rely on maintaining coherence and controllable correlations in open systems, yet these resources are fragile under dissipation and noise. To address this challenge, we investigate a hybrid platform composed of two identical three-level atoms in a V-type configuration coupled to a single-mode cavity field prepared in a squeezed coherent state. Using the Lindblad master equation, we numerically simulate the system dynamics, allowing a rigorous treatment of coherent atom–field interactions, interatomic couplings, and cavity losses. Our analysis reveals that squeezing introduces nonclassical correlations that enhance field coherence and support the generation of entanglement under specific regimes. Strong interatomic coupling stabilizes entanglement, while squeezing mitigates decoherence-induced losses. Conversely, large photon amplitudes and cavity dissipation degrade both coherence and bipartite correlations. Quantum steering emerges as the most fragile correlation, yet its persistence can be moderately extended through squeezing. These results identify squeezing and interatomic interactions as complementary resources for optimizing coherence, entanglement, and steering, offering practical strategies for robust quantum communication, information processing, and engineered nonclassical states.
Quantum mechanics is fundamentally governed by the Schrödinger equation, which is linear in the wave function. Nevertheless, quantum systems can exhibit highly nonlinear behavior in their observable dynamics. Such nonlinearities can emerge from many-body interactions, nonlinear coupling mechanisms, or the interplay between coherent evolution and dissipation. In the collective limit, microscopic quantum interactions can give rise to qualitatively new macroscopic behavior. Open quantum systems provide a rich setting for such phenomena, as environmental coupling introduces dissipation and fluctuations that compete with coherent dynamics and can alter the steady states and dynamical phases of a system. Combined with nonlinear interactions, this competition can produce behavior with no direct counterpart in conventional linear light--matter systems. In this thesis, I investigate such collective phenomena through nonlinear two-photon light--matter interactions and engineered quantum reservoirs. I first investigate the driven--dissipative two-photon Dicke model and demonstrate the emergence of a dissipative superradiant phase transition. The quadratic light--matter interaction introduces distinct stability requirements in the presence of dissipation. In particular, two-photon loss stabilizes the superradiant phase, allowing its steady states and critical behavior to be characterized. I next investigate photon blockade and transient quadrature-squeezed radiation in the two-photon Tavis--Cummings model. I show that two-photon interactions collectively enhance photon blockade and squeezing, in contrast to the conventional one-photon model, where the effective nonlinearity diminishes in the collective limit. Finally, I consider collective behavior induced by reservoir engineering. Two spatially separated open quantum systems without direct coherent interaction can undergo a nonlocal quantum phase transition when coupled to correlated quantum reservoirs. Remarkably, the transition is hidden from local observables and emerges only through nonlocal correlations and collective observables. Together, these results demonstrate how nonlinear interactions and engineered dissipation can reshape collective behavior in open quantum systems.
The generation of entanglement in atomic systems plays a central topic in the fields of quantum information storage and processing. Moreover, a special category of entangled states of multi-atom ensembles, spin squeezed states, have been proven to lead to considerable improvement in the sensitivity of precision measurements compared to systems involving uncorrelated atoms. A treatment of entanglement in open systems is, however, incomplete without a precise description of the process of decoherence which necessarily accompanies it. The theory of entanglement and decoherence are the two main topics of this thesis. Methods are described for the generation of strong correlations in large atomic ensembles using either cavity quantum electrodynamics or measurement outcome conditioned quantum dynamics. Moreover, the description of loss of entanglement resulting from the coupling to a noise reservoir (electromagnetic vacuum) is explored. A spin squeezing parameter is used throughout this thesis as both a measure of entanglement strength and as an indication of the sensitivity improvement above the so-called standard quantum limit (sensitivity obtained with uncorrelated particles) in metrology. The first scheme considered consists of a single mode cavity field interacting with a collection of atoms for which spin squeezing is produced in both resonant and off-resonant regimes. In the resonant case, transfer of squeezing from a field state to the atoms is analyzed, while in the off-resonant regime squeezing is produced via an effective nonlinear interaction (one-axis twisting Hamiltonian). A second, more experimentally realistic case, is one involving the interaction of free space atoms with laser pulses; a projective measurement of a source field originating from atomic fluctuations provides a means of preparing atomic collective states such as spin squeezed and Schrodinger cat states. A new unravelling is proposed, that employs the detection of photon number in a single output channel and is capable of producing mesoscopic Schrodinger cat states in a single step. As a first step to understanding the role of cooperative decoherence, of importance in the case of dense pencil-shaped atomic ensembles, the collective spin decoherence of a two multilevel atom system is derived. This calculation is also relevant to entanglement loss for two qubits manipulated using with reading/writing pulses. Finally, a scheme is proposed in which arbitrarily strong entanglement can be produced in a four-wave mixing setup, where the preparation of the atoms in a dark state limits the decoherence to negligible values.