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arXiv:1211.7060 · Physical Review Letters

Dissipative Many-Body Quantum Optics in Rydberg Media

Alexey Vyacheslavovich Gorshkov, Rejish Nath, Thomas Pohl

Published Apr 9, 2013• 104 citations
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Abstract

We develop a theoretical framework for the dissipative propagation of quantized light under conditions of electromagnetically induced transparency in atomic media involving strongly interacting Rydberg states. The theory allows us to determine the peculiar spatiotemporal structure of the output of the recently demonstrated single-photon filter and the recently proposed single-photon subtractor, which, respectively, let through and absorb a single photon. In addition to being crucial for applications of these and other optical quantum devices, the theory opens the door to the study of exotic dissipative many-body dynamics of strongly interacting photons in nonlinear nonlocal media.

DOI
10.1103/physrevlett.110.153601

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We develop a theoretical framework for the dissipative propagation of quantized light under conditions of electromagnetically induced transparency in atomic media involving strongly interacting Rydberg states. The theory allows us to determine the peculiar spatiotemporal structure of the output of the recently demonstrated single-photon filter and the recently proposed single-photon subtractor, which, respectively, let through and absorb a single photon. In addition to being crucial for applications of these and other optical quantum devices, the theory opens the door to the study of exotic dissipative many-body dynamics of strongly interacting photons in nonlinear nonlocal media.
We study the dissipative propagation of quantized light in interacting Rydberg media under the conditions of electromagnetically induced transparency. Rydberg blockade physics in optically dense atomic media leads to strong dissipative interactions between single photons. The regime of high incoming photon flux constitutes a challenging many-body dissipative problem. We experimentally study in detail the pulse shapes and the second-order correlation function of the outgoing field and compare our data with simulations based on two novel theoretical approaches well-suited to treat this many-photon limit. At low incoming flux, we report good agreement between both theories and the experiment. For higher input flux, the intensity of the outgoing light is lower than that obtained from theoretical predictions. We explain this discrepancy using a simple phenomenological model taking into account pollutants, which are nearly stationary Rydberg excitations coming from the reabsorption of scattered probe photons. At high incoming photon rates, the blockade physics results in unconventional shapes of measured correlation functions.
Rydberg blockade physics in optically dense atomic media under the conditions of electromagnetically induced transparency (EIT) leads to strong dissipative interactions between single photons. We introduce a new approach to analyzing this challenging many-body problem in the limit of a large optical depth per blockade radius. In our approach, we separate the single-polariton EIT physics from Rydberg-Rydberg interactions in a serialized manner while using a hard-sphere model for the latter, thus capturing the dualistic particle-wave nature of light as it manifests itself in dissipative Rydberg-EIT media. Using this approach, we analyze the saturation behavior of the transmission through one-dimensional Rydberg-EIT media in the regime of nonperturbative dissipative interactions relevant to current experiments. Our model is able to capture the many-body dynamics of bright, coherent pulses through these strongly interacting media. We compare our model with available experimental data in this regime and find good agreement. We also analyze a scheme for generating regular trains of single photons from continuous-wave input and derive its scaling behavior in the presence of imperfect single-photon EIT.
We develop the theory of light propagation under the conditions of electromagnetically induced transparency in systems involving strongly interacting Rydberg states. Taking into account the quantum nature and the spatial propagation of light, we analyze interactions involving few-photon pulses. We show that this system can be used for the generation of nonclassical states of light including trains of single photons with an avoided volume between them, for implementing photon-photon gates, as well as for studying many-body phenomena with strongly correlated photons.
Coupling light to ensembles of strongly interacting particles has emerged as a promising route toward achieving few photon nonlinearities. One specific way to implement this kind of nonlinearity is to interface light with highly excited atomic Rydberg states by means of electromagnetically induced transparency, an approach which allows freely propagating photons to acquire synthetic interactions of hitherto unprecedented strength. Here, we present an overview of this rapidly developing field, from classical effects to quantum manifestations of the nonlocal nonlinearities emerging in such systems. With an emphasis on underlying theoretical concepts, we describe the many experimental breakthroughs so far demonstrated and discuss potential applications looming on the horizon.
We discuss electromagnetically induced transparency in a cold ensemble of atoms optically excited to the Rydberg states. Strong dipole-dipole or van der Waals interactions between the atomic Rydberg states translate into large nonlocal nonlinearities for a propagating probe field. In the case of weak quantum fields, this can be used to attain a conditional phase shift of π between pairs of single photons realizing a deterministic photonic phase gate. For stronger fields, long-range interactions between the atoms constrain the medium to behave as a collection of superatoms, each comprising a blockade volume that can accommodate at most one Rydberg excitation. The propagation of a probe field is affected by its two-photon correlations within the blockade distance, which are strongly damped due to low saturation threshold of the superatoms. Our calculations reproduce and interpret the results of recent experiments.
Abstract Rydberg atoms, characterized by their giant polarizability and strong long-range interactions, provide an ideal platform for exploring optical nonlinearities. By coupling light to ensembles of Rydberg atoms, one can map the strong and nonlocal interactions between Rydberg atoms and light fields. A particularly important scheme for realizing such nonlinearity is electromagnetically induced transparency (EIT). This article presents a review of the research progress in nonlinear optics based on Rydberg-EIT systems, particularly nonlinear light propagation in Rydberg atomic gases. We first introduce the fundamental properties of Rydberg atoms and the physical mechanism of EIT-enhanced nonlinearity, emphasizing how the Rydberg blockade effect endows the system with a giant nonlocal Kerr nonlinearity. Subsequently, we discuss some typical nonlinear optical phenomena in such a system with focusing and defocusing nonlocal nonlinearities. In the focusing regime, we discuss spatial solitons, vortex solitons, soliton cloning, soliton molecules, optical bullets, and self-induced transparency solitons. Other topics are also discussed. In the defocusing regime, we analyze pattern formation and shock wave dynamics. Finally, we provide an outlook on the future development of this field toward quantum control, hybrid-system integration, and novel functional devices.