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arXiv:1810.11086 · Physical Review Letters

Sign-Changing Photon-Mediated Atom Interactions in Multimode Cavity Quantum Electrodynamics

Yudan Guo, Ronen M. Kroeze, Varun Vaidya, Jonathan Keeling, Benjamin Lev

Published May 14, 2019• 79 citations
arXivHTMLPDF

Abstract

Sign-changing interactions constitute a crucial ingredient in the creation of frustrated many-body systems such as spin glasses. We present here the demonstration of a photon-mediated sign-changing interaction between Bose-Einstein-condensed atoms in a confocal cavity. The interaction between two atoms is of an unusual, nonlocal form proportional to the cosine of the inner product of the atoms' position vectors. This interaction arises from the differing Gouy phase shifts of the cavity's degenerate modes. The interaction drives a nonequilibrium Dicke-type phase transition in the system leading to atomic checkerboard density-wave order. Because of the Gouy phase anomalies, the checkerboard pattern can assume either a sinelike or cosinelike character. This state is detected via the holographic imaging of the cavity's superradiant emission. Together with a companion paper [Y. Guo, V. D. Vaidya, R. M. Kroeze, R. A. Lunney, B. L. Lev, and J. Keeling, Emergent and broken symmetries of atomic self-organization arising from Gouy phases in multimode cavity QED, Phys. Rev. A 99, 053818 (2019)PLRAAN2469-992610.1103/PhysRevA.99.053818], we explore this interaction's influence on superradiant phase transitions in multimode cavities. Employing this interaction in cavity QED spin systems may enable the creation of artificial spin glasses and quantum neural networks.

