Highly coherent spin states in carbon nanotubes coupled to cavity photons
Tino Cubaynes, Matthieu R. Delbecq, Matthieu Dartiailh, Réouven Assouly, M. M. Desjardins, Lauriane C. Contamin, Laure E. Bruhat, Zaki Leghtas, F. Mallet, Audrey Cottet, Takis Kontos
Abstract Spins confined in quantum dots are considered as a promising platform for quantum information processing. While many advanced quantum operations have been demonstrated, experimental as well as theoretical efforts are now focusing on the development of scalable spin quantum bit architectures. One particularly promising method relies on the coupling of spin quantum bits to microwave cavity photons. This would enable the coupling of distant spins via the exchange of virtual photons for two qubit gate applications, which still remains to be demonstrated with spin qubits. Here, we use a circuit QED spin–photon interface to drive a single electronic spin in a carbon nanotube-based double quantum dot using cavity photons. The microwave spectroscopy allows us to identify an electrically controlled spin transition with a decoherence rate which can be tuned to be as low as 250 kHz. We show that this value is consistent with the expected hyperfine coupling in carbon nanotubes. These coherence properties, which can be attributed to the use of pristine carbon nanotubes stapled inside the cavity, should enable coherent spin–spin interaction via cavity photons and compare favorably to the ones recently demonstrated in Si-based circuit QED experiments. Our clean and controlled nano-assembly technique of carbon nanotubes in the cavity could be further improved by purified 12 C growth to get rid of the nuclear spins resulting in an even higher spin coherence.
Abstract Spins confined in quantum dots are considered as a promising platform for quantum information processing. While many advanced quantum operations have been demonstrated, experimental as well as theoretical efforts are now focusing on the development of scalable spin quantum bit architectures. One particularly promising method relies on the coupling of spin quantum bits to microwave cavity photons. This would enable the coupling of distant spins via the exchange of virtual photons for two qubit gate applications, which still remains to be demonstrated with spin qubits. Here, we use a circuit QED spin–photon interface to drive a single electronic spin in a carbon nanotube-based double quantum dot using cavity photons. The microwave spectroscopy allows us to identify an electrically controlled spin transition with a decoherence rate which can be tuned to be as low as 250 kHz. We show that this value is consistent with the expected hyperfine coupling in carbon nanotubes. These coherence properties, which can be attributed to the use of pristine carbon nanotubes stapled inside the cavity, should enable coherent spin–spin interaction via cavity photons and compare favorably to the ones recently demonstrated in Si-based circuit QED experiments. Our clean and controlled nano-assembly technique of carbon nanotubes in the cavity could be further improved by purified 12 C growth to get rid of the nuclear spins resulting in an even higher spin coherence.
This thesis investigates experimentally the coupling mechanism of the charge and spin degrees of freedom in double quantum dots to high finesse superconducting microwave cavities. We use carbon nanotubes as a coherent conductor to host our quantum dots.We conceived an experimental setup and developed new fabrication methods in order to achieve control over these devices. With these methods, we scrutinize the resonant coupling of the dot's charge electronic transitions to a microwave cavity. We drive the system out of equilibrium to characterise its dynamics and extract its relevant intrinsic parameters. We examine a possible coupling of single photons to a single electron spin, using non-collinear exchange fields induced from ferromagnetic interfaces as a key ingredient to engineer this coupling. The preliminary results in this circuit architecture are promising for future spin-based QED experiments with single spins.
In this thesis we present a spin based QuBit Architecture that implements single-QuBit gates in the QuBit itself and is predicted to have a long coherence time.
This architecture has been physically realized in a Ferromagnetic Double Quantum Dot hosted in a Single Wall Carbon Nanotube, and studied through a coupled Microwave cavity. We present a Linear Response Theory model that ties the transmitted amplitude and phase of the microwave signal through the cavity to the microscopic charge susceptibility of the Double Quantum Dot. We fit those two channels of experimental data to a simple 4 level master equation model that allows us to extract the inter-dot tunneling rate, the charge-photons coupling rate and the charge dephasing rate. We also present a numerical algorithm that allows to evolve in time the quantum state of the device also considering the effect of charge noise. This algorithm is used to study the effect of fast Landau-Zener style pulses on the QuBit, giving the ideal shape of the control pulses.
We present our recent experiments where we demonstrate a hybrid architecture consisting of a quantum dot circuit coupled to a single mode of the electromagnetic ¯eld. We use single wall carbon nanotube based circuits inserted in superconducting microwave cavities. By probing the nanotube dot using a dispersive readout in the Coulomb blockade and the Kondo regime, we determine an electron-photon coupling strength which should enable circuit QED experiments with more complex quantum dot circuits. We extend our architecture to two quantum dot circuits in a microwave cavity. These circuits are separated by 200 times their own size, but share the same anti-node of the cavity ¯eld. We demonstrate their interaction mediated by the cavity photons.
