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arXiv:1807.07586 · Physical Review Research

Photon propagation through dissipative Rydberg media at large input rates

Przemyslaw Bienias, James Douglas, Asaf Paris-Mandoki, Paraj Titum, Ivan Mirgorodskiy, Christoph Tresp, Emil Zeuthen, Michael J. Gullans, Marco Manzoni, Sebastian Hofferberth, Darrick Chang, Alexey V. Gorshkov

Published Jul 10, 2020• 33 citations

Abstract

We study the dissipative propagation of quantized light in interacting Rydberg media under the conditions of electromagnetically induced transparency. Rydberg blockade physics in optically dense atomic media leads to strong dissipative interactions between single photons. The regime of high incoming photon flux constitutes a challenging many-body dissipative problem. We experimentally study in detail the pulse shapes and the second-order correlation function of the outgoing field and compare our data with simulations based on two novel theoretical approaches well-suited to treat this many-photon limit. At low incoming flux, we report good agreement between both theories and the experiment. For higher input flux, the intensity of the outgoing light is lower than that obtained from theoretical predictions. We explain this discrepancy using a simple phenomenological model taking into account pollutants, which are nearly stationary Rydberg excitations coming from the reabsorption of scattered probe photons. At high incoming photon rates, the blockade physics results in unconventional shapes of measured correlation functions.

DOI: 10.1103/physrevresearch.2.033049

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Rydberg blockade physics in optically dense atomic media under the conditions of electromagnetically induced transparency (EIT) leads to strong dissipative interactions between single photons. We introduce a new approach to analyzing this challenging many-body problem in the limit of a large optical depth per blockade radius. In our approach, we separate the single-polariton EIT physics from Rydberg-Rydberg interactions in a serialized manner while using a hard-sphere model for the latter, thus capturing the dualistic particle-wave nature of light as it manifests itself in dissipative Rydberg-EIT media. Using this approach, we analyze the saturation behavior of the transmission through one-dimensional Rydberg-EIT media in the regime of nonperturbative dissipative interactions relevant to current experiments. Our model is able to capture the many-body dynamics of bright, coherent pulses through these strongly interacting media. We compare our model with available experimental data in this regime and find good agreement. We also analyze a scheme for generating regular trains of single photons from continuous-wave input and derive its scaling behavior in the presence of imperfect single-photon EIT.

We develop a theoretical framework for the dissipative propagation of quantized light under conditions of electromagnetically induced transparency in atomic media involving strongly interacting Rydberg states. The theory allows us to determine the peculiar spatiotemporal structure of the output of the recently demonstrated single-photon filter and the recently proposed single-photon subtractor, which, respectively, let through and absorb a single photon. In addition to being crucial for applications of these and other optical quantum devices, the theory opens the door to the study of exotic dissipative many-body dynamics of strongly interacting photons in nonlinear nonlocal media.

We discuss electromagnetically induced transparency in a cold ensemble of atoms optically excited to the Rydberg states. Strong dipole-dipole or van der Waals interactions between the atomic Rydberg states translate into large nonlocal nonlinearities for a propagating probe field. In the case of weak quantum fields, this can be used to attain a conditional phase shift of π between pairs of single photons realizing a deterministic photonic phase gate. For stronger fields, long-range interactions between the atoms constrain the medium to behave as a collection of superatoms, each comprising a blockade volume that can accommodate at most one Rydberg excitation. The propagation of a probe field is affected by its two-photon correlations within the blockade distance, which are strongly damped due to low saturation threshold of the superatoms. Our calculations reproduce and interpret the results of recent experiments.

Light propagation through an ensemble of ultracold Rydberg atoms in an electromagnetically-induced-transparency (EIT) configuration is studied. In strongly interacting Rydberg EIT media, nonlinear optical effects lead to a nontrivial dependence of the degree of probe-beam attenuation on the medium density and on its initial intensity. We develop a Monte Carlo rate equation model that self-consistently includes the effect of the probe-beam attenuation to investigate the steady state of the Rydberg medium driven by two laser fields. We compare our results to recent experimental data and to results of other state-of-the-art models for light propagation in Rydberg EIT media. We find that for low probe field intensities, our results match the experimental data best if a density-dependent dephasing rate is included in the model. At higher probe intensities, our model deviates from other theoretical approaches, because it predicts a spectral asymmetry together with line broadening. These are likely due to off-resonant excitation channels, which, however, have not been observed in recent experiments. Atomic motion and coupling to additional Rydberg levels are discussed as possible origins for these deviations.

We develop the theory of light propagation under the conditions of electromagnetically induced transparency in systems involving strongly interacting Rydberg states. Taking into account the quantum nature and the spatial propagation of light, we analyze interactions involving few-photon pulses. We show that this system can be used for the generation of nonclassical states of light including trains of single photons with an avoided volume between them, for implementing photon-photon gates, as well as for studying many-body phenomena with strongly correlated photons.

We present a theory of electromagnetically induced transparency in a cold ensemble of strongly interacting Rydberg atoms. Long-range interactions between the atoms constrain the medium to behave as a collection of superatoms, each comprising a blockade volume that can accommodate at most one Rydberg excitation. The propagation of a probe field is affected by its two-photon correlations within the blockade distance, which are strongly damped due to low saturation threshold of the superatoms. Our model is computationally very efficient and is in quantitative agreement with the results of the recent experiment of Pritchard et al. [Phys. Rev. Lett. 105, 193603 (2010)].