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arXiv:1901.05905 · Physical review. B./Physical review. B

SU(4) topological resonating valence bond spin liquid on the square lattice

Olivier Gauthé, Sylvain Capponi, Didier Poilblanc

Published Jun 26, 2019• 8 citations
arXivHTMLPDF

Abstract

We generalize the construction of the spin-1/2 SU(2) resonating valence bond (RVB) state to the case of the self-conjugate $\mathbf{6}$ representation of SU(4). As for the case of SU(2) [J.-Y. Chen and D. Poilblanc, Phys. Rev. B 97, 161107(R) (2018)], we use the projected entangled pair state (PEPS) formalism to derive a simple (two-dimensional) family of generalized SU(4) RVB states on the square lattice. We show that, when longer-range SU(4)-singlet bonds are included, a local gauge symmetry is broken down from U(1) to ${\mathbb{Z}}_{2}$, leading to the emergence of a short-range spin liquid. Evidence for the topological nature of this spin liquid is provided by the investigation of the Renyi entanglement entropy of infinitely long cylinders and of the modular matrices. Relevance to microscopic models and experiments of ultracold atoms is discussed.

DOI
10.1103/physrevb.99.241112

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We generalize the construction of the spin-1/2 SU(2) resonating valence bond (RVB) state to the case of the self-conjugate 6\mathbf{6}6 representation of SU(4). As for the case of SU(2) [J.-Y. Chen and D. Poilblanc, Phys. Rev. B 97, 161107(R) (2018)], we use the projected entangled pair state (PEPS) formalism to derive a simple (two-dimensional) family of generalized SU(4) RVB states on the square lattice. We show that, when longer-range SU(4)-singlet bonds are included, a local gauge symmetry is broken down from U(1) to Z2{\mathbb{Z}}_{2}Z2​, leading to the emergence of a short-range spin liquid. Evidence for the topological nature of this spin liquid is provided by the investigation of the Renyi entanglement entropy of infinitely long cylinders and of the modular matrices. Relevance to microscopic models and experiments of ultracold atoms is discussed.
Topological chiral phases are ubiquitous in the physics of the fractional quantum Hall effect. Nonchiral topological spin liquids are also well known. Here, using the framework of projected entangled pair states (PEPS), we construct a family of chiral spin liquids on the square lattice, which are generalized spin-1/2 resonating valence bond (RVB) states obtained from deformed local tensors with d+idd+i\phantom{\rule{0.16em}{0ex}}dd+id symmetry. On a cylinder, we construct four topological sectors with even or odd number of spinons on the boundary and even or odd number of (Z2{\mathbb{Z}}_{2}Z2​) fluxes penetrating the cylinder, which, we argue, remain orthogonal in the limit of infinite perimeter. The analysis of the transfer matrix provides evidence of short-range (long-range) triplet (singlet) correlations as for the critical (nonchiral) RVB state. The entanglement spectrum exhibits chiral edge modes, which we confront to predictions of the conformal field theory, and the corresponding entanglement Hamiltonian is shown to be long-ranged.
A one-parameter family of long-range resonating-valence-bond (RVB) state on the square lattice was previously proposed to describe a critical spin liquid (SL) phase of the spin-1/2 frustrated Heisenberg model. We provide evidence that this RVB state in fact also realizes a topological (long-range entangled) Z2{\mathbb{Z}}_{2}Z2​ SL, limited by two transitions to critical SL phases. The topological phase is naturally connected to the Z2{\mathbb{Z}}_{2}Z2​ gauge symmetry of the local tensor. This Rapid Communication shows that, on one hand, spin-1/2 topological SL with C4v{C}_{4v}C4v​ point-group symmetry and SU(2)SU(2)SU(2) spin rotation symmetry exists on the square lattice and, on the other hand, criticality and nonbipartiteness are compatible. We also point out that strong similarities between our phase diagram and the ones of classical interacting dimer models suggest both can be described by similar Kosterlitz-Thouless transitions. This scenario is further supported by the analysis of the one-dimensional boundary state. Forms of parent Hamiltonians hosting the Z2{\mathbb{Z}}_{2}Z2​ SL are suggested.
