The interaction of spatially structured light fields with atomic media can generate spatial structures inscribed in the atomic populations and coherences, allowing for example the storage of optical images in atomic vapours. Typically, this involves coherent optical processes based on Raman or EIT transitions. Here we study the simpler situation of shaping atomic populations via spatially dependent optical depletion. Using a near resonant laser beam with a holographically controlled 3D intensity profile, we imprint 3D population structures into a thermal rubidium vapour. This 3D population structure is simultaneously read out by recording the spatially resolved fluorescence of an unshaped probe laser. We find that the reconstructed atomic population structure is largely complementary to the intensity structure of the control beam, however appears blurred due to global repopulation processes. We identify and model these mechanisms which limit the achievable resolution of the 3D atomic population. We expect this work to set design criteria for future 2D and 3D atomic memories.
The interaction of spatially structured light fields with atomic media can generate spatial structures inscribed in the atomic populations and coherences, allowing for example the storage of optical images in atomic vapours. Typically, this involves coherent optical processes based on Raman or EIT transitions. Here we study the simpler situation of shaping atomic populations via spatially dependent optical depletion. Using a near resonant laser beam with a holographically controlled 3D intensity profile, we imprint 3D population structures into a thermal rubidium vapour. This 3D population structure is simultaneously read out by recording the spatially resolved fluorescence of an unshaped probe laser. We find that the reconstructed atomic population structure is largely complementary to the intensity structure of the control beam, however appears blurred due to global repopulation processes. We identify and model these mechanisms which limit the achievable resolution of the 3D atomic population. We expect this work to set design criteria for future 2D and 3D atomic memories.
In recent years great progress was made in the spatial control of light with dynamic phase and amplitude modulators such as spatial light modulators and digital micromirror devices. In this work we describe the theory and practice of light shaping with such devices, detailing the spatial control of amplitude, phase and polarisation of coherent laser beams. We use our expertise in generating and measuring light fields with spatially dependent polarisation structures to characterise the correlations between spatial modes and polarisation in such light fields. We do this by adapting concurrence, a quantum measure of entanglement, to these classical correlations. One of the most promising application of coherent laser light is in the control of atomic media via atom-light interactions. In this work we describe the construction of simple external cavity diode lasers designed for the generation of resonant light for atomic physics applications. We exploit these lasers and spatial light modulators to create and measure three-dimensional atomic population structures in a warm rubidium vapour. We also implement a magneto-optic and a dynamic dark spontaneous-force optical trap for rubidium. These traps produce dense (~ 10^11 cm^-3) and cold (~100 uK) clouds of rubidium atoms. We develop the theory of spatially dependent electromagnetically induced transparency in such traps using rate equations. We find that the absorption of linearly polarised light depends on the relative direction of a magnetic field and the light polarisation. We use the cold atom clouds to measure the direction of magnetic fields by using this dependence and laser beams with structured polarisation.
We present a technique for mapping the complete 3D spatial intensity profile of a laser beam from its fluorescence in an atomic vapour. We propagate shaped light through a rubidium vapour cell and record the resonant scattering from the side. From a single measurement we obtain a camera limited resolution of 200 × 200 transverse points and 659 longitudinal points. In constrast to invasive methods in which the camera is placed in the beam path, our method is capable of measuring patterns formed by counterpropagating laser beams. It has high resolution in all 3 dimensions, is fast and can be completely automated. The technique has applications in areas which require complex beam shapes, such as optical tweezers, atom trapping and pattern formation.
The development of new laser beam shaping methods is important in a variety of fields within optics, atomic physics and biophotonics. Spatial light modulators offer a highly versatile method of time-dependent beam shaping, based on imprinting a phase profile onto an incident laser beam that determines the intensity in the trapping plane laser field. The calculation of the required phase is a well-known inverse problem, which can be tackled with different approaches. Our method based on conjugate gradient minimisation [1] not only allows the calculation of smooth and accurate intensity profiles suitable for trapping cold atoms, but can also be used to generate multi-wavelength traps [2] and for simultaneous control over both the intensity and the phase of the light [3], with exceptionally high reconstruction fidelity. References: [1] T Harte, et al., "Conjugate gradient minimisation approach to generating holographic traps for ultracold atoms" Opt. Express 22, 26548 (2014) [2] D Bowman, et al., "Multi-wavelength holography with a single spatial light modulator for ultracold atom experiments" Opt. Express 23, 8365 (2015) [3] D Bowman, et al., "High-fidelity phase and amplitude control of phase-only computer generated holograms using conjugate gradient minimisation" Opt. Express 25, 11692 (2017)
Effective and unrestricted engineering of atom-photon interactions requires precise spatially resolved control of light beams. The significant potential of such manipulations lies in a set of disciplines ranging from solid-state to atomic physics. Here we use a Zeeman-like ac-Stark shift caused by a shaped laser beam to perform rotations of spins with spatial resolution in a large ensemble of cold rubidium atoms. We show that inhomogeneities of light intensity are the main source of dephasing and, thus, decoherence; yet, with proper beam shaping, this deleterious effect is strongly mitigated allowing rotations of 15 rad within one spin-precession lifetime. Finally, as a particular example of a complex manipulation enabled by our scheme, we demonstrate a range of collapse-and-revival behaviors of a free-induction decay signal by imprinting comb-like patterns on the atomic ensemble.
Laser light can exhibit nonlinear behaviour when interacting with dense atomic vapours.\nThis can give rise to a variety of interesting phenomena such as slow light and optically induced transparency. Recently A.~J. van Lange measured nonlinear transmission of light through a Rubidium vapour and developed a physical model to describe these measurements. Van Lange also investigated the formation of different beam profiles, in a dense Rubidium vapour and from Gaussian input beams, as a function of intensity and optical frequency.\n\nHere we expand on van Lange's measurements by measuring over a large frequency range which includes multiple atomic transition lines and by employing