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arXiv:1107.2195 · Physical Review B

Quantum criticality out of equilibrium in the pseudogap Kondo model

Chung‐Hou Chung, Kenneth Yi-Jie Zhang

Published May 3, 2012• 5 citations
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Abstract

Quantum phase transitions out of equilibrium are outstanding emergent subjects in condensed matter physics with great fundamental importance and challenges. We theoretically investigate here the nonequilibrium quantum phase transition in a generic nano-setup: the pseudogap Kondo model where a Kondo quantum dot couples to two---left (L) and right (R)---voltage-biased fermionic leads with power-law density of states (DOS) with respect to their Fermi levels ${\ensuremath{\mu}}_{L/R}$, ${\ensuremath{\rho}}_{c,L(R)}(\ensuremath{\omega})\ensuremath{\propto}{|\ensuremath{\omega}\ensuremath{-}{\ensuremath{\mu}}_{L(R)}|}^{r}$ with $0<r<1$. In equilibrium (${\ensuremath{\mu}}_{L}\ensuremath{-}{\ensuremath{\mu}}_{R}=0$) and for $0<r<1/2$, with increasing Kondo correlations this model exhibits a quantum phase transition from a unscreened local moment (LM) phase to the Kondo screened phase. At finite bias voltages and near criticality, we discover new nonequilibrium universal scaling behaviors in conductance, conduction electron $T$ matrix, and local spin susceptibility via a controlled frequency-dependent renormalization group (RG) approach. The current-induced decoherence is key to understanding these distinct universal nonequilibrium quantum critical regimes. The relevance of our results to experiment is discussed.

