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arXiv:1807.03414 · Physical review. B./Physical review. B

Gauge-invariant microscopic kinetic theory of superconductivity in response to electromagnetic fields

Fan Yang, M. W. Wu

Published Sep 10, 2018• 26 citations
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Abstract

Within a gauge-invariant microscopic kinetic theory, we study the electromagnetic response in the superconducting states. Both superfluid and normal-fluid dynamics are involved. We predict that the normal fluid is present only when the excited superconducting velocity ${v}_{s}$ is larger than a threshold ${v}_{L}=|\mathrm{\ensuremath{\Delta}}|/{k}_{F}$. Interestingly, with the normal fluid, we find that there exists friction between the normal-fluid and superfluid currents. Due to this friction, part of the superfluid becomes viscous. Therefore a three-fluid model, normal fluid and nonviscous and viscous superfluids, is proposed. For the stationary magnetic response, at ${v}_{s}<{v}_{L}$ with only the nonviscous superfluid, the Meissner supercurrent is excited and the gap equation can be reduced to the Ginzburg-Landau equation. At ${v}_{s}\ensuremath{\ge}{v}_{L}$, with the normal fluid and nonviscous and viscous superfluids, in addition to the directly excited Meissner supercurrent in the superfluid, a normal-fluid current is also induced through the friction drag with the viscous superfluid current. Due to the normal-fluid and viscous-superfluid currents, the penetration depth is influenced by the scattering effect. In addition, a modified Ginzburg-Landau equation is proposed. We predict an exotic phase in which both the resistivity and superconducting gap are finite. As for the optical response, the excited ${v}_{s}$ oscillates with time. When ${v}_{s}<{v}_{L}$, only the nonviscous superfluid is present, whereas at ${v}_{s}\ensuremath{\ge}{v}_{L}$, normal fluid and nonviscous and viscous superfluids are present. We show that the excited normal-fluid current exhibits the Drude-model behavior, while the superfluid current consists of the Meissner supercurrent and Bogoliubov quasiparticle current. Due to the friction between the superfluid and normal-fluid currents, the optical conductivity is captured by the three-fluid model. Finally, we also study the optical excitation of the Higgs mode. By comparing the contributions from the drive and Anderson-pseudospin pump effects, we find that the drive effect is dominant at finite temperature whereas at zero temperature, both effects contribute.

