We address a fundamental question of quantum optics: Can a beam of light mediate coherent Hamiltonian interactions between two distant quantum systems? This is an intriguing question whose answer is not a priori clear, since the light carries away information about the systems and might be subject to losses, giving rise to intrinsic decoherence channels associated with the coupling. Our answer is affirmative and we derive a particularly simple sufficient condition for the interactions to be Hamiltonian: The light field needs to interact twice with the systems and the second interaction has to be the time reversal of the first. We demonstrate that, even in the presence of significant optical loss, coherent interactions can be realized and generate substantial amounts of entanglement between the systems. Our method is directly applicable for building hybrid quantum systems, with relevant applications in the fields of optomechanics and atomic ensembles.
We address a fundamental question of quantum optics: Can a beam of light mediate coherent Hamiltonian interactions between two distant quantum systems? This is an intriguing question whose answer is not a priori clear, since the light carries away information about the systems and might be subject to losses, giving rise to intrinsic decoherence channels associated with the coupling. Our answer is affirmative and we derive a particularly simple sufficient condition for the interactions to be Hamiltonian: The light field needs to interact twice with the systems and the second interaction has to be the time reversal of the first. We demonstrate that, even in the presence of significant optical loss, coherent interactions can be realized and generate substantial amounts of entanglement between the systems. Our method is directly applicable for building hybrid quantum systems, with relevant applications in the fields of optomechanics and atomic ensembles.
This thesis presents theoretical and experimental work on light-mediated coupling between a collective atomic spin and a micromechanical membrane oscillator. With our work we address a fundamental question of quantum optics: Can a beam of light mediate coherent Hamiltonian interactions between two distant quantum systems? This is an intriguing question whose answer is not a priori clear, since the light carries away information about the systems and might be subject to losses, giving rise to intrinsic decoherence channels associated with the coupling. Our answer is affirmative and we derive a particularly simple sufficient condition for the interactions to be Hamiltonian: The light field needs to interact twice with the systems and the second interaction has to be the time reversal of the first. We demonstrate theoretically that, even in the presence of significant optical loss, coherent interactions can be realized and generate substantial amounts of entanglement between the systems. \n \nIn our experiments, we employ this approach to strongly couple a spin-polarized atomic ensemble and a micromechanical oscillator via a free-space laser beam across a distance of one meter in a room-temperature environment. The atomic ensemble consists of about ten million laser-cooled Rubidium atoms in an optical dipole trap that interact with the coupling laser via an off-resonant Faraday interaction. The mechanical oscillator is a silicon nitride membrane which is mounted in a single-sided optical cavity and couples to the laser field via radiation-pressure forces. In order to mediate a bidirectional Hamiltonian interaction between spin and membrane, the coupling beam is arranged in a loop such that it couples twice to the spin. This looped geometry enables destructive interference of quantum back-action by the light field on the spin. \n \nUsing this setup, we experimentally demonstrate for the first time strong Hamiltonian coupling between remote quantum systems and explore different dynamical regimes of cascaded light-mediated interactions: With the spin initialized in its ground state we observe normal-mode splitting and coherent energy exchange oscillations, both hallmarks of strong coupling. If we invert the spin to its highest energy state, we observe parametric-gain interactions, resulting in two-mode thermal noise squeezing. Furthermore, by shifting the phase of the light field between spin and membrane we can switch to non-Hamiltonian coupled dynamics, allowing us to observe level attraction and exceptional points. This high level of control in a strongly coupled modular system gives access to a unique toolbox for designing hybrid quantum systems and coherent optical feedback loops. Our approach to engineer coherent long-distance interactions with light makes it possible to couple very different systems in a modular way, opening up a range of new opportunities for quantum control. \n
Quantum networks are composed of quantum nodes which coherently interact by way of quantum channels. They offer powerful capabilities for quantum computation, communication, and metrology. A generic requirement for these realizations is the capability to generate and store quantum states among multiple quantum nodes, and to disseminate these resources throughout the network via the quantum channels. In this thesis, I describe a series of experiments whereby single excitations in atomic ensembles are strongly coupled to optical modes and provide efficient means for the coherent control of entangled states between matter and light. By following the seminal proposal by Duan et al., we have generated measurement-induced entanglement of an excitation between two cold atomic ensembles. Using this system, we investigated the relationship for the global bipartite entanglement and local correlations in its subsystems. In addition, we achieved functional quantum nodes for entanglement distribution. Two pairs of remote ensembles at two quantum nodes were prepared into entangled states in a heralded and asynchronous fashion by the conditional controls of the entanglement. The quantum states of the ensembles were then distributed into polarization entangled states of photons. We also prepared an analogous quantum state and transferred the nonlocal coherence between two pairs of heralded entangled atomic ensembles, providing a step towards entanglement connection. Beyond such probabilistic approaches, we demonstrated an experiment where entanglement between two quantum memories is created by the reversible and deterministic mapping of an entangled state of light via dynamic electromagnetically induced transparency. This experiment opens novel prospects of integrating hybrid quantum systems by way of reversible quantum interfaces between light and matter. Then, we extended our work to multipartite quantum systems. We theoretically investigated the characterization of multipartite mode-entangled states by way of quantum uncertainty relations, and introduced theoretical tools to verify the entanglement orders in multipartite systems. In particular, we achieved entanglement for one delocalized photon among multiple optical modes (N > 2). Finally, we have achieved measurement-induced entanglement of spin waves among four quantum memories. The individual atomic components for the entangled W state of the four ensembles were then coherently converted into four propagating entangled beams of light via superradiant emissions. We observed the statistical and dynamic transitions for the multipartite entangled spin waves. Experiments described in this thesis thereby represent significant advances of experimental and theoretical capabilities to generate, store, transfer, and characterize entanglement of matter and light over quantum networks.
