Pyrochlore systems (A_{2}B_{2}O_{7}) with A-site rare-earth local moments and B-site 5d conduction electrons offer excellent material platforms for the discovery of exotic quantum many-body ground states. Notable examples include U(1) quantum spin liquid of the local moments and semimetallic non-Fermi liquid of the conduction electrons. Here we investigate emergent quantum phases and their transitions driven by the Kondo lattice coupling between such highly entangled quantum ground states. Using the renormalization group method, it is shown that weak Kondo lattice coupling is irrelevant, leading to a fractionalized semimetal phase with decoupled local moments and conduction electrons. Upon increasing the Kondo lattice coupling, this phase is unstable to the formation of broken symmetry states. Particularly important is the opposing influence of the Kondo lattice coupling and long-range Coulomb interaction. The former prefers to break the particle-hole symmetry while the latter tends to restore it. The characteristic competition leads to possibly multiple phase transitions, first from a fractionalized semimetal phase to a fractionalized Fermi surface state with particle-hole pockets, followed by the second transition to a fractionalized ferromagnetic state. Multiscale quantum critical behaviors appear at nonzero temperatures and with external magnetic field near such quantum phase transitions. We discuss the implication of these results to the experiments on Pr_{2}Ir_{2}O_{7}.
Pyrochlore systems (A_{2}B_{2}O_{7}) with A-site rare-earth local moments and B-site 5d conduction electrons offer excellent material platforms for the discovery of exotic quantum many-body ground states. Notable examples include U(1) quantum spin liquid of the local moments and semimetallic non-Fermi liquid of the conduction electrons. Here we investigate emergent quantum phases and their transitions driven by the Kondo lattice coupling between such highly entangled quantum ground states. Using the renormalization group method, it is shown that weak Kondo lattice coupling is irrelevant, leading to a fractionalized semimetal phase with decoupled local moments and conduction electrons. Upon increasing the Kondo lattice coupling, this phase is unstable to the formation of broken symmetry states. Particularly important is the opposing influence of the Kondo lattice coupling and long-range Coulomb interaction. The former prefers to break the particle-hole symmetry while the latter tends to restore it. The characteristic competition leads to possibly multiple phase transitions, first from a fractionalized semimetal phase to a fractionalized Fermi surface state with particle-hole pockets, followed by the second transition to a fractionalized ferromagnetic state. Multiscale quantum critical behaviors appear at nonzero temperatures and with external magnetic field near such quantum phase transitions. We discuss the implication of these results to the experiments on Pr_{2}Ir_{2}O_{7}.
In this thesis, several cases of non-equilibrium phenomena and quantum phase transitions in strongly correlated electron systems are analyzed. The unconventional critical behavior near magnetic quantum phase transitions in various heavy-fermion metals has triggered proposals on the breakdown of the Kondo effect at the critical point. In part I, we investigate, within one specific scenario, the fate of such a zero-temperature transition upon coupling of the electronic to lattice degrees of freedom. We study a Kondo-Heisenberg model with volume-dependent Kondo coupling � this model displays both Kondo volume collapse and Kondo-breakdown transitions. Within a large-N treatment, we find that the Kondo breakdown transition remains of second order except for very soft lattices. Finally, we relate our findings to current heavy-fermion experiments. Using non-equilibrium Green�s functions, we derive transport equations for the degrees of freedom participating in the quantum critical region of the Kondo breakdown transition. We discuss conditions under which the transport of electrical charge is described by the independent motion of conduction electrons and auxiliary bosons. Under these conditions, we derive a semiclassical transport equation for the bosons and quantitatively discuss the electrical conductivity of the whole system. Motivated by pressure experiments on FeAs-122 superconductors, in part II we propose a scenario based on local-moment physics to explain salient features at the magnetic phase boundary of CaFe2As2. In this scenario, the low-pressure magnetic phase derives from Fe moments, which become screened in the paramagnetic high-pressure phase. The quantum phase transition can be described as an orbital-selective Mott transition, which is rendered first order by coupling to the lattice. These ideas are illustrated by a suitable mean-field analysis of an Anderson lattice model. An analytical description of non-equilibrium phenomena in interacting quantum systems is rarely possible. In part III we present one example where such a description can be achieved, namely the ferromagnetic Kondo model. In equilibrium, this model is tractable via perturbative renormalization-group techniques. We employ a recently developed extension of the flow-equation method to calculate the non-equilibrium decay of the local magnetization at zero temperature. The flow equations admit analytical solutions which become exact at short and long times, in the latter case revealing that the system always retains a memory of its initial state. Finally, in part IV we analyze the Nernst effect resulting from normal state quasiparticles in the cuprates in presence of various types of translational symmetry breaking. In the electron-doped cuprates, the Nernst signal resulting from a reconstruction of the Fermi surface due to spin density wave order is discussed. An order parameter consistent with the reconstruction of the Fermi surface detected in electron-doped materials is shown to sharply enhance the Nernst signal close to optimal doping. Within a semiclassical treatment, the obtained magnitude and position of the enhanced Nernst signal agrees with Nernst measurements in electron-doped cuprates. In the hole-doped cuprates, we discuss relations between the normal-state Nernst effect and stripe order. We find that Fermi pockets caused by translational symmetry breaking lead to a strongly enhanced Nernst signal with a sign depending on the modulation period of the ordered state and other details of the Fermi surface. This implies differences between antiferromagnetic and charge-only stripes. We compare our findings with recent data from La1.6−xNd0.4SrxCuO4 and YBa2Cu3Oy.
