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arXiv:1810.10385

Design, Fabrication and Characterization of nanoplasmonic lattice for trapping of ultracold atoms

Sunil Kumar, Manav Shah, Ajith Padyana Ravishankar, Chetan Vishwakarma, Arindam Dasgupta, Jay Mangaonkar, Venu Gopal Achanta, Umakant D. Rapol

Published Oct 24, 2018• 0 citations
arXivHTMLPDF

Abstract

Ultracold atom-traps on a chip enhances the practical application of atom traps in quantum information processing, sensing, and metrology. Plasmon mediated near-field optical potentials are promising for trapping atoms. The combination of plasmonic nanostructures and ultracold atoms has the potential to create a two dimensional array of neutral atoms with lattice spacing smaller than that of lattices created from interfering light fields -- the optical lattices. We report the design, fabrication and characterization of a nano-scale array of near-field optical traps for neutral atoms using plasmonic nanostructures. The building block of the array is a metallic nano-disc fabricated on the surface of an ITO-coated glass substrate. We numerically simulate the electromagnetic field-distribution using Finite Difference Time Domain method around the nanodisc, and calculate the intensity, optical potential and the dipole force for $^{87}$Rb atoms. The optical near-field generated from the fabricated nanostructures is experimentally characterized by using Near-field Scanning Optical Microscopy. We find that the optical potential and dipole force has all the desired characteristics to trap cold atoms when a blue-detuned light-field is used to excite the nanostructures. This trap can be used for effective trapping and manipulation of isolated atoms and also for creating a lattice of neutral atoms having sub-optical wavelength lattice spacing. Near-field measurements are affected by the influence of tip on the sub-wavelength structure. We present a deconvolution method to extract the actual near-field profile from the measured data.