DOI
10.1103/physrevb.98.094507

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Within a gauge-invariant microscopic kinetic theory, we study the electromagnetic response in the superconducting states. Both superfluid and normal-fluid dynamics are involved. We predict that the normal fluid is present only when the excited superconducting velocity vs{v}_{s}vs​ is larger than a threshold vL=∣\ensuremathΔ∣/kF{v}_{L}=|\mathrm{\ensuremath{\Delta}}|/{k}_{F}vL​=∣\ensuremathΔ∣/kF​. Interestingly, with the normal fluid, we find that there exists friction between the normal-fluid and superfluid currents. Due to this friction, part of the superfluid becomes viscous. Therefore a three-fluid model, normal fluid and nonviscous and viscous superfluids, is proposed. For the stationary magnetic response, at vs<vL{v}_{s}<{v}_{L}vs​<vL​ with only the nonviscous superfluid, the Meissner supercurrent is excited and the gap equation can be reduced to the Ginzburg-Landau equation. At vs\ensuremath≥vL{v}_{s}\ensuremath{\ge}{v}_{L}vs​\ensuremath≥vL​, with the normal fluid and nonviscous and viscous superfluids, in addition to the directly excited Meissner supercurrent in the superfluid, a normal-fluid current is also induced through the friction drag with the viscous superfluid current. Due to the normal-fluid and viscous-superfluid currents, the penetration depth is influenced by the scattering effect. In addition, a modified Ginzburg-Landau equation is proposed. We predict an exotic phase in which both the resistivity and superconducting gap are finite. As for the optical response, the excited vs{v}_{s}vs​ oscillates with time. When vs<vL{v}_{s}<{v}_{L}vs​<vL​, only the nonviscous superfluid is present, whereas at vs\ensuremath≥vL{v}_{s}\ensuremath{\ge}{v}_{L}vs​\ensuremath≥vL​, normal fluid and nonviscous and viscous superfluids are present. We show that the excited normal-fluid current exhibits the Drude-model behavior, while the superfluid current consists of the Meissner supercurrent and Bogoliubov quasiparticle current. Due to the friction between the superfluid and normal-fluid currents, the optical conductivity is captured by the three-fluid model. Finally, we also study the optical excitation of the Higgs mode. By comparing the contributions from the drive and Anderson-pseudospin pump effects, we find that the drive effect is dominant at finite temperature whereas at zero temperature, both effects contribute.
We show that the gauge-invariant kinetic equation of superconductivity provides an efficient approach to study the electromagnetic response of the gapless Nambu-Goldstone and gapful Higgs modes on an equal footing. We prove that the Fock energy in the kinetic equation is equivalent to the generalized Ward's identity. Hence, the gauge invariance directly leads to the charge conservation. Both linear and second-order optical responses are analytically investigated. The linear response of the Higgs mode vanishes in the long-wave limit, whereas the linear response of the Nambu-Goldstone mode interacts with the long-range Coulomb interaction, causing the original gapless energy spectrum effectively lifted up to the plasma frequency as a result of the Anderson-Higgs mechanism, consistent with previous work. The second-order response exhibits interesting physics. On the one hand, a finite second-order optical response of the Higgs mode is obtained in the long-wave limit. We reveal that this response, which has been experimentally observed, is attributed solely to the drive effect rather than the widely considered Anderson-pump effect. On the other hand, the second-order optical response of the Nambu-Goldstone mode, free from the influence of the long-range Coulomb interaction and hence the Anderson-Higgs mechanism, is predicted. We find that both Anderson-pump and drive effects play important role in this response. A tentative scheme to detect this second-order response is proposed.
This thesis reports on theoretical investigations of the ultrafast nonequilibrium dynamics in superconductors. In particular, two nonequilibrium scenarios are modeled by combining several analytical and numerical methods: transient superconducting phase transition and collective excitations of a superconducting condensate. In the first part of the thesis the possibility to induce singlet superconducting correlations far from equilibrium is explored by applying time-dependent Lanczos algorithm to the one-dimensional extended Hubbard model. Here, the system is driven into a nonequilibrium state by (i) interaction quench and (ii) quench by pulse. In both cases the buildup of the superconducting correlations is studied in view of several correlation functions. Moreover, a transient Meissner effect, which reflects fingerprints of the induced superconductivity, is observed in calculations of the important for experiments time-dependent optical conductivity. In addition, the differences between nonequilibrium dynamics of the extended Hubbard model initiated by interaction quench and by pulse quench are discussed in detail. The second part is devoted to the excitation of collective modes in a superconductor out of equilibrium. First of all, focus is given to the properties of collective modes close to equilibrium conditions, where a linearized response can be expected. Within the framework of the (Nambu-) matrix kinetic theory in the clean limit a comprehensive gauge-invariant description of the collective modes associated with phase fluctuations of the order parameter is analytically formulated for the generalized case of two- band superconducting systems. Particular emphasis is on the application to the recently discovered noncentrosymmetric superconductors. A detailed analysis of the collective modes includes specification of the gauge mode (common to all superconductors) and the Leggett mode (collective fluctuations of the interband phase difference), and investigation of their subtle interplay in view of validity of the charge conservation law and the participation in the Anderson-Higgs mechanism. Further, the nonequilibrium excitation of the superconducting gaps for the case of two-band superconductors with singlet pairing correlations is investigated in a view of optical pump-probe experiments. For this purpose a semi-numerical method based on the density- matrix theory is formulated. In this case additional amplitude (Higgs) modes were identified, which allow to directly detect the properties of the superconducting condensates as a function of time. Moreover, a new interplay between the phase (Leggett) and amplitude (Higgs) modes is studied in detail. In particular it was found that the nonadiabatic excitation process leads to strong coupling between both modes. Finally, based on calculations of the time-dependent optical conductivity the prediction is made that the coupled Higgs and Leggett modes can be clearly visible in the pump-probe absorption spectra.
