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arXiv:1902.02932 · Journal of Magnetism and Magnetic Materials

Magnetic excitations and transport properties in frustrated ferromagnetic chain

Hiroaki Onishi

Published Feb 4, 2019• 2 citations
arXivHTMLPDF
DOI
10.1016/j.jmmm.2019.02.006

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Abstract We investigate magnetic excitations and spin transport properties of a frustrated spin chain with ferromagnetic nearest-neighbor and antiferromagnetic next-nearest-neighbor exchange couplings in a magnetic field by density-matrix renormalization group methods. In the field-induced quadrupole and octupole regimes, the low-energy excitation is governed by two-and three-magnon bound states, respectively, so that bound magnon clusters would contribute to the spin transport. We show that spin current correlations decrease when the system goes from the quadrupole regime into the octupole regime. This indicates that the spin transport is suppressed in the octupole regime, although bound three-magnon clusters carry a larger amount of angular momentum than bound two-magnon clusters.
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The thermodynamics of coupled frustrated ferromagnetic chains is studied within a spin-rotation-invariant Green's-function approach. We consider an isotropic Heisenberg spin-half system with a ferromagnetic in-chain coupling J1<0{J}_{1}<0J1​<0 between nearest neighbors and a frustrating antiferromagnetic next-nearest-neighbor in-chain coupling J2>0{J}_{2}>0J2​>0. We focus on the moderate strength of frustration J2<∣J1∣/4{J}_{2}<|{J}_{1}|/4J2​<∣J1​∣/4 such that the in-chain spin-spin correlations are predominantly ferromagnetic. We consider two interchain couplings (ICs) ${J}_{\ensuremath{\perp},y}$ and ${J}_{\ensuremath{\perp},z}$, corresponding to the two axes perpendicular to the chain, where ferromagnetic as well as antiferromagnetic ICs are taken into account. We discuss the influence of frustration on the ground-state properties for antiferromagnetic ICs, where the ground state is of a quantum nature. The major part of our study is devoted to the finite-temperature properties. We calculate the critical temperature Tc{T}_{c}Tc​ as a function of the competing exchange couplings ${J}_{2},{J}_{\ensuremath{\perp},y},{J}_{\ensuremath{\perp},z}$. We find that for fixed ICs, Tc{T}_{c}Tc​ decreases monotonically with increasing frustration J2{J}_{2}J2​, where as ${J}_{2}\ensuremath{\rightarrow}|{J}_{1}|/4$ the Tc(J2){T}_{c}({J}_{2})Tc​(J2​) curve drops down rapidly. To characterize the magnetic ordering below and above Tc{T}_{c}Tc​, we calculate the spin-spin correlation functions $\ensuremath{\langle}{\mathbf{S}}_{0}{\mathbf{S}}_{\mathbf{R}}\ensuremath{\rangle}$, the magnetic order parameter MMM, the uniform static susceptibility ${\ensuremath{\chi}}_{0}$, as well as the correlation length $\ensuremath{\xi}$. Moreover, we discuss the specific heat CV{C}_{V}CV​ and the temperature dependence of the excitation spectrum ${\ensuremath{\omega}}_{\mathbf{q}}$. As ${J}_{2}\ensuremath{\rightarrow}|{J}_{1}|/4$, some unusual frustration-induced features were found, such as an increase of the in-chain spin stiffness (in the case of ferromagnetic ICs) or of the in-chain spin-wave velocity (in the case of antiferromagnetic ICs) with growing temperature.