Quantum criticality, a manifestation of emergent scale invariance in electron wavefunctions arises from intricate many-body quantum entanglement. One of the natural venues for the criticality is clean undoped Dirac semimetals, known as a marginally-renormalized critical phase. The ground state is only slightly modified from the Slater-type product wavefunction because the scatterings from weak disorder and Coulomb interactions are suppressed. Here, using the renormalization group (RG) analysis, we show that a novel class of quantum criticality appears in Dirac semimetals when the disorder strength becomes sufficiently strong in the presence of Coulomb interactions so that a quantum phase transition from the marginally-renormalized critical phase to a disorder-dominated phase arises. The ground state at the critical point is a quantum critical non-Fermi liquid (NFL), characterized by the properties of strongly entangled low-energy states such as the absence of quasi-particles. Near the critical point, unusually wide temperature regions with NFL behaviors emerge.
There has been significant recent interest in the potential exotic properties of multichannel Kondo lattices and their connection to quantum materials, but the strongly coupled nature of these models has posed challenges to theoretical investigations. We study the emergence of topological order in a two-dimensional two-channel Kondo lattice (2CKL) in a time-reversal symmetry-broken channel symmetric phase using a coupled-wire construction from one-dimensional (1D) 2CKLs. Through bosonization and symmetry analysis, we show that away from particle-hole symmetry, the 1D 2CKL model flows to an infrared fixed point with an emergent $\mathrm{SO}(3,1)\ifmmode\times\else\texttimes\fi{}\mathrm{SU}(2)$ symmetry and a Z2 gauge structure. Interwire couplings induce a transition to a topologically ordered metallic state characterized by fractionalized excitations and eightfold ground state degeneracy on a torus. Our findings connect impurity-based non-Fermi-liquid behavior to lattice topological order, with potential implications for quantum materials and topological quantum computation.
The physical properties of a material tuned to the cusp between two distinct ground states can be quite exotic, and unlike those in either of the neighboring phases. The prospect of capturing such behavior in a simple model is tantalizing; for example, the interplay between heavy fermion physics and magnetic ordering in certain materials is often rationalized in terms of the quantum phase transition in the two-impurity Kondo model. However, this model is oversimplified for the purpose: its quantum critical point does not reflect the distinctive properties of a magnetic lattice surrounded by mobile electrons. In this work, we study a tunable nanoelectronic circuit comprising two coupled charge-Kondo quantum islands, realizing a new model which captures the essence of competition between local and collective screening of magnetic moments. This may have relevance for materials in which collective many-body effects drive lattice coherence. We tune our device to a novel quantum critical point, and show experimentally that deviations as we tune away from this point match non-trivial predictions from the model. This work on the crucial role of inter-island interactions is a necessary first step in scaling up such circuits from individual sites to networks or lattices.
Quantum phase transitions out of equilibrium are outstanding emergent subjects in condensed matter physics with great fundamental importance and challenges. We theoretically investigate here the nonequilibrium quantum phase transition in a generic nano-setup: the pseudogap Kondo model where a Kondo quantum dot couples to two---left (L) and right (R)---voltage-biased fermionic leads with power-law density of states (DOS) with respect to their Fermi levels ${\ensuremath{\mu}}_{L/R}$, ${\ensuremath{\rho}}_{c,L(R)}(\ensuremath{\omega})\ensuremath{\propto}{|\ensuremath{\omega}\ensuremath{-}{\ensuremath{\mu}}_{L(R)}|}^{r}$ with 0<r<1. In equilibrium (${\ensuremath{\mu}}_{L}\ensuremath{-}{\ensuremath{\mu}}_{R}=0$) and for 0<r<1/2, with increasing Kondo correlations this model exhibits a quantum phase transition from a unscreened local moment (LM) phase to the Kondo screened phase. At finite bias voltages and near criticality, we discover new nonequilibrium universal scaling behaviors in conductance, conduction electron T matrix, and local spin susceptibility via a controlled frequency-dependent renormalization group (RG) approach. The current-induced decoherence is key to understanding these distinct universal nonequilibrium quantum critical regimes. The relevance of our results to experiment is discussed.
We study the competition between Kondo physics and dissipation within an Anderson model of a magnetic impurity level that hybridizes with a metallic host and is also coupled, via the impurity charge, to the displacement of a bosonic bath having a spectral density proportional to ${\ensuremath{\omega}}^{s}$. As the impurity-bath coupling increases from zero, the effective Coulomb interaction between two electrons in the impurity level is progressively renormalized from its repulsive bare value until it eventually becomes attractive. For weak hybridization, this renormalization in turn produces a crossover from a conventional spin-sector Kondo effect to a charge Kondo effect. At particle-hole symmetry, and for sub-Ohmic bath exponents 0<s<1, further increase in the impurity-bath coupling results in a continuous zero-temperature transition to a broken-symmetry phase in which the ground-state impurity occupancy ${\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{n}}_{d}$ acquires an expectation value ${⟨{\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{n}}_{d}⟩}_{0}\ensuremath{\ne}1$. The response of the impurity occupancy to a locally applied electric potential features the hyperscaling of critical exponents and $\ensuremath{\omega}∕T$ scaling that are expected at an interacting critical point. The numerical values of the critical exponents suggest that the transition lies in the same universality class as that of the sub-Ohmic spin-boson model. For the Ohmic case s=1, the transition is instead of Kosterlitz-Thouless type. Away from particle-hole symmetry, the quantum phase transition is replaced by a smooth crossover but signatures of the symmetric quantum critical point remain in the physical properties at elevated temperatures and/or frequencies.