We construct a short-range resonating-valence-bond (RVB) state on the ruby lattice, using projected entangled-pair states with bond dimension D=3D=3D=3. By introducing nonlocal moves to the dimer patterns on the torus, we distinguish four distinct sectors in the space of dimer coverings, which is a signature of the topological nature of the RVB wave function. Furthermore, by calculating the reduced density matrix of a bipartition of the RVB state on an infinite cylinder and exploring its entanglement entropy, we confirm the topological nature of the RVB wave function by obtaining a nonzero topological contribution, $\ensuremath{\gamma}=\ensuremath{-}\mathrm{ln}\phantom{\rule{4pt}{0ex}}2$, consistent with that of a Z2{\mathbb{Z}}_{2}Z2​ topological quantum spin liquid. We also calculate the ground-state energy of the spin-12\frac{1}{2}21​ antiferromagnetic Heisenberg model on the ruby lattice and compare it with the RVB energy. Finally, we construct a quantum dimer model for the ruby lattice and discuss it as a possible parent Hamiltonian for the RVB wave function.
We introduce a spin-orbital entangled (SOE) resonating valence bond (RVB) state on a square lattice of spins 12\frac{1}{2}21​ and orbitals represented by pseudospins 12\frac{1}{2}21​. Like the standard RVB state, it is a superposition of nearest-neighbor hard-core coverings of the lattice by spin singlets, but adjacent singlets are favored to have perpendicular orientations and, more importantly, an orientation of each singlet is entangled with orbitals state on its two lattice sites. The SOE-RVB state can be represented by a projected entangled pair state (PEPS) with a bond dimension D=4D=4D=4. This representation helps to reveal that the state is a superposition of striped coverings conserving a topological quantum number. The stripes are a critical quantum spin liquid. We propose a spin-orbital Hamiltonian supporting a SOE-RVB ground state.
We consider the phase diagram of the most general SU(4)-symmetric two-site Hamiltonian for a system of two fermions per site (i.e., self-conjugate 6\mathbf{6}6 representation) on the square lattice. It is known that this model hosts magnetic phases breaking SU(4) symmetry and quantum disordered dimerlike phases breaking lattice translation symmetry. Motivated by a previous work [O. Gauth\'e, S. Capponi, and D. Poilblanc, Phys. Rev. B 99, 241112(R) (2019)], we investigate the possibility of the existence of SU(4) quantum spin liquid phases in this model, using SU(4)-symmetric projected entangled pair states (PEPS) of small bond dimensions, which can be classified according to point group and charge (C) symmetries. Among several (disconnected) families of SU(4)-symmetric PEPS, breaking or not C-symmetry, we identify critical or topological spin liquids which may be stable in some regions of the phase diagram. These results are confronted to exact diagonalization (ED) and density matrix renormalization group (DMRG) calculations.
We examine in details the connections between topological and entanglement properties of short-range resonating valence bond (RVB) wave functions using projected entangled pair states (PEPS) on kagome and square lattices on (quasi)infinite cylinders with generalized boundary conditions (and perimeters with up to 20 lattice spacings). By making use of disconnected topological sectors in the space of dimer lattice coverings, we explicitly derive (orthogonal) ``minimally entangled'' PEPS RVB states. For the kagome lattice, using the quantum Heisenberg antiferromagnet as a reference model, we obtain the finite-size scaling with increasing cylinder perimeter of the vanishing energy separations between these states. In particular, we extract two separate (vanishing) energy scales corresponding (i) to insert a vison line between the two ends of the cylinder and (ii) to pull out and freeze a spin at either end. We also investigate the relations between bulk and boundary properties and show that, for a bipartition of the cylinder, the boundary Hamiltonian defined on the edge can be written as a product of a highly nonlocal projector, which fundamentally depends upon boundary conditions, with an emergent (local) SU(2)(2)(2)-invariant one-dimensional (superfluid) ttt-JJJ Hamiltonian, which arises due to the symmetry properties of the auxiliary spins at the edge. This multiplicative structure, a consequence of the disconnected topological sectors in the space of dimer lattice coverings, is characteristic of the topological nature of the states. For minimally entangled RVB states, it is shown that the entanglement spectrum, which reflects the properties of the (gapless or gapped) edge modes, is a subset of the spectrum of the local Hamiltonian, e.g., half of it for the kagome RVB state, providing a simple argument on the origin of the topological entanglement entropy ${S}_{0}=\ensuremath{-}\mathrm{ln}2$ of the Z2{\mathbb{Z}}_{2}Z2​ spin liquid. We propose to use these features to probe topological phases in microscopic Hamiltonians, and some results are compared to existing density matrix renormalization group data.