Collective-mode fluctuations play an essential role in ensuring the electromagnetic response of superfluids is gauge invariant. The contribution of these fluctuations, however, is known to drop out from the Meissner response of uniform superfluids. The same phenomenon is not so established in the context of nonuniform superfluids. To clarify this issue, we revisit how collective modes appear in the Meissner effect. We find that their contribution vanishes both in uniform and nonuniform systems, unless an external length scale is present---as in Fulde-Ferrell or finite-sized superfluids. As examples, we consider sss-wave and chiral p+ipp+ipp+ip superconductors. To facilitate this analysis, we formulate a path-integral matrix methodology for computing the response of fermionic fluids in the presence of multiple collective modes. Closed-form expressions are provided, incorporating effects from phase and amplitude of the superconducting order parameter and electronic density fluctuations. All microscopic symmetries and invariances are manifestly satisfied in this approach, and it can be straightforwardly extended to other scenarios.
In this thesis we demonstrate the power of the Gross-Pitaevskii and the time-dependent Ginzburg-Landau equations by numerically solving them for various fundamental problems related to superfluidity and superconductivity. We start by studying the motion of a massive object through a quantum fluid modelled by the Gross-Pitaevskii equation. Below a critical velocity, the object does not exchange momentum or energy with the fluid. This is a manifestation of its superfluid nature. We discuss the effect of applying a constant force to the object and show that for small forces a vortex ring is created to which the object becomes attached. For a larger force the object detaches from the vortex ring and we observe periodic shedding of rings. All energy transfered to the system is contained within the vortex rings and the drag force on the object is due to the recoil of the vortex emission. If we exceed the speed of sound, there is an additional contribution to the drag from sound emission. To make a link to superconductivity, we then discuss vortex states in a rotating system. In the ground state, regular arrays of vortices are observed which, for systems containing many vortices, mimic solid-body rotation. In the second part of the thesis, we initially review solutions to the Ginzburg-Landau equations in an applied magnetic field. For superconducting disks we observe vortex arrays similar to those in rotating superfluids. Finally, we study an electrical current flow along a superconducting wire subject to an external magnetic field. We observe the motion of flux lines, and hence dissipation, due to the Lorentz force. We measure the V - I curve which is analogous to the drag force in a superfluid. With the introduction of impurities, flux lines become pinned which gives rise to an increased critical current. (author)
The Meissner effect is a hallmark of superconductivity arising from the interplay between charged superfluids and electromagnetic fields. However, superfluidity can also occur in systems of charge-neutral particles with magnetic or electric dipole moments, such as Bose-Einstein condensates of magnons or excitons. Despite this interest, the electromagnetic response of dipole superfluids, including potential analogues or contrasts to the Meissner effect, remains poorly understood. Here we develop a Ginzburg-Landau theory to describe dipole superfluids subjected to a pseudo-magnetic field, which is induced by a spatially modulating electromagnetic field. In magnetic dipole superfluids, the response differs strikingly from the conventional Meissner effect: the external field is enhanced by a positive feedback, forming a vortex lattice separated by singular domain walls with diverging electric charges. In contrast, electric dipole superfluids exhibit screening akin to superconductors, where the pseudo-magnetic field is suppressed except near vortices. The electromagnetic response of dipole superfluids, including potential analogues to the Meissner effect, remains poorly understood. This paper develops a phenomenological theory and shows that magnetic-dipole superfluids form vortex lattices separated by singular domain walls with concentrated electric charge, while electric-dipole superfluids exhibit vortex lattices resembling those in conventional superconductors.
An alternative approach to the derivation of the force on a vortex based in an adiabatic approximation in the action of the superfluid system is developed. Assuming that the vortex motion is relatively slow compared with the characteristic times involved in the microscopic degrees of freedom, the effect of the superfluid and its excitations is reduced to a gauge potential, and the associated transverse force. The vortex velocity part of the transverse force is found in terms of the thermal expectation of the angular momentum of the fluid around the vortex. The excitations countercirculate the vortex reducing the effective density to that of the superfluid part only. Non-adiabatic contributions appear in this formalism as a non-Abelian gauge potential connecting different microscopic states, in particular the renormalization of the vortex mass is given by the lowest order diagonal correction to the adiabatic theory, and the long wavelength contributions found to depend only on the static structure factor for the fluid.