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arXiv:1902.00583 · Physical review. B./Physical review. B

Critical opalescence across the doping-driven Mott transition in optical lattices of ultracold atoms

C. Walsh, P. Sémon, G. Sordi, A.–M. S. Tremblay

Published Apr 30, 2019• 22 citations
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Abstract

The authors show that critical opalescence - enhanced density fluctuations at all length scales - occurs in quantum matter, specifically in a doped Mott-insulating system that can be realized with ultracold atoms in optical lattices. These findings provide a theoretical framework and new predictions for ultracold-atom experiments. Looking for critical opalescence across the doping-driven Mott transition in ultracold systems may give insights on the origin of the pseudogap in cuprate high-temperature superconductors.

DOI
10.1103/physrevb.99.165151

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The authors show that critical opalescence - enhanced density fluctuations at all length scales - occurs in quantum matter, specifically in a doped Mott-insulating system that can be realized with ultracold atoms in optical lattices. These findings provide a theoretical framework and new predictions for ultracold-atom experiments. Looking for critical opalescence across the doping-driven Mott transition in ultracold systems may give insights on the origin of the pseudogap in cuprate high-temperature superconductors.
Divergent carrier-density fluctuations equivalent to the critical opalescence of gas-liquid transitions emerge around a metal-insulator critical point at a finite temperature. In contrast to the gas-liquid transitions, however, the critical temperature can be lowered to zero, which offers a challenging quantum phase transition. We present a microscopic description of such quantum critical phenomena in two dimensions. The conventional scheme of phase transitions by Ginzburg, Landau and Wilson is violated and an unconventional universality appears. It offers a clear insight into the criticalities of metal-insulator transitions associated with Mott or charge-order transitions. Fermi degeneracy involving the diverging density fluctuations generates emergent phenomena near the endpoint of the first-order transition and must shed new light on remarkable phenomena found in correlated metals like unconventional cuprate superconductors. It indeed accounts for otherwise puzzling criticality of the Mott transition recently discovered in an organic conductor. We propose to measure enhanced dielectric fluctuations at small wavenumbers by accurate probes.
We establish that a doping-driven first-order metal-to-metal transition, from a pseudogap metal to Fermi Liquid, can occur in correlated quantum materials. Our result is based on the exact Dynamical Mean Field Theory solution of the Dimer Hubbard Model. This transition elucidates the origin of many exotic features in doped Mott materials, like the pseudogap in cuprates, incoherent bad metals, enhanced compressibility and orbital selective Mott transition. This phenomenon is suggestive to be at the roots of the many exotic phases appearing in the phase diagram of correlated materials.
Quantum criticality emerges when a many-body system is in the proximity of a continuous phase transition that is driven by quantum fluctuations. In the quantum critical regime, exotic, yet universal properties are anticipated; ultracold atoms provide a clean system to test these predictions. We report the observation of quantum criticality with two-dimensional Bose gases in optical lattices. On the basis of in situ density measurements, we observe scaling behavior of the equation of state at low temperatures, locate the quantum critical point, and constrain the critical exponents. We observe a finite critical entropy per particle that carries a weak dependence on the atomic interaction strength. Our experiment provides a prototypical method to study quantum criticality with ultracold atoms.
In this thesis I report on experiments that enter a new regime in the many body physics of ultracold atomic gases. A Bose-Einstein condensate is loaded into a three-dimensional optical lattice potential formed by a standing wave laser light field. In this novel quantum system we have been able to both realize a quantum phase transition from a superfluid to a Mott insulator, and to observe the collapse and revival of a macroscopic matter wave field. Quantum phase transitions are driven by quantum fluctuations and occur, even at zero temperature, as the relative strength of two competing energy terms in the underlying Hamiltonian is varied across a critical value. In the first part of this work I report on the observation of such a quantum phase transition in a Bose-Einstein condensate with repulsive interactions, held in a three-dimensional optical lattice potential. In the superfluid ground state, each atom is spread-out over the entire lattice, whereas in the Mott insulating state, exact numbers of atoms are localized at individual lattice sites. We observed the reversible transition between those states and detected the gap in the excitation spectrum of the Mott insulator. A Bose-Einstein condensate is usually described by a macroscopic matter wave field. However, a quantized field underlies such a "classical" matter wave field of a Bose-Einstein condensate. The striking behavior of ultracold matter due to the field quantization and the nonlinear interactions between the atoms is the focus of the second part of this work. The matter wave field of a Bose-Einstein condensate is observed to undergo a series of collapses and revivals as time evolves. Furthermore, we show that the collisions between individual pairs of atoms lead to a fully coherent collisional phase shift in the corresponding many-particle state, which is a crucial cornerstone of proposed novel quantum computation schemes with neutral atoms. With these experiments we enter a new field of physics with ultracold quantum gases. In this strongly correlated regime, interactions between atoms dominate the behavior of the many-body system such that it can no longer be described by the usual theories for weakly interacting Bose gases. This novel quantum system offers the unique possibility to experimentally address fundamental questions of modern solid state physics, atomic physics, quantum optics, and quantum information.
Considering a system of ultracold atoms in an optical lattice, we propose a simple and robust implementation of a quantum simulator for the homogeneous ttt-JJJ model with a well-controlled fraction of holes xxx. The proposed experiment can provide valuable insight into the physics of cuprate superconductors. A similar scheme applied to bosons, moreover, allows one to investigate experimentally the subtle role of inhomogeneity when a system passes from one quantum phase to another.
Ultracold quantum gases in optical lattices form almost ideal conditions to analyze the physics of strongly correlated quantum phases in periodic potentials. Such strongly correlated quantum phases are of fundamental interest in condensed matter physics, because they lie at the heart of topical quantum materials, such as high-Tc superconductors and quantum magnets, which pose a challenge to our basic understanding of interacting many-body systems. Quite generally, such strongly interacting quantum phases arise when the interaction energy between two particles dominates over the kinetic energy of the two particles. Such a regime can either be achieved by increasing the interaction strength between the atoms via Feshbach resonances or by decreasing the kinetic energy, such that eventually the interaction energy is the largest energy scale in the system. The latter can, for example, simply be achieved by increasing the optical lattice depth. This chapter tries gives an introduction into the field of optical lattices and the physics of strongly interacting quantum phases. A prominent example hereof is the superfluid-to-Mott insulator transition, which transforms a weakly interacting quantum gas into a strongly correlated many body system. Dominating interactions between the particles are in fact crucial for the Mott insulator transition and also for the realization of controlled interaction-based quantum gates, of which several have been successfully realized experimentally.