This thesis investigates experimentally the coupling mechanism of the charge and spin degrees of freedom in double quantum dots to high finesse superconducting microwave cavities. We use carbon nanotubes as a coherent conductor to host our quantum dots.We conceived an experimental setup and developed new fabrication methods in order to achieve control over these devices. With these methods, we scrutinize the resonant coupling of the dot's charge electronic transitions to a microwave cavity. We drive the system out of equilibrium to characterise its dynamics and extract its relevant intrinsic parameters. We examine a possible coupling of single photons to a single electron spin, using non-collinear exchange fields induced from ferromagnetic interfaces as a key ingredient to engineer this coupling. The preliminary results in this circuit architecture are promising for future spin-based QED experiments with single spins.
This thesis investigates experimentally the coupling mechanism of the charge and spin degrees of freedom in double quantum dots to high finesse superconducting microwave cavities. We use carbon nanotubes as a coherent conductor to host our quantum dots.We conceived an experimental setup and developed new fabrication methods in order to achieve control over these devices. With these methods, we scrutinize the resonant coupling of the dot's charge electronic transitions to a microwave cavity. We drive the system out of equilibrium to characterise its dynamics and extract its relevant intrinsic parameters. We examine a possible coupling of single photons to a single electron spin, using non-collinear exchange fields induced from ferromagnetic interfaces as a key ingredient to engineer this coupling. The preliminary results in this circuit architecture are promising for future spin-based QED experiments with single spins.
The recent development of hybrid circuit quantum electrodynamics allows one to study how cavity photons interact with a system driven out of equilibrium by fermionic reservoirs. We study here one of the simplest combination: a double quantum dot coupled to a single mode of the electromagnetic field. We are able to couple resonantly the charge levels of a carbon-nanotube-based double dot to cavity photons. We perform a microwave readout of the charge states of this system, which allows us to unveil features of the out-of-equilibrium charge dynamics, otherwise invisible in the DC current. We extract the relaxation rate, dephasing rate, and photon number of the hybrid system using a theory based on a master equation technique. These findings open the path for manipulating other degrees of freedom, e.g., the spin and/or the valley in nanotube-based double dots using microwave light.
Coupling on-chip microwave cavities to superconducting microcircuits has provided a new platform to study the light/matter interaction at the most elementary level [1]. Coupling such cavities to more complex quantum circuits, like quantum dot circuits, is of high interest since it would allow the use of different degrees of freedom, like for instance the electronic spin, in a cavity quantum electrodynamics context. In this talk, I will present various theoretical proposals which would exploit this possibility. First, I will present a scheme allowing a strong coupling between cavity photons and a single spin trapped in a double quantum dot with ferromagnetic contacts [2]. Such a scheme would enable a scalable spin quantum bit architecture. Second, I will discuss theoretically the coupling of a double-quantum dot based Cooper pair splitter to a cavity [3]. Such a scheme can be used to test the entanglement of split Cooper pairs, due to a subradiance property of the Cooper pairs singlet state. Third, I will present recent experiments on carbon nanotube based quantum dots coupled to microwave cavities. In particular, I will discuss the observation of a charge coupling between two distant quantum dots mediated by cavity photons. [1] A. Wallraff, D. I. Schuster, A. Blais, L. Frunzio, R.- S. Huang, J. Majer, S. Kumar, S.M. Girvin, and R. J. Schoelkopf, Nature (London) 431, 162 (2004). [2] A. Cottet and T. Kontos, Phys. Rev. Lett. 105, 160502 (2010) [3] A. Cottet, T. Kontos, and A. Levy Yeyati, Phys. Rev. Lett. 108, 166803 (2012). [5] M.R. Delbecq, V. Schmitt, F.D. Parmentier, N. Roch, J.J. Viennot, G. Fève, B. Huard, C. Mora, A. Cottet, and T. Kontos, Phys. Rev. Lett. 107,256804 (2011) [6] M.R. Delbecq et al., unpublished
In this thesis we present a spin based QuBit Architecture that implements single-QuBit gates in the QuBit itself and is predicted to have a long coherence time.
This architecture has been physically realized in a Ferromagnetic Double Quantum Dot hosted in a Single Wall Carbon Nanotube, and studied through a coupled Microwave cavity. We present a Linear Response Theory model that ties the transmitted amplitude and phase of the microwave signal through the cavity to the microscopic charge susceptibility of the Double Quantum Dot. We fit those two channels of experimental data to a simple 4 level master equation model that allows us to extract the inter-dot tunneling rate, the charge-photons coupling rate and the charge dephasing rate. We also present a numerical algorithm that allows to evolve in time the quantum state of the device also considering the effect of charge noise. This algorithm is used to study the effect of fast Landau-Zener style pulses on the QuBit, giving the ideal shape of the control pulses.