In this dissertation, I explore interactions between matter and propagating light. The electromagnetic field is modeled as a reservoir of quantum harmonic oscillators successively streaming past a quantum system. Each weak and fleeting interaction entangles the light and the system, and the light continues its course. Within the framework of open quantum systems, the light is eventually traced out, leaving the reduced quantum state of the system as the primary mathematical subject. Two major results are presented. The first is a master equation approach for a quantum system interacting with a traveling wave packet prepared with a definite number of photons. In contrast to quasi-classical states, such as coherent or thermal fields, these N-photon states possess temporal mode entanglement, and local interactions in time have nonlocal consequences. The second is a model for a three-dimensional light-matter interface for an atomic ensemble interacting with a paraxial laser beam and its application to the generation of QND spin squeezing. Both coherent and incoherent dynamics due to spatially inhomogeneous atom-light coupling across the ensemble are accounted for. Measurement of paraxially scattered light can generate squeezing of an atomic spin wave, while diffusely scattered photons lead to spatially local decoherence.
Interfacing between matter qubits and light is a crucial provision for numerous quantum technological applications. However, a generic qubit may not directly interact with a relevant optical field mode, and hence, one could necessitate adjusting frequencies to match resonance conditions between parties. In this work, we show how a parametric coupling of the qubit with a mechanical oscillator, in conjunction with the trilinear radiation pressure coupling of the same object with light, can induce maximal qubit-light entanglement at an optimal time. Furthermore, we show how our method enables conditional (dynamical) nonclassical state preparation of the optical field via qubit measurement in the weak (moderate-to-strong) optomechanical coupling regime. Our scheme benefits from not requiring any cooling of the mechanical component and not needing an adjusting of the detunings and transition frequencies to have resonance between any pairs of quantum systems.
In this thesis we have focused on the study of various systems which are presently widely studied in different areas of quantum optics and quantum information sciences. These, for example, include the coupled system of photonic waveguides which are known to be highly efficient in manipulating the flow of light. The Hamiltonian describing the evolution of field mode in coupled waveguides is effectively identical to the well-known tight binding Hamiltonian used in solid state physics. The advantage of waveguide system is the possibility to control various interactions by design and their low decoherence rate. The excellent stability offered by coupled waveguides has led to the observation of many key coherent effects such as quantum walk, Bloch oscillation, and discrete Talbot effect. For example, Bloch oscillations have been investigated in coupled waveguides using coherent beam of light. We wanted to inquire whether coherent phenomena such as Bloch oscillations can be possible with incoherent single photon sources. We discovered that Bloch oscillations are indeed possible with single photons provided we prepare single photons in a W state. Moreover, coupled waveguides also find applications in the field of quantum information processing. Since entanglement plays a prominent role in all these applications, it is important to understand the entanglement dynamics in these structures. We considered the case of squeezed input in one of the waveguide and showed that one can generate entanglement between the waveguide modes. We further continued our work on the entanglement generation in coupled waveguides by incorporating the effect of loss in the waveguide structure for the squeezed and photon number input states. We considered relevant experimental parameters and showed that waveguide structures are reasonably robust against the effect of loss. Another system which has attracted a great deal of interest is the optomechanical system. We consider an optomechanical system where an optical cavity mode is coupled to the square of the position of a mechanical oscillator. The optomechanical system can then be regarded as a quantum optical spring, i.e., a spring whose spring constant depends on the quantum state of another system. In particular, we consider the situation where the field inside the cavity is in a coherent state and the oscillator is prepared in its ground state. The quantized nature of the field produces new features in the optomechanical system.
