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arXiv:1805.08190 · Communications Physics

Spiral bandwidth of four-wave mixing in Rb vapour

Rachel F. Offer, Dalius Stulga, Erling Riis, Sonja Franke‐Arnold, Aidan S. Arnold

Published Nov 15, 2018• 57 citations
arXivHTMLPDF

Abstract

Abstract Laguerre-Gauss beams, and more generally the orbital angular momentum of light (OAM) provide valuable research tools for optical manipulation, processing, imaging and communication. High-efficiency frequency conversion of OAM is possible via four-wave mixing in rubidium vapour. Conservation of the OAM in the two pump beams determines the total OAM shared by the generated light fields at 420 nm and 5.2 μm—but not its distribution between them. Here we experimentally investigate the spiral bandwidth of the generated light modes as a function of pump OAM. A small pump OAM is transferred almost completely to the 420 nm beam. Increasing the total pump OAM broadens the OAM spectrum of the generated light, indicating OAM entanglement between the generated light fields. This clears the path to high-efficiency OAM entanglement between widely disparate wavelengths.

DOI
10.1038/s42005-018-0077-5

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Abstract Laguerre-Gauss beams, and more generally the orbital angular momentum of light (OAM) provide valuable research tools for optical manipulation, processing, imaging and communication. High-efficiency frequency conversion of OAM is possible via four-wave mixing in rubidium vapour. Conservation of the OAM in the two pump beams determines the total OAM shared by the generated light fields at 420 nm and 5.2 μm—but not its distribution between them. Here we experimentally investigate the spiral bandwidth of the generated light modes as a function of pump OAM. A small pump OAM is transferred almost completely to the 420 nm beam. Increasing the total pump OAM broadens the OAM spectrum of the generated light, indicating OAM entanglement between the generated light fields. This clears the path to high-efficiency OAM entanglement between widely disparate wavelengths.
Atomic vapours are an experimentally simple and efficient system in which to study nonlinear wave mixing. We study a four-wave mixing (FWM) process in rubidium vapour which efficiently converts 780 and 776 nm light to 420 nm and 5.2 μm fields. In particular, we quantitatively investigate the transfer of orbital angular momentum (OAM) between the FWM fields. OAM, and structured light more generally, is an important research tool for optical manipulation, imaging and communication. Phase-matched nonlinear processes are both longitudinally and transversely phase coherent, and therefore OAM, which is associated with spiral phase fronts, must be conserved between the pump and generated fields. This makes wave mixing an ideal tool for frequency conversion and generation of a variety of OAM states for use in both classical and quantum communication.
Abstract The manipulation of the orbital angular momentum (OAM) contributes to understand the OAM multiplexing, is significant in free-space optical communication and information processing. We theoretically simulate and experimentally demonstrate the regularity of the OAM transfer, including the angular and radial modes, of Laguerre–Gaussian beam via four-wave mixing process in 85Rb vapor. The 420 nm coherent blue light output field inherits the phase characteristic of 780 nm and 776 nm beams with different OAM modes. The output field OAM modes show the transfer as a typical arithmetic operation of the input field OAM modes with equal-handed angular indice l, while, the conversion between angular and radial modes occurs with the opposite angular indice l. Such rules of the OAM transfer and manipulation have implications on the research of high-capacity information transfer and quantum communication.
We explore the conservation of orbital angular momentum (OAM) in the four-wave mixing (FWM) process in hot rubidium vapor. Since most modern communication systems send data in pulses corresponding to bits, we can use OAM to encode more information in each pulse by assigning structure to each signal. Furthermore, because FWM can be used to generate entangled photon pairs, we can use this process to bring enhanced signal security. We experimentally studied FWM with a wide range of Laguerre-Gaussian modes and their superpositions and observed OAM transfer from the probe field to a generated Stokes field. By studying the output Stokes intensity and phase distributions, we confirm l mode (OAM) conservation for pure l and p modes, as well as for the superpositions of l and -l for the mode numbers up to l = 4, p = 4. We also found that p index is generally not conserved and its conservation is highly dependent on the relative sizes of the probe and pump beams in the Rb cell. We also identify parameters to improve FWM gain with OAM transfer and propose an analytical method for determining OAM p number.
Abstract Up-conversion in an atomic vapor is known to produce photon pairs. If addressed by vortex beams, it produces pairs of orbital angular momenta (OAM), that are valuable bricks for quantum processes with OAM. The perfect vortex (PV) beam is a vortex class very pertinent in this context, because its ring radius and its Gouy phase are —in principle— independent of the OAM, giving a huge spiral bandwidth compared to the usual Laguerre-Gaussian (LG) beam. Our experimental study clarifies this point. The PV ring radius and thickness are found to vary hyperbolic-like vs . the OAM, which will limit the spiral bandwidth, but, unlike LG, the number of generated OAM pairs still remains quite comfortable for entanglement applications.
Airy vortex beams, which integrate orbital angular momentum with diffraction-resistant and self-accelerating characteristics of Airy beams, offer unique capabilities for high-capacity optical communication and high-resolution imaging. Here, we experimentally demonstrate the generation and manipulation of frequency-converted Airy vortex beams through four-wave mixing in hot Rb vapor. A 780 nm vortex beam and a 776 nm two-dimensional Airy beam coherently participate in the four-wave mixing process, generating a 420 nm output beam that combines the orbital angular momentum of the vortex beam with the spatial structure of the Airy beam. The generated beam exhibits pronounced quasi-nondiffracting propagation and self-acceleration, with an intensity decay rate reduced by a factor of ∼1.88 relative to the input vortex beam and a transverse acceleration ∼1.84 times that of the input Airy beam. Moreover, both the intensity and the spatial profile of the generated beam are flexibly manipulated by varying the Rb vapor temperature and the pump beam power. This work provides a versatile approach for generating and controlling structured light at what we believe are new wavelengths, opening opportunities for short-wavelength optical manipulation and optical information processing.
Abstract This study presents a theoretical exploration of generating 420 nm Bessel-Gaussian beam with orbital angular momentum (OAM) via nonlinear processes in a four-level 85 Rb atomic system. A non-degenerate four-wave mixing (FWM) configuration, driven by two strong control fields at wavelengths 780 nm and 776 nm along with a weak field, enables the generation of the desired blue Bessel-Gaussian beam. Our analysis examines how the Bessel-Gaussian properties of the initial beams including intensity, phase profiles, and topological charges are transferred into the generated 420 nm beam at specific transverse positions. Using Maxwell’s wave equations, we explicitly explore how these spatial profiles evolve with varying topological charges over different propagation distances, providing deeper insights into Bessel-Gaussian information transfer mechanisms. The generation and characterization of 420 nm structured beam highlight promising applications, particularly in the precise manipulation of microparticles, due to their enhanced resolution and superior trapping abilities. This comprehensive theoretical framework establishes a foundation for future experimental and applied research in optical manipulation and high-resolution imaging.