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arXiv:1810.00584 · Physical Review Letters

Stabilizing Mechanism for Bose-Einstein Condensation of Interacting Magnons in Ferrimagnets and Ferromagnets

Naoya Arakawa

Published Oct 31, 2018• 14 citations
arXivHTMLPDF

Abstract

We propose a stabilizing mechanism for the Bose-Einstein condensation (BEC) of interacting magnons in ferrimagnets and ferromagnets. By studying the effects of the magnon-magnon interaction on the stability of the magnon BEC in a ferrimagnet and two ferromagnets, we show that the magnon BEC remains stable even in the presence of the magnon-magnon interaction in the ferrimagnet and ferromagnet with a sublattice structure, while it becomes unstable in the ferromagnet without a sublattice structure. This indicates that the existence of a sublattice structure is the key to stabilizing the BEC of interacting magnons, and the difference between the spin alignments of a ferrimagnet and a ferromagnet is irrelevant. Our result can resolve a contradiction between experiment and theory in the magnon BEC of yttrium iron garnet. Our theoretical framework may provide a starting point for understanding the physics of the magnon BEC including the interaction effects.

DOI
10.1103/physrevlett.121.187202

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We propose a mechanism for destabilizing or stabilizing Bose-Einstein condensation (BEC) of interacting magnons in an antiferromagnet. We study how the interaction between magnons affects the magnon BEC in a two-sublattice antiferromagnet without and with an external magnetic field. We show that in the absence of the magnetic field the magnon BEC is destabilized by the attractive interband interaction, which is larger than the repulsive intraband interaction. We also show that in the presence of the magnetic field the magnon BEC is stabilized only if the magnetic field is large enough to make the intraband interaction larger than the interband interaction. Our results provide the first step for understanding the interaction effects on the magnon BEC in antiferromagnets and may open interaction physics of multicomponent BEC of magnons in magnets.

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The Bose-Einstein condensation (BEC) of magnons created by a strong pumping in ferromagnetic thin films of yttrium iron garnet used as systems of finite size is considered analytically. Such a peculiarity, typical for this magnetic material, as the presence of a minimum in the spectrum of spin waves at a finite value of the wave vector is taken into account. The definition of hightemperature BEC is introduced and its characteristics are discussed. A role of boundary conditions for spin variables is analyzed, and it is shown that in the case of free spins on the boundary the magnon lattice can form in the system. The factors responsible for its appearance are discussed.