Circuit quantum electrodynamics has received an increasing amount of attention over the last decade in light of its potential use in quantum information processing. The underlying principle of this architecture is the coherent coupling between microwave photons stored in superconducting resonators and superconducting qubits made from non-linear, non-dissipative electrical circuits. This architecture can be extended to other solid-state systems with transition frequencies in the microwave regime, such as nuclear and electron spins or Andreev bound states. These hybrid devices would allow the coherent exchange of information between such systems and superconducting qubits mediated by a microwave resonator. This could lead to advances in quantum information processing and new insights in the physics governing these interacting systems. In this dissertation experimental work with different types of hybrid quantum circuits is presented. A first experiment investigates the coherent coupling of microwave photons with a spin ensemble in a correlated and uncorrelated state. The coupling strength and magnetic resonance is studied as a function of temperature and magnetic field direction. A pronounced temperature dependent anisotropy of the magnetic resonance is observed, which can be attributed to the onset of antiferromagnetic correlations in the spin ensemble when cooled below T=4 K. A simple one-dimensional model gives a good description of this anisotropy. A next experiment studies the transport characteristics of carbon nanotubes electrically accessed with normal and superconducting contacts. These devices were characterised using both DC and RF reflectometry techniques. The carbon nanotube devices with superconducting contacts exhibit transport characteristics of Josephson junctions with critical currents of up to Ic~18 nA, as well as multiple Andreev reflections. These semiconductor-superconductor hybrid Josephson junctions are then used to realise a carbon-nanotube-based superconducting qubit with voltage tunable transition frequency using a local electrostatic gate. Strong coupling (g~100 MHz) to a coplanar waveguide resonator is demonstrated via a resonator frequency shift dependent on applied gate voltage. Qubit parameters are extracted from spectroscopy and correspond well to the DC measurements of the carbon nanotube Josephson junctions. Qubit relaxation and coherence times in the range 10-100 ns are observed. The hybrid devices investigated in this work present potential building blocks for more extensive hybrid architectures for quantum information processing.
Coupling on-chip microwave cavities to superconducting microcircuits has provided a new platform to study the light/matter interaction at the most elementary level [1]. Coupling such cavities to more complex quantum circuits, like quantum dot circuits, is of high interest since it would allow the use of different degrees of freedom, like for instance the electronic spin, in a cavity quantum electrodynamics context. In this talk, I will present various theoretical proposals which would exploit this possibility. First, I will present a scheme allowing a strong coupling between cavity photons and a single spin trapped in a double quantum dot with ferromagnetic contacts [2]. Such a scheme would enable a scalable spin quantum bit architecture. Second, I will discuss theoretically the coupling of a double-quantum dot based Cooper pair splitter to a cavity [3]. Such a scheme can be used to test the entanglement of split Cooper pairs, due to a subradiance property of the Cooper pairs singlet state. Third, I will present recent experiments on carbon nanotube based quantum dots coupled to microwave cavities. In particular, I will discuss the observation of a charge coupling between two distant quantum dots mediated by cavity photons. [1] A. Wallraff, D. I. Schuster, A. Blais, L. Frunzio, R.- S. Huang, J. Majer, S. Kumar, S.M. Girvin, and R. J. Schoelkopf, Nature (London) 431, 162 (2004). [2] A. Cottet and T. Kontos, Phys. Rev. Lett. 105, 160502 (2010) [3] A. Cottet, T. Kontos, and A. Levy Yeyati, Phys. Rev. Lett. 108, 166803 (2012). [5] M.R. Delbecq, V. Schmitt, F.D. Parmentier, N. Roch, J.J. Viennot, G. Fève, B. Huard, C. Mora, A. Cottet, and T. Kontos, Phys. Rev. Lett. 107,256804 (2011) [6] M.R. Delbecq et al., unpublished
Coupling double-quantum-dot circuits to microwave cavities provides a powerful means to control, couple, and manipulate qubits based on the charge or spin of individual electrons. Here, we revisit this standard configuration by adding superconductivity to the circuit. We combine theory and experiment to study a superconductor--double-quantum-dot circuit coupled to microwave cavity photons. First, we use the cavity as a spectroscopic probe. This allows us to determine the low-energy spectrum of the device and to reveal directly Cooper-pair-assisted tunneling between the two dots. Second, we observe a vacuum Rabi splitting which is a signature of strong charge photon coupling and a premiere with carbon-nanotube-based quantum-dot circuits. We show that our circuit design intrinsically combines a set of key features to achieve the strong coupling regime to the cavity. A low charging energy reduces the device sensitivity to charge noise, while sufficient coupling is provided by the shaping of the spectrum of the double quantum dot by the superconducting reservoir. Our findings could be adapted to many other circuit designs and shed light on the coupling of superconducting nanoscale devices to microwave fields.