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Phase Transitions

Bose–Einstein condensation of magnons in ferromagnetic thin films

Rakesh Kar, Anirban Misra, Norman Henry March, Douglas J. Klein

Published May 8, 2012• 0 citations
Publisher

Abstract

Experimental evidence for Bose–Einstein condensation (BEC) of magnons at room temperature in a thin film of yttrium iron garnet (YIG) excited by parallel pumping is already available and different features of the experimental results have been explained qualitatively [Nature 443, 430 (2006)]. In the present work, we explain quantitatively different aspects of this experimental observation through spin wave treatment. In the case of parallel pumping field, we have developed a formula for the time required for the formation of magnon BEC in a thin film of ferromagnetic material. This relation is found to be in good agreement with known experimental results. In a similar treatment we predict the condition for the formation of BEC of magnons in the case of perpendicular pumping.

DOI
10.1080/01411594.2012.682060

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Experimental evidence for Bose–Einstein condensation (BEC) of magnons at room temperature in a thin film of yttrium iron garnet (YIG) excited by parallel pumping is already available and different features of the experimental results have been explained qualitatively [Nature 443, 430 (2006)]. In the present work, we explain quantitatively different aspects of this experimental observation through spin wave treatment. In the case of parallel pumping field, we have developed a formula for the time required for the formation of magnon BEC in a thin film of ferromagnetic material. This relation is found to be in good agreement with known experimental results. In a similar treatment we predict the condition for the formation of BEC of magnons in the case of perpendicular pumping.
The Bose-Einstein condensation (BEC) of magnons created by a strong pumping in ferromagnetic thin films of yttrium iron garnet used as systems of finite size is considered analytically. Such a peculiarity, typical for this magnetic material, as the presence of a minimum in the spectrum of spin waves at a finite value of the wave vector is taken into account. The definition of high-temperature BEC is introduced and its characteristics are discussed. A role of boundary conditions for spin variables is analyzed, and it is shown that in the case of free spins on the boundary the magnon lattice can form in the system. The factors responsible for its appearance are discussed
The conventional magnon Bose-Einstein condensation (BEC of magnons with k = 0) is a coherent state of excited magnons described by a common wave function. It was observed first in antiferromagnetic superfluid states of 3He. Here we report on the discovery of a very similar magnon BEC in ferrimagnetic film at room temperature. The experiments were performed in Yttrium Iron Garnet (YIG) films at a magnetic field oriented perpendicular to the film. The high-density quasiequilibrium state of excited magnon was formed by methods of pulse and/or Continuous Waves (CW) magnetic resonance. We have observed a Long Lived Induction Decay Signals (LLIDS), well known as a signature of spin superfluidity. We demonstrate that the BEC state may maintain permanently by continuous replenishment of magnons with a small radiofrequency (RF) field. Our finding opens the way for development of potential supermagnonic applications at an ambient conditions.
The Bose-Einstein condensation (BEC) of magnons created by a strong pumping in ferromagnetic thin films of yttrium iron garnet used as systems of finite size is considered analytically. Such a peculiarity, typical for this magnetic material, as the presence of a minimum in the spectrum of spin waves at a finite value of the wave vector is taken into account. The definition of hightemperature BEC is introduced and its characteristics are discussed. A role of boundary conditions for spin variables is analyzed, and it is shown that in the case of free spins on the boundary the magnon lattice can form in the system. The factors responsible for its appearance are discussed.
The formation of a Bose—Einstein condensate of magnons in a perpendicularly magnetized iron yttrium garnet film under radio-frequency pumping in a stripline has been studied experimentally. The characteristics of the nonlinear magnetic resonance and spatial distribution of the Bose—Einstein condensate of magnons in the gradient of a magnetic field have been analyzed. In these experiments, the system of bosonic magnons behaves in much the same way as the Bose—Einstein condensate of magnons in antiferromagnetic superfluid 3 He-B, which was previously studied in detail. The Bose—Einstein condensate of magnons forms a coherently precessing state having the properties of magnon superfluidity. Its stability is determined by the repulsion potential between excited magnons, which compensates the inhomogeneity of the magnetic field.
A quantised spin wave – magnon – in magnetic films can undergo Bose-Einstein condensation (BEC) into two energetically degenerate lowest-energy quantum states with nonzero wave vectors ±k BEC . This corresponds to two interfering condensates forming spontaneously in momentum space. Brillouin Light Scattering studies for a microwavepumped film with submicrometer spatial resolution experimentally confirm the existence of the two wavefunctions and show that their interference results in a nonuniform ground state of the condensate with the density oscillating in space. Moreover, fork dislocations in the density fringes provide direct experimental evidence for the formation of pinned half-quantum vortices in the magnon condensate. The measured amplitude of the density oscillation implies the formation of a nonsymmetric state that corresponds to nonequal occupation of two energy minima. We discuss the experimental findings and consider the theory of magnon condensates, which includes, to leading order, the contribution from the noncondensed magnons. The effect of the noncondensed magnon cloud is to increase the contrast of the asymmetric state and to bring about the experimental measurements. Introduction Magnons are quasiparticles corresponding to quantised spin waves that describe the collective motion of spins [1]. In recent years, it has become possible to realise a BEC of magnons in two remarkably different systems: in superfluid phases of an isotope of helium – Helium-3 at ultralow temperatures [2, 3] and in ferrimagnetic insulators [4, 5, 6, 7]. In the normal, noncondensed state, these magnetic materials exhibit a magnetically ordered state with a gas of magnons whose phases are not correlated. However, once condensation occurs, spins develop phase coherence resulting in a common global frequency and phase of precession. At room temperature, ferrimagnetic insulators, such as yttrium-iron garnet (YIG) films, together with a combination of an in-plane magnetic field and microwave radiation, are required for the magnon condensation [4, 5, 6, 7]. Therefore, in analogy with exciton– polariton condensates, this provides yet another example of a BEC of quasiparticle excitations in a solid-state system. Experimental Realisation of a Bose-Einstein Condensate of Magnons in an Epitaxial YIG-film A room-temperature Bose-Einstein condensate of magnons was created in an epitaxial YIG-film using an experimental setup shown in Fig. 25.1a, which, in general, is similar to that used in our previous studies [4, 5]. Given that magnons are quasiparticle excitations, their number is not conserved and, therefore, the chemical potential is zero.
Parameters of the transition from classical dynamics of spin waves to the formation of a coherent magnon Bose–Einstein condensate have been obtained experimentally for the first time. The studies are performed on an yttrium iron garnet film beyond the radio frequency excitation region; thus, the coherent state of magnons is an eigenstate rather than a state induced by an external radio frequency field. The critical magnon density at the formation of the Bose–Einstein condensate is in good agreement with a theoretically predicted value. The transition is obtained at room temperature, which is possible owing to a small mass of magnons and their high density.