DOI
10.1103/physrevb.85.195106

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Quantum phase transitions out of equilibrium are outstanding emergent subjects in condensed matter physics with great fundamental importance and challenges. We theoretically investigate here the nonequilibrium quantum phase transition in a generic nano-setup: the pseudogap Kondo model where a Kondo quantum dot couples to two---left (L) and right (R)---voltage-biased fermionic leads with power-law density of states (DOS) with respect to their Fermi levels \ensuremathμL/R{\ensuremath{\mu}}_{L/R}\ensuremathμL/R​, \ensuremathρc,L(R)(\ensuremathω)\ensuremath∝∣\ensuremathω\ensuremath−\ensuremathμL(R)∣r{\ensuremath{\rho}}_{c,L(R)}(\ensuremath{\omega})\ensuremath{\propto}{|\ensuremath{\omega}\ensuremath{-}{\ensuremath{\mu}}_{L(R)}|}^{r}\ensuremathρc,L(R)​(\ensuremathω)\ensuremath∝∣\ensuremathω\ensuremath−\ensuremathμL(R)​∣r with 0<r<10<r<10<r<1. In equilibrium (\ensuremathμL\ensuremath−\ensuremathμR=0{\ensuremath{\mu}}_{L}\ensuremath{-}{\ensuremath{\mu}}_{R}=0\ensuremathμL​\ensuremath−\ensuremathμR​=0) and for 0<r<1/20<r<1/20<r<1/2, with increasing Kondo correlations this model exhibits a quantum phase transition from a unscreened local moment (LM) phase to the Kondo screened phase. At finite bias voltages and near criticality, we discover new nonequilibrium universal scaling behaviors in conductance, conduction electron TTT matrix, and local spin susceptibility via a controlled frequency-dependent renormalization group (RG) approach. The current-induced decoherence is key to understanding these distinct universal nonequilibrium quantum critical regimes. The relevance of our results to experiment is discussed.
The quantum criticality of the two-lead two-channel pseudogap Anderson impurity model is studied. Based on the non-crossing approximation (NCA) and numerical renormalization group (NRG) approaches, we calculate both the linear and nonlinear conductance of the model at finite temperatures with a voltage bias and a power-law vanishing conduction electron density of states, ρc(ω) proportional |ω − μF|(r) (0 < r < 1) near the Fermi energy μF. At a fixed lead-impurity hybridization, a quantum phase transition from the two-channel Kondo (2CK) to the local moment (LM) phase is observed with increasing r from r = 0 to r = rc < 1. Surprisingly, in the 2CK phase, different power-law scalings from the well-known [Formula: see text] or [Formula: see text] form is found. Moreover, novel power-law scalings in conductances at the 2CK-LM quantum critical point are identified. Clear distinctions are found on the critical exponents between linear and non-linear conductance at criticality. The implications of these two distinct quantum critical properties for the non-equilibrium quantum criticality in general are discussed.
Correlations are a central ingredient of modern condensed matter physics. With the advent of mesoscopic physics, it became possible to study correlated systems in non-equilibrium situations, which can be reached by e.g. driving a constant current through a quantum dot. A basic question is how correlations on the one hand and a non-equilibrium current on the other hand influence each other. Here this interplay is studied for the model system of a quantum dot in the Kondo regime using the real time renormalization group (RTRG) method. This method is a functional renormalization group (RG) method allowing a non-perturbative description of correlated systems in non-equilibrium. For the Kondo quantum dot the method is generalized to the case of double vertices. The RTRG method not only provides equations for the calculation of the renormalized coupling between the quantum dot spin and the reservoir electrons, but also equations for the calculation of the non-equilibrium decoherence rate and the non-equilibrium current.The RG equations are derived to second order. This approximation is expected to be valid as long as the quantum dot does not enter the strong coupling regime, i.e. the effective coupling strength between the quantum dot spin and the electrons does not become too large. It is found that this is the case if the bias voltage applied to the dot or the temperature is much larger than the Kondo temperature.It is shown that the RG equations lead to coupling functions depending on the energy of the incident and the scattered electron. This dependence is simplified to the dependence on the average energy of the incident and the scattered electron in the weak coupling regime.A closer inspection of the RG equations for the couplings shows that they not only contain terms leading to a logarithmic increase of the coupling strength but also subleading terms which are unimportant in the weak coupling regime. The RG equations are solved analytically for the case where the subleading terms are neglected. It is found that the coupling functions develop resonances at energies associated with the chemical potentials of the reservoirs. The height of these resonances is determined by the decoherence rate. However, for bias voltages much larger than the Kondo temperature these resonances do not affect the conductance for a two terminal setup, so the conductance does not provide a measure for the decoherence rate in this case. It is found that the conductance for the two terminal setup is a universal function of voltage/Kondo temperature and temperature/Kondo temperature in the weak coupling regime. This function is calculated analytically in the limits of vanishing voltage or temperature. Furthermore, it is found that for zero temperature the decoherence rate is proportional to the non-equilibrium current flowing through the system. This supports the physical picture that a non-equilibrium current is associated with a decoherence rate, which cuts the logarithmic scaling of the coupling strength.Finally, the RG equations are solved numerically for zero temperature including the subleading corrections found before. As expected, the subleading corrections have no impact on the decoherence rate and the conductance in the weak coupling regime. On the other hand, it is found that they lead to strong deviations from the results of the analytic leading logarithmic approximation if the bias voltage approaches the Kondo temperature. Generally, it is found that the subleading corrections lead to a saturation of the decoherence rate and the conductance to some finite value. However, for the numerical solution a numerical regularization parameter has to be introduced. It turns out that the saturation value found depends on its value, so no statements on the precise value of the decoherence rate and the current can be made in this regime.
We study equilibrium and nonequilibrium properties of the single-impurity Anderson model with a power-law pseudogap in the density of states. In equilibrium, the model is known to display a quantum phase transition from a generalized Kondo to a local moment phase. In the present work, we focus on the extension of these phases beyond equilibrium, i.e., under the influence of a bias voltage. Within the auxiliary master equation approach combined with a scheme based on matrix product states (MPS) we are able to directly address the current-carrying steady state. Starting with the equilibrium situation, we first corroborate our results by comparing to a direct numerical evaluation of ground-state spectral properties of the system by MPS. Here, a scheme to locate the phase boundary by extrapolating the power-law exponent of the self energy produces a very good agreement with previous results obtained by the numerical renormalization group. Our nonequilibrium study as a function of the applied bias voltage is then carried out for two points on either side of the phase boundary. In the Kondo regime the resonance in the spectral function is split as a function of the increasing bias voltage. The local moment regime, instead, displays a dip in the spectrum near the position of the chemical potentials. Similar features are observed in the corresponding self energies. The Kondo split peaks approximately obey a power-law behavior as a function of frequency whose exponents depend only slightly on voltage. Finally, the differential conductance in the Kondo regime shows a peculiar maximum at finite voltages, whose height, however, is below the accuracy level.
We investigate the critical behavior of the Kondo compensation in the presence of a power-law pseudogap in the density of states, $\ensuremath{\rho}(\ensuremath{\omega})\ensuremath{\sim}{|\ensuremath{\omega}|}^{\ensuremath{\epsilon}}$. For $\ensuremath{\epsilon}<1$, generically---in the absence of particle-hole symmetry---this model exhibits a quantum phase transition from a partially screened doublet ground state to a fully screened many-body ground state upon increasing the exchange coupling jjj. At the critical point jc{j}_{\text{c}}jc​, the Kondo compensation is found to scale as $\ensuremath{\kappa}(j<{j}_{\text{c}})=1\ensuremath{-}g(j)$ with the local ggg-factor vanishing as $g\ensuremath{\sim}|j\ensuremath{-}{j}_{\text{c}}{|}^{\ensuremath{\beta}}$. We combine the perturbative drone fermion method with the nonperturbative numerical renormalization group computations to determine the critical exponent $\ensuremath{\beta}(\ensuremath{\epsilon})$, which exhibits a nonmonotonous behavior as a function of $\ensuremath{\epsilon}$. Our results confirm that the Kondo cloud builds up continuously in the presence of a weak pseudogap as one approaches the phase transition.
We study the out-of-equilibrium steady-state properties of the Bose-Fermi-Kondo model, describing a local magnetic moment coupled to two ferromagnetic leads that support bosonic (magnons) and fermionic (Stoner continuum electrons) low-energy excitations. This model describes the destruction of the Kondo effect as the coupling to the bosons is increased. Its phase diagram comprises three non-trivial fixed points. Using a dynamical large-N approach on the Keldysh contour, we study two different non-equilibrium setups: a) a finite bias voltage and b) a finite temperature gradient, imposed across the leads. The scaling behavior of the charge and energy currents is identified and characterized for all fixed points. We report the existence of a fixed-point-dependent effective temperature, defined though the fluctuation-dissipation relations of the local spin-susceptibility in the scaling regime, which permits to recover the equilibrium behavior of both dynamical and static spin-susceptibilities. Copyright (c) EPLA, 2013
We study the out-of-equilibrium steady-state properties of the Bose-Fermi-Kondo model, describing a local magnetic moment coupled to two ferromagnetic leads that support bosonic (magnons) and fermionic (Stoner continuum electrons) low-energy excitations. This model describes the destruction of the Kondo effect as the coupling to the bosons is increased. Its phase diagram comprises three non-trivial fixed points. Using a dynamical large- N approach on the Keldysh contour, we study two different non-equilibrium setups: a) a finite bias voltage and b) a finite temperature gradient, imposed across the leads. The scaling behavior of the charge and energy currents is identified and characterized for all fixed points. We report the existence of a fixed-point–dependent effective temperature, defined though the fluctuation-dissipation relations of the local spin-susceptibility in the scaling regime, which permits to recover the equilibrium behavior of both dynamical and static spin-susceptibilities.