Circuit quantum electrodynamics has received an increasing amount of attention over the last decade in light of its potential use in quantum information processing. The underlying principle of this architecture is the coherent coupling between microwave photons stored in superconducting resonators and superconducting qubits made from non-linear, non-dissipative electrical circuits. This architecture can be extended to other solid-state systems with transition frequencies in the microwave regime, such as nuclear and electron spins or Andreev bound states. These hybrid devices would allow the coherent exchange of information between such systems and superconducting qubits mediated by a microwave resonator. This could lead to advances in quantum information processing and new insights in the physics governing these interacting systems. In this dissertation experimental work with different types of hybrid quantum circuits is presented. A first experiment investigates the coherent coupling of microwave photons with a spin ensemble in a correlated and uncorrelated state. The coupling strength and magnetic resonance is studied as a function of temperature and magnetic field direction. A pronounced temperature dependent anisotropy of the magnetic resonance is observed, which can be attributed to the onset of antiferromagnetic correlations in the spin ensemble when cooled below T=4 K. A simple one-dimensional model gives a good description of this anisotropy. A next experiment studies the transport characteristics of carbon nanotubes electrically accessed with normal and superconducting contacts. These devices were characterised using both DC and RF reflectometry techniques. The carbon nanotube devices with superconducting contacts exhibit transport characteristics of Josephson junctions with critical currents of up to Ic~18 nA, as well as multiple Andreev reflections. These semiconductor-superconductor hybrid Josephson junctions are then used to realise a carbon-nanotube-based superconducting qubit with voltage tunable transition frequency using a local electrostatic gate. Strong coupling (g~100 MHz) to a coplanar waveguide resonator is demonstrated via a resonator frequency shift dependent on applied gate voltage. Qubit parameters are extracted from spectroscopy and correspond well to the DC measurements of the carbon nanotube Josephson junctions. Qubit relaxation and coherence times in the range 10-100 ns are observed. The hybrid devices investigated in this work present potential building blocks for more extensive hybrid architectures for quantum information processing.
This dissertation describes a set of experiments with the goal of creating a super-conductor-semiconductor hybrid circuit quantum electrodynamics architecture with single electron spins. Single spins in silicon quantum dots have emerged as attractive qubits for quantum computation. However, how to scale up spin qubit systems remains an open question. The hybrid architecture considered here could provide a route to realizing large networks of quantum dot–based spin qubit registers. The first experiment in this thesis is aimed at achieving strong coupling between a single electron spin and a single microwave photon. The electron is trapped in a gate-defined double quantum dot in a Si/SiGe heterostructure and the photon is stored in an on-chip superconducting high-impedance NbTiN cavity. The photon is coupled directly to the electron charge, and indirectly to the electron spin, mediated through a synthetic spin-orbit field. We observe a vacuum Rabi splitting that depends on the spin-charge hybridization. The ratio of spin-photon coupling strength to decoherence rates of the spin and cavity combined is larger than unity, confirming the strong coupling regime has been reached. In addition, we find an optimal degree of spin-charge hybridization for which this ratio is maximized. The demonstration of strong spin-photon coupling not only opens a new range of physics experiments, but fulfills also a crucial requirement for coupling spin qubits at a distance via a cavity. The second experiment is focused on spin readout with the on-chip cavity. Instead of the direct dispersive readout of a single spin, we use the cavity to detect whether the electron is allowed to tunnel between the two dots or not. We benchmark the charge sensitivity and bandwidth of the detector and find that rapid detection of the electron charge with high SNR is possible. In the two-electron regime, electron tunneling is contingent on the total spin state (Pauli spin blockade). This spin-to-charge conversion scheme enables single-shot detection of singlet states with high-fidelity. The demonstration of single-shot spin readout with a cavity is an essential step towards readout in dense spin qubit arrays, such as the crossbar network, where it is not possible to integrate electrometers and accompanying reservoirs adjacent to the qubit dots. In the third experiment, we develop on-chip microwave filters to suppress microwave photon leakage from the cavity through the gate electrodes that are necessary to form quantum dots. We introduce a new cavity design that is compatible with long-distance connectivity between spins, but is also more susceptible to microwave leakage. We test and compare two low-pass filter variations in terms of performance, footprint and integrability. They use the same nanowire inductor, but different implementations of the capacitor: one with a planar interdigitated capacitor and one novel design with an overlapping thin-film capacitor. We find that both approaches are effective against microwave leakage. However, the large footprint of the interdigitated capacitor makes this solution inconvenient as the number of gate lines increases. The thin-film capacitor, with its much smaller footprint, is better suited for our devices. The final part of this dissertation contains concluding remarks and possible future directions are proposed.
Coherent and strong coupling between photons and solid-state qubits, in the form of circuit quantum electrodynamics (QED), has been harnessed for two-qubit gates mediated by photons and high-fidelity quantum non-demolition readout, which are the building blocks of large-scale quantum computation. Recently, circuit QED has been extended to gate-defined semiconductor quantum dots. In this thesis, we develop a novel hybrid circuit QED architecture composed of a high-impedance superconducting microwave resonator and spins localized in silicon-MOS quantum dots. To control and measure the spin degrees of freedom, this hybrid system needs to operate at finite magnetic field. Consequently, we develop and characterize microwave resonators based on thin niobium nitride (NbN) films featuring a high kinetic inductance. We demonstrate high-impedance resonators with magnetic field resilience and low photon loss rates. We then co-integrate the NbN resonators on silicon spin qubit chips. With a hole confined in a double quantum dot (DQD), we report the first realization of a strong hole charge-photon interaction bordering the ultra-strong coupling regime. At finite magnetic field, putting the spin transition energy in resonance with the microwave cavity, we observe large vacuum Rabi mode splittings, signature of a strong spin-photon coupling. Our findings are well captured by the modelling of a hole DQD with different anisotropic Zeeman response in each dot and spin-orbit coupling dependent tunnel rates. We also find a sizeable spin-photon coupling when the hole is localized in the single quantum dot, in line with recent theoretical predictions. The different works presented in this manuscript pave the way for circuit QED with hole spins in gate-defined semiconductor quantum dots.