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We propose a stabilizing mechanism for the Bose-Einstein condensation (BEC) of interacting magnons in ferrimagnets and ferromagnets. By studying the effects of the magnon-magnon interaction on the stability of the magnon BEC in a ferrimagnet and two ferromagnets, we show that the magnon BEC remains stable even in the presence of the magnon-magnon interaction in the ferrimagnet and ferromagnet with a sublattice structure, while it becomes unstable in the ferromagnet without a sublattice structure. This indicates that the existence of a sublattice structure is the key to stabilizing the BEC of interacting magnons, and the difference between the spin alignments of a ferrimagnet and a ferromagnet is irrelevant. Our result can resolve a contradiction between experiment and theory in the magnon BEC of yttrium iron garnet. Our theoretical framework may provide a starting point for understanding the physics of the magnon BEC including the interaction effects.
We propose a mechanism for destabilizing or stabilizing Bose-Einstein condensation (BEC) of interacting magnons in an antiferromagnet. We study how the interaction between magnons affects the magnon BEC in a two-sublattice antiferromagnet without and with an external magnetic field. We show that in the absence of the magnetic field the magnon BEC is destabilized by the attractive interband interaction, which is larger than the repulsive intraband interaction. We also show that in the presence of the magnetic field the magnon BEC is stabilized only if the magnetic field is large enough to make the intraband interaction larger than the interband interaction. Our results provide the first step for understanding the interaction effects on the magnon BEC in antiferromagnets and may open interaction physics of multicomponent BEC of magnons in magnets.
Experimental evidence for Bose–Einstein condensation (BEC) of magnons at room temperature in a thin film of yttrium iron garnet (YIG) excited by parallel pumping is already available and different features of the experimental results have been explained qualitatively [Nature 443, 430 (2006)]. In the present work, we explain quantitatively different aspects of this experimental observation through spin wave treatment. In the case of parallel pumping field, we have developed a formula for the time required for the formation of magnon BEC in a thin film of ferromagnetic material. This relation is found to be in good agreement with known experimental results. In a similar treatment we predict the condition for the formation of BEC of magnons in the case of perpendicular pumping.
A quantised spin wave – magnon – in magnetic films can undergo Bose-Einstein condensation (BEC) into two energetically degenerate lowest-energy quantum states with nonzero wave vectors ±k BEC . This corresponds to two interfering condensates forming spontaneously in momentum space. Brillouin Light Scattering studies for a microwavepumped film with submicrometer spatial resolution experimentally confirm the existence of the two wavefunctions and show that their interference results in a nonuniform ground state of the condensate with the density oscillating in space. Moreover, fork dislocations in the density fringes provide direct experimental evidence for the formation of pinned half-quantum vortices in the magnon condensate. The measured amplitude of the density oscillation implies the formation of a nonsymmetric state that corresponds to nonequal occupation of two energy minima. We discuss the experimental findings and consider the theory of magnon condensates, which includes, to leading order, the contribution from the noncondensed magnons. The effect of the noncondensed magnon cloud is to increase the contrast of the asymmetric state and to bring about the experimental measurements. Introduction Magnons are quasiparticles corresponding to quantised spin waves that describe the collective motion of spins [1]. In recent years, it has become possible to realise a BEC of magnons in two remarkably different systems: in superfluid phases of an isotope of helium – Helium-3 at ultralow temperatures [2, 3] and in ferrimagnetic insulators [4, 5, 6, 7]. In the normal, noncondensed state, these magnetic materials exhibit a magnetically ordered state with a gas of magnons whose phases are not correlated. However, once condensation occurs, spins develop phase coherence resulting in a common global frequency and phase of precession. At room temperature, ferrimagnetic insulators, such as yttrium-iron garnet (YIG) films, together with a combination of an in-plane magnetic field and microwave radiation, are required for the magnon condensation [4, 5, 6, 7]. Therefore, in analogy with exciton– polariton condensates, this provides yet another example of a BEC of quasiparticle excitations in a solid-state system. Experimental Realisation of a Bose-Einstein Condensate of Magnons in an Epitaxial YIG-film A room-temperature Bose-Einstein condensate of magnons was created in an epitaxial YIG-film using an experimental setup shown in Fig. 25.1a, which, in general, is similar to that used in our previous studies [4, 5]. Given that magnons are quasiparticle excitations, their number is not conserved and, therefore, the chemical potential is zero.
The formation of a Bose—Einstein condensate of magnons in a perpendicularly magnetized iron yttrium garnet film under radio-frequency pumping in a stripline has been studied experimentally. The characteristics of the nonlinear magnetic resonance and spatial distribution of the Bose—Einstein condensate of magnons in the gradient of a magnetic field have been analyzed. In these experiments, the system of bosonic magnons behaves in much the same way as the Bose—Einstein condensate of magnons in antiferromagnetic superfluid 3 He-B, which was previously studied in detail. The Bose—Einstein condensate of magnons forms a coherently precessing state having the properties of magnon superfluidity. Its stability is determined by the repulsion potential between excited magnons, which compensates the inhomogeneity of the magnetic field.
The Bose-Einstein condensation (BEC) of magnons created by a strong pumping in ferromagnetic thin films of yttrium iron garnet used as systems of finite size is considered analytically. Such a peculiarity, typical for this magnetic material, as the presence of a minimum in the spectrum of spin waves at a finite value of the wave vector is taken into account. The definition of high-temperature BEC is introduced and its characteristics are discussed. A role of boundary conditions for spin variables is analyzed, and it is shown that in the case of free spins on the boundary the magnon lattice can form in the system. The factors responsible for its appearance are discussed
The Bose-Einstein condensation (BEC) of magnons created by a strong pumping in ferromagnetic thin films of yttrium iron garnet used as systems of finite size is considered analytically. Such a peculiarity, typical for this magnetic material, as the presence of a minimum in the spectrum of spin waves at a finite value of the wave vector is taken into account. The definition of hightemperature BEC is introduced and its characteristics are discussed. A role of boundary conditions for spin variables is analyzed, and it is shown that in the case of free spins on the boundary the magnon lattice can form in the system. The factors responsible for its appearance are discussed.