Photodetection plays a key role in basic science and technology, with exquisite performance having been achieved down to the single-photon level. Further improvements in photodetectors would open new possibilities across a broad range of scientific disciplines and enable new types of applications. However, it is still unclear what is possible in terms of ultimate performance and what properties are needed for a photodetector to achieve such performance. Here, we present a general modeling framework for photodetectors whereby the photon field, the absorption process, and the amplification process are all treated as one coupled quantum system. The formalism naturally handles field states with single or multiple photons as well as a variety of detector configurations and includes a mathematical definition of ideal photodetector performance. The framework reveals how specific photodetector architectures introduce limitations and tradeoffs for various performance metrics, providing guidance for optimization and design.
Photodetection plays a key role in basic science and technology, with exquisite performance having been achieved down to the single-photon level. Further improvements in photodetectors would open new possibilities across a broad range of scientific disciplines and enable new types of applications. However, it is still unclear what is possible in terms of ultimate performance and what properties are needed for a photodetector to achieve such performance. Here, we present a general modeling framework for photodetectors whereby the photon field, the absorption process, and the amplification process are all treated as one coupled quantum system. The formalism naturally handles field states with single or multiple photons as well as a variety of detector configurations and includes a mathematical definition of ideal photodetector performance. The framework reveals how specific photodetector architectures introduce limitations and tradeoffs for various performance metrics, providing guidance for optimization and design.
Photodetection plays a key role in basic science and technology, with exquisite performance having been achieved down to the single photon level. Further improvements would open new possibilities across a broad range of scientific disciplines, and enable new types of applications. However, it is still unclear what is possible in terms of ultimate performance, and what properties are needed to achieve such performance. Here, we present a general modeling framework for photodetectors whereby the photon field, the absorption process, and the amplification process are all treated as one coupled quantum system. The formalism naturally handles field states with single or multiple photons as well as a variety of detector configurations, and includes a mathematical definition of ideal photodetector performance. The framework reveals how specific photodetector architectures introduce limitations and tradeoffs for various performance metrics, providing guidance for optimization and design.
Single-photon detectors have achieved impressive performance and have led to a number of new scientific discoveries and technological applications. Existing models of photodetectors are semiclassical in that the field-matter interaction is treated perturbatively and time-separated from physical processes in the absorbing matter. An open question is whether a fully quantum detector, whereby the optical field, the optical absorption, and the amplification are considered as one quantum system, could have improved performance. Here we develop a theoretical model of such photodetectors and employ simulations to reveal the critical role played by quantum coherence and amplification backaction in dictating the performance. We show that coherence and backaction lead to trade-offs between detector metrics and also determine optimal system designs through control of the quantum-classical interface. Importantly, we establish the design parameters that result in a ideal photodetector with 100% efficiency, no dark counts, and minimal jitter, thus paving the route for next-generation detectors.
Quantum mechanics cements the intimate relationship between the nature of light and its detection. Historically, quantum theories of photodetection have generally fallen into two categories: the first tries to determine what quantum field observable is measured when photoelectrons are detected, laying the theoretical groundwork for photodetection being possible. The second type are phenomenological theories, which take great care to model the details of specific photodetectors. In this dissertation, we fill in the gap between these two models in the modern literature on photodetection by constructing a fully quantum-mechanical and sufficiently realistic model that includes all stages of the photodetection process. We accomplish this within the framework of quantum information theory using the language of positive operator valued measures (POVMs). \n\nA POVM provides the most general description of a quantum measurement. In the context of single-photon detection, the photodetector POVM provides a complete characterization of the single-photon detector (SPD) from which all figures of merit can be calculated. Each element of the POVM is comprised of a weighted sum over single-photon state projectors. To construct SPD POVMs, we identify the states projected onto by a measurement and the associated weights. We first accomplish this for a simple time-dependent system, laying out how to efficiently project onto arbitrary single-photon states. Then, we describe the three stages of a realistic SPD: transmission, amplification, and measurement.\n\nIn the transmission stage of photodetection a photon enters a network of discrete energy levels, its energy propagating through that network and finally exiting into another output continuum of modes, a process entirely described by a single complex function. In the amplification stage of photodetection, a single excitation is amplified into a macroscopic signal via a nonlinear amplification mechanism. In the final stage, an inefficient ``classical'' measurement is made on the macroscopic signal. By combining these three stages we form a chain of inference from the final ``click'' to the input photon and construct a POVM projecting onto the input Hilbert space. Lastly, we discuss limits and tradeoffs that arise at each stage and implications for photodetection applications.\n\nThis dissertation contains previously published and unpublished material.
Quantum mechanics cements the intimate relationship between the nature of light and its detection. Historically, quantum theories of photodetection have generally fallen into two categories: the first tries to determine what quantum field observable is measured when photoelectrons are detected, laying the theoretical groundwork for photodetection being possible. The second type are phenomenological theories, which take great care to model the details of specific photodetectors. In this dissertation, we fill in the gap between these two models in the modern literature on photodetection by constructing a fully quantum mechanical and sufficiently realistic model that includes all stages of the photodetection process: transmission, amplification, and a final classical measurement. We accomplish this within the framework of quantum information theory using the language of positive operator valued measures (POVMs). This dissertation contains material previously published in three papers: Propp, Tz. B & van Enk, S. J. (2019). On nonlinear amplification: improved quantum limits for photon counting. Optics Express 27, 16, 23454-23463. Propp, Tz. B & van Enk, S. J. (2019). Quantum networks for single photon detection. Physical Review A, 100, 033836. Propp, Tz. B & van Enk, S. J. (2020). How to project onto an arbitrary single-photon wavepacket. Physical Review A, 102, 053707.
In optical quantum information processing, two of the most basic elements are the sources of quantum mechanical states of light, and the devices that can detect these states. In this chapter, we narrow this down to photon sources and photodetectors. We will describe first how detectors work, starting from abstract ideal detectors, via a complete description of realistic detectors in terms of POVMS, to a brief overview of current photodetectors. Subsequently, we will define what is a single-photon source, and how we can determine experimentally whether a source produces single photons or something else. Having laid down the ground rules, we will survey some of the most popular ways photons are produced in the laboratory. Finally, we take a look at the production of entangled photon sources and quantum non-demolition measurements of photons. A mathematical model of photodetectors Photodetectors are devices that produce a macroscopic signal when triggered by one or more photons. In the ideal situation, every photon that hits the detector contributes to the macroscopic signal, and there are no ‘ghost’ signals, or so-called dark counts. In this situation we can define two types of detector, namely the ‘photon-number detector’, and ‘detectors without number resolution’. First, the photon number detector is a (largely hypothetical) device that tells us how many photons there are in a given optical mode that is properly localized in space and time. This property is called ‘photon-number resolution’.
Abstract Single photon detectors play a key role across several basic science and technology applications. While progress has been made in improving performance, single photon detectors that can maintain high performance while also resolving the photon frequency are still lacking. By means of quantum simulations, we show that nanoscale elements cooperatively interacting with the photon field in a photodetector architecture allow to simultaneously achieve high efficiency, low jitter, and high frequency resolution. We discuss how such cooperative interactions are essential to reach this performance regime, analyzing the factors that impact performance and trade-offs between metrics. We illustrate the potential performance for frequency resolution over a 1 eV bandwidth in the visible range, indicating near perfect detection efficiency, jitter of a few hundred femtoseconds, and frequency resolution of tens of meV. Finally, a potential physical realization of such an architecture is presented based on carbon nanotubes functionalized with quantum dots.