DOI
10.48550/arxiv.1810.10385

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Ultracold atom-traps on a chip enhances the practical application of atom traps in quantum information processing, sensing, and metrology. Plasmon mediated near-field optical potentials are promising for trapping atoms. The combination of plasmonic nanostructures and ultracold atoms has the potential to create a two dimensional array of neutral atoms with lattice spacing smaller than that of lattices created from interfering light fields -- the optical lattices. We report the design, fabrication and characterization of a nano-scale array of near-field optical traps for neutral atoms using plasmonic nanostructures. The building block of the array is a metallic nano-disc fabricated on the surface of an ITO-coated glass substrate. We numerically simulate the electromagnetic field-distribution using Finite Difference Time Domain method around the nanodisc, and calculate the intensity, optical potential and the dipole force for 87^{87}87Rb atoms. The optical near-field generated from the fabricated nanostructures is experimentally characterized by using Near-field Scanning Optical Microscopy. We find that the optical potential and dipole force has all the desired characteristics to trap cold atoms when a blue-detuned light-field is used to excite the nanostructures. This trap can be used for effective trapping and manipulation of isolated atoms and also for creating a lattice of neutral atoms having sub-optical wavelength lattice spacing. Near-field measurements are affected by the influence of tip on the sub-wavelength structure. We present a deconvolution method to extract the actual near-field profile from the measured data.
We propose a scheme to tailor nanostructured trapping potentials for ultracold atoms. Our trapping scheme combines an engineered extension of repulsive optical dipole forces at short distances and attractive Casimir-Polder forces at long distances between an atom and a nanostructured surface. This extended dipole force scheme takes advantage of excited-state dressing by plasmonically-enhanced optical fields to doubly dress the ground state and create a strongly repulsive potential with spatially tunable characteristics. In this paper, we show that, under realistic experimental conditions, this method can be used to trap Rubidium atoms close to surfaces (tens of nanometers). The influence of the various losses and heating rate mechanism in such traps is characterized. As an example we present a near-field optical lattice with subwavelength period (100 nm) and study the tunability of lattice and trapping depths. Such lattices can enhance energy scales with interesting perspectives for the simulation of strongly-correlated physics. Our method can be extended to other atomic species and to other cold atom near-field hybrid systems.
Abstract This paper reports on conceptual and experimental work towards the realization of plasmonic surface traps for cold atoms. The trapping mechanism is based on the combination of a repulsive and an attractive potential generated by evanescent light waves that are plasmonically enhanced. The strength of enhancement can be locally manipulated via the thickness of a metal nanolayer deposited on top of a dielectric substrate. Thus, in principle the trapping geometry can be predefined by the metal layer design. We present simulations of a plasmonic lattice potential using a gold grating with sinusoidally modulated thickness. Experimentally, a first plasmonic test structure is presented and characterized. Furthermore, the surface potential landscape is detected by reflecting ultracold atom clouds from the test structure revealing the influence of both evanescent waves. A parameter range is identified where stable traps can be expected.
We theoretically propose blue-detuned optical trapping for neutral atoms via strong near-field interfacing in a plasmonic nanohole array. The optical field at resonance forms a nanoscale-trap potential with an FWHM of 200 nm and about ∼370  nm away from the nanohole; thus, a stable 3D atom trapping independent of the surface potential is demonstrated. The effective trap depth is more than 1 mK when the optical power of trapping light is only about 0.5 mW, while the atom scattering rate is merely about 3.31  s−1, and the trap lifetime is about 800 s. This compact plasmonic structure provides high uniformity of trap depths and a two-layer array of atom nanotraps, which should have important applications in the manipulation of cold atoms and collective resonance fluorescence.
The entry into the new millennium was marked in the quantum community by the first experimental realizations of the Bose-Einstein condensation of atoms in a vapor, achieved in different research groups. Twenty-five years later, such systems are 'routinely' produced and are the core of many experiments. At the frontier between condensed matter their y, quantum optics, and atomic physics, ultra-cold atoms are subjects of high scientific interest.Ultra-cold gas can be trapped in optical lattices, giving a realistic way of experimentally realizing a new range of lattice Hamiltonians, that are used to simulate condensed matter systems. In these simulations, ultra-cold atoms are used to mimic the behavior of electrons in a solid-state material and could be used to simulate a wide range of complex condensed matter phenomena, such as the fractional quantum Hall effect, topological insulators, and high-temperature superconductivity.In order to study such systems, diffraction-limited quantum gas microscopes have emerged as a way to manipulate and detect atoms trapped in lattice potentials. Using far-field interference, experiments have mainly been restricted to a lattice spacing of 500 nm. This limits the speed of dynamics of all physical processes.Higher energy regimes could be accessed by reducing the lattice spacing. For this purpose, one of the long-term goals of the team is to trap atoms in the near-field of a surface and to make use of the Casimir-Polder forces to shape sub-wavelength potentials. Thanks to nano-fabrication capabilities, the spacing can be reduced to a few tens of nanometers. However, this requires to adapt the imaging techniques to observe cold-atoms with sub-wavelength spatial resolutions.In this PhD thesis, I report first on the advances toward implementing an atom chip in our experiment, which will serve as an integrated platform to manipulate the quantum gas. I present simulations and study an experimental solution allowing the cloud to be transported to the near-field. The method is based on the interference of a laser radiation in the near field of a rotating surface. It has been fully simulated, and the limitations have been numerically and experimentally assessed. I conclude this part by presenting the first model of chip that has been fabricated.In a second part, I report on the development of a sub-wavelength imaging method of cold Rubidium 87 atoms which is based on excited state dressing. I detail the concept of this nano-metric spatial resolution method and apply it to super-resolve a single longitudinal wave function trapped in a tight lattice that exhibits a width below 30 nm.
We propose to use subwavelength confinement of light associated with the near field of plasmonic systems to create nanoscale optical lattices for ultracold atoms. Our approach combines the unique coherence properties of isolated atoms with the subwavelength manipulation and strong light-matter interaction associated with nanoplasmonic systems. It allows one to considerably increase the energy scales in the realization of Hubbard models and to engineer effective long-range interactions in coherent and dissipative many-body dynamics. Realistic imperfections and potential applications are discussed.
We describe several novel techniques for the optical trapping of ultracold atoms and for the production of wavelength-stabilised, coherent light at the frequencies required for use in atomic physics experiments. The greater part of this thesis deals with work towards the creation of regular arrays of microscopic optical dipole traps formed at the foci of truncated spherical cavities in a metallic film, in which the inter-site spacing can be set anywhere between one and several hundred micrometers. Arrays of such cavities are synthesised and structurally characterised via optical and electron microscopy, and numerical simulations of the light intensity distribution near the foci of such cavities under normal illumination are used to confirm their suitability for dipole trap production. A method for the construction of arrays of magneto-optical traps based on such structures is proposed and theoretically examined, and some preliminary experimental work towards the synthesis of the required microstructures is also described. Possible approaches to the loading of such traps and the imaging of the atoms contained therein are discussed - experimental work towards ballistic atom transfer from a specialised form of magneto-optical trap that can be formed close to a microstructured surface is carried out, and the efficacy of wavelength-selective fluorescence imaging as a means of reducing the effects of background scatter from the surface is experimentally demonstrated. Further work described herein includes the proposal and experimental demonstration of two novel techniques for the removal of the carrier wave from a phase-modulated laser beam, one of which is based on a fiber-optic Mach-Zehnder interferometer that is shown to be an effective device for splitting or combining beams of nearly equal frequencies. A spontaneous-force based atom trapping mechanism that does not rely on the use of a magnetic field, but rather on spatially-dependent optical pumping between different metastable atomic states, is also proposed, and a proof of principle experiment is carried out to demonstrate the validity of the suggested mechanism. We find that this trapping scheme allows the spatial dependence of the trapping force to be tailored with a greater degree of flexibility than is usually possible with magneto-optical trapping, and that it is also capable of producing traps with stronger spring constants than are typically achievable with magneto-optical trapping under realistic experimental constraints.