In this thesis I explore the use of collective spin angular momentum as a platform for quantum information processing. Such systems have several nice features that make them excellent choices for such protocols, especially ones where information is also stored in photonic variables. The longer coherence times of atoms makes it possible to store information from light in atoms for future use, and it is generally easier to couple atomic variables than to create nonlinear interactions of light. Above and beyond the advantages of atomic systems, collective atomic systems have additional strengths. In the limit of a large number of atoms, the collective variables of atomic systems have a natural connection to the bosonic algebra of light (known as the Holstein-Primakoff or HP approximation) where components of the collective spin angular momentum effectively act as quadratures, making them natural systems for coupling to light. Also, collectively addressing the atoms allows one to access a large state space without individual addressing of the atoms. A natural first step towards control of these collective variables is generating large amounts of atomic spin squeezing. In the HP approximation going from rotations to squeezing corresponds to going from linear to quadratic interactions in the atomic quadratures; for extremely large squeezing one should see the breakdown of the HP approximation and the ability to generate arbitrary collective atomic states. I have sought to improve previous schemes for the spin squeezing of atomic ensembles, such as the proposal of Takeuchi et. al. based on coherent quantum feedback. In this scheme a beam of linearly polarized light passes through the atomic ensemble (prepared in a coherent state), coupling to the atoms through a state-dependent index of refraction (the Faraday effect). The light is then passed through a wave-plate and reflected back through the atoms for a second pass. This double-pass scheme leads to an effective nonlinearity as the atomic fluctuations are mapped onto the light on the first pass and then back on to the atoms in the second pass. The light acts as a bus coupling each atom to each of the others. This nonlinear interaction forms a shearing of the atomic coherent state that results in squeezing. The light is entangled to the atoms through these interactions, and remains entangled as it escapes the system. This leads to decoherence of the atoms as the light is lost to the environment, reducing the amount of spin squeezing achieved. The first step towards improving the double-pass scheme was to add a quantum eraser step in which the light is disentangled from the squeezed atoms. By first measuring one quadrature of the light, and then performing a measurement-dependent rotation on the atomic ensemble, it is possible to decouple the atoms and light so that the loss of the light does not reduce the atomic squeezing. This results in an improvement of the rate of atomic spin squeezing. The nonlinear shearing interaction that remains still falls short of the exponential squeezing seen in optical parametric amplification. The reason for this can be seen by decomposing the shearing interaction into squeezing along a given quadrature followed by a rotation. The rotation leads to a constantly changing axis along which the squeezing occurs, and thus the squeezing builds up more slowly. This can be corrected for by breaking up the light pulse into a sequence of small pulses, and performing a small phase matching rotation after each pulse. The squeezing then adds up along a constant direction, rather than along a constantly varying direction. This results in still further improvement of the rate of atomic spin squeezing. A complete model includes the effects of photon-atom scattering and other noise and loss effects on the overall rate of squeezing. Previous derivations of noise due to photon-atom scattering have started with the unjustified assumptions that the atomic and photonic decoherence channels were both Gaussian and independent of correlations between the two subsystems. They then proceed with very general statistical arguments that rely upon these simplifications. My work begins with the more fundamental master equation picture in which I find the Linblad jump operators. I find that in general the photonic and atomic loss channels are not independent, with the intensity of the light dictating the details of this dependence, and find the conditions under which the Gaussian approximation holds. Squeezing and loss is initially treated assuming ensembles of spin-1/2 atoms, but this work is further extended to higher dimensional subsystems. For a higher spin case, preparing the atoms in spin coherent states is not optimal. One can engineer a stronger interaction by preparing the atoms in an atomic "cat state", i.e., a superposition of the two stretch states along the direction of propagation of the light beam. The fluctuations of such a state are more strongly coupled to the light, resulting in a stronger nonlinearity. This leads to strong correlations between the atoms, but they are not immediately useful for squeezing; the cat state must be coherently mapped to a coherent state to achieve atomic spin squeezing. The state created in this manner is ultimately more squeezed than that achieved with the same interaction but prepared initially in a coherent state.