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arXiv:1902.01292 · Physical review. B./Physical review. B

Magnetic phase separation in a frustrated ferrimagnetic chain under a magnetic field

A.M. do Nascimento-Junior, R. R. Montenegro-Filho

Published Feb 4, 2019• 11 citations
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Abstract

We use density-matrix renormalization group to study the first-order quantum phase transition induced by a magnetic field $h$ in a frustrated ferrimagnetic chain. The magnetization ($m$) curve as a function of $h$ presents a macroscopic jump and the energy curve as a function of $m$ has two global minima. We characterize the two competing phases and study the phase-separated states in the coexistence region. Also, we observe that the transition is accompanied by an increase in the number of itinerant singlet pairs between sites in the unit cells of the chain. Finally, we identify the critical point at the end of the first-order transition line and a crossover line.

DOI
10.1103/physrevb.99.064404

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We use density-matrix renormalization group to study the first-order quantum phase transition induced by a magnetic field hhh in a frustrated ferrimagnetic chain. The magnetization (mmm) curve as a function of hhh presents a macroscopic jump and the energy curve as a function of mmm has two global minima. We characterize the two competing phases and study the phase-separated states in the coexistence region. Also, we observe that the transition is accompanied by an increase in the number of itinerant singlet pairs between sites in the unit cells of the chain. Finally, we identify the critical point at the end of the first-order transition line and a crossover line.
We use the density matrix renormalization group (DMRG) and a hard-core boson map to investigate the quantum phase transitions present in the phase diagram of the frustrated Heisenberg ladder in a magnetic field. The quantum bicritical point is observed at the end of a first-order transition line, which is at the meeting of the two second-order transition lines that bound the fully polarized plateau. The characterization of the bicritical point was made using a hard-core boson mapping of the low-energy excitations from the fully polarized phase and through DMRG by studying the probability density of finding the rung spins in a singlet or a triplet state with zero spin component along the magnetic field. In particular, we give conditions for the exchange couplings for the presence of the first-order transition line and the bicritical point in the phase diagram. Moreover, we unveil the phase-separated states for magnetization values inside the magnetization jump and, in particular, the dependence on the system size of the energy curve as a function of magnetization. Finite-size scaling analysis of the transverse spin correlation functions has been used to estimate the critical points of the Kosterlitz-Thouless transitions from the fractional magnetization plateau m=1/2m=1/2m=1/2 to the respective gapless Luttinger liquid phases for some sets of parameters.
Using density-matrix renormalization group (DMRG) method, we studied the effect of magnetic frustrations due to next-nearest- neighbor bonds in a system of quasi-one-dimensional Heisenberg antiferromagnetic chain but with ferrimagnetic properties. In this paper, the ground state energy per unit cell, spin correlation function and spin gap are calculated. As a result of the frustrations, the quantum disordered phase with the spin gap appears at the spin order-disorder phase transition point αC≈0.412 to α＝1. And in the region of magnetic-order phase, the increasing magnetic frustrations reduce the magnetic order.
The frustrated ferromagnetic spin-1∕21∕21∕2 Heisenberg chain is studied by means of a low-energy field theory as well as the density-matrix renormalization group and exact diagonalization methods. First, we study the ground-state phase diagram in a magnetic field and find an ``even-odd'' (EO) phase characterized by bound pairs of magnons in the region of two weakly coupled antiferromagnetic chains. A jump in the magnetization curves signals a first-order transition at the boundary of the EO phase, but otherwise the curves are smooth. Second, we discuss thermodynamic properties at zero field, where we confirm a double-peak structure in the specific heat for moderate frustrating next-nearest-neighbor interactions.
Magnetization curves of the ferrimagnetic mixed spin-(1/2,S) Heisenberg chains are calculated with the help of density-matrix renormalization group method for several quantum spin numbers S=1, 3/2, 2 and 5/2.It is shown that the ferrimagnetic mixed spin-(1/2,S) Heisenberg chains exhibit irrespective of the spin value S exactly one intermediate magnetization plateau, which can be identified with the gapped Lieb-Mattis ferrimagnetic ground state.The magnetization plateau due to the Lieb-Mattis ferrimagnetism breaks down at a quantum phase transition towards the Luttinger spin liquid, which is characterized by a continuous change of the magnetization with the magnetic field until another quantum critical point is reached at the saturation field.
We give a short review of our recent works on the first-order quantum phase transitions in frustrated spin chains with orthogonal-dimer structure. When the ratio of the competing antiferromagnetic exchange couplings is varied, a first-order transition occurs between the dimer phase and the plaquette phase, which is accompanied by the discontinuity in the spin excitation gap. We further show that strong frustration triggers the phase transitions in a magnetic field, which exhibit plateaus and jumps in the magnetization curve. The hole-doping effect is also addressed for the orthogonal-dimer chain with linked-tetrahedra structure. It is found that the competing antiferromagnetic interactions result in a first-order metal-insulator transition upon hole doping.
We give a short review of our recent works on the first-order quantum phase transitions in frustrated spin chains with orthogonal-dimer structure. When the ratio of the competing antiferromagnetic exchange couplings is varied, a first-order transition occurs between the dimer phase and the plaquette phase, which is accompanied by the discontinuity in the spin excitation gap. We further show that strong frustration triggers the phase transitions in a magnetic field, which exhibit plateaus and jumps in the magnetization curve. The hole-doping effect is also addressed for the orthogonal-dimer chain with linked-tetrahedra structure. It is found that the competing antiferromagnetic interactions result in a firstorder metal-insulator transition upon hole doping. Recently antiferromagnetic quantum spin systems with strong frustration have been studied intensively. A typical example is SrCu2(BO3)2 1) where the spin-1/2 magnetic Cu ions are located on the orthogonal-dimer lattice (the so-called Shastry-Sutherland model). 2) Various interesting phenomena were observed for this compound