DOI
10.1103/physrevlett.122.193601

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•Sep 18, 2012•0 citations
Sign-changing interactions constitute a crucial ingredient in the creation of frustrated many-body systems such as spin glasses. We present here the demonstration of a photon-mediated sign-changing interaction between Bose-Einstein-condensed atoms in a confocal cavity. The interaction between two atoms is of an unusual, nonlocal form proportional to the cosine of the inner product of the atoms' position vectors. This interaction arises from the differing Gouy phase shifts of the cavity's degenerate modes. The interaction drives a nonequilibrium Dicke-type phase transition in the system leading to atomic checkerboard density-wave order. Because of the Gouy phase anomalies, the checkerboard pattern can assume either a sinelike or cosinelike character. This state is detected via the holographic imaging of the cavity's superradiant emission. Together with a companion paper [Y. Guo, V. D. Vaidya, R. M. Kroeze, R. A. Lunney, B. L. Lev, and J. Keeling, Emergent and broken symmetries of atomic self-organization arising from Gouy phases in multimode cavity QED, Phys. Rev. A 99, 053818 (2019)PLRAAN2469-992610.1103/PhysRevA.99.053818], we explore this interaction's influence on superradiant phase transitions in multimode cavities. Employing this interaction in cavity QED spin systems may enable the creation of artificial spin glasses and quantum neural networks.
We report on the first experimental realization of the Dicke quantum phase transition realized in the quantum motion of a Bose–Einstein condensate coupled to an optical cavity. Conceptually, the transition is driven by cavity-mediated long-range interactions, giving rise to the emergence of a self-organized supersolid phase. The Dicke phase transition, predicted in 1973, has not been demonstrated experimentally before this work, both due to fundamental and technological reasons. These challenges have been overcome in the present thesis by employing atomic momentum states of a Bose-Einstein condensate, which are coupled via two-photon Raman transitions involving a cavity photon and a free-space pump photon. This open-system implementation of the Dicke model allows to tune all relevant parameters and offers a unique detection scheme to monitor the manybody system in real time. We demonstrate that the phase transition is accompanied by a macroscopically occupied cavity field and a striking change in the atomic momentum distribution, due to spontaneous self-organization of the atomic density on a checkerboard lattice. The boundary of the transition is mapped out by scanning two parameters of the Dicke model, to reveal a phase diagram in close agreement with the model description. Two different ordered configurations are allowed in the superradiant phase, giving rise to the concept of spontaneous symmetry breaking at the phase transition. We experimentally distinguish the symmetry-broken states and study the origin of the symmetry-breaking process. The finite spatial extension of our system induces a small symmetry-breaking field which changes randomly on each experimental realization. The influence of this field is studied and shown to diminish upon dynamically crossing the transition point with increasing transition rates.
In the context of ultracold atoms in multimode optical cavities, the appearance of a quantum-critical glass phase of atomic spins has been predicted recently. Due to the long-range nature of the cavity-mediated interactions, but also the presence of a driving laser and dissipative processes such as cavity photon loss, the quantum optical realization of glassy physics has no analog in condensed matter and could evolve into a ``cavity glass microscope'' for frustrated quantum systems out of equilibrium. Here we develop the nonequilibrium theory of the multimode Dicke model with quenched disorder and Markovian dissipation. Using a unified Keldysh path integral approach, we show that the defining features of a low-temperature glass, representing a critical phase of matter with algebraically decaying temporal correlation functions, are seen to be robust against the presence of dissipation due to cavity loss. The universality class, however, is modified due to the Markovian bath. The presence of strong disorder leads to an enhanced equilibration of atomic and photonic degrees of freedom, including the emergence of a common low-frequency effective temperature. The imprint of the atomic spin-glass physics onto the photon subsystem realizes a ``photon glass'' state and makes it possible to detect the glass state by standard experimental techniques of quantum optics. We provide an unambiguous characterization of the superradiant and glassy phases in terms of fluorescence spectroscopy, homodyne detection, and the temporal photon correlation function ${g}^{(2)}(\ensuremath{\tau})$.
Ultracold atoms trapped in laser-generated optical lattices serve as a versatile platform for quantum simulations. However, as these lattices are infinitely stiff, they do not allow to emulate phonon degrees of freedom. This restriction can be lifted in emerged optical lattices inside multimode cavities. Motivated by recent experimental progress in multimode cavity QED, we propose a scheme to implement and study supersolid and droplet states with phononlike lattice excitations by coupling a Bose gas to many longitudinal modes of a ring cavity. The interplay between contact collisional and tunable-range cavity-mediated interactions leads to a rich phase diagram, which includes elastic supersolid as well as insulating droplet phases exhibiting roton-type mode softening for a continuous range of momenta across the superradiant phase transition. The nontrivial dynamic response of the system to a local density perturbation further proves the existence of phononlike modes.
We observe the joint spin-spatial (spinor) self-organization of a two-component Bose-Einstein condensate (BEC) strongly coupled to an optical cavity. This unusual nonequilibrium Hepp-Lieb-Dicke phase transition is driven by an off-resonant Raman transition formed from a classical pump field and the emergent quantum dynamical cavity field. This mediates a spinor-spinor interaction that, above a critical strength, simultaneously organizes opposite spinor states of the BEC on opposite checkerboard configurations of an emergent 2D lattice. The resulting spinor density-wave polariton condensate is observed by directly detecting the atomic spin and momentum state and by holographically reconstructing the phase of the emitted cavity field. The latter provides a direct measure of the spin state, and a spin-spatial domain wall is observed. The photon-mediated spin interactions demonstrated here may be engineered to create dynamical gauge fields and quantum spin glasses.
"Spatially modulated ordered states, such as crystals, liquid crystals, and antiferromagnets, are ubiquitous in nature but relatively difficult to realize in ultracold atomic systems. In the present work, we present a scheme for generating controllable cavity-mediated interactions between atoms, and show that these interactions give rise to a crystallization transition in the case of a transversely pumped optical cavity. We focus on the case of multimode cavities, in which the interactions are relatively local and the range of possible ordered configurations (and consequently of low-energy fluctuations) is large; as we show, the crystallization transition for a Bose-Einstein condensate in a multimode cavity is driven first-order by fluctuations, through the Brazovskii effect. The ordered state to which this crystallization transition gives rise is a ""supersolid,"" possessing both superfluid and solid order. We address the crystallization transition and the properties of the ordered state, discuss the experimental feasibility of observing these, and finally show how ordering in layered systems of atoms is geometrically frustrated. We then introduce a more straightforward realization of frustrated cavity-mediated interactions, viz. systems of randomly-positioned spins in multimode cavities. We show by means of a mapping to a variant of the Hopfield associative-memory model that such systems exhibit a spin-glass phase. Finally, we consider a different ultracold-atomic setting---that of spin-orbit-coupled Bose gases---in which the Brazovskii effect has a profound influence on the low-temperature phases, leading to a universal preference for stripe-like ordering at zero temperature and bosonic pair condensation at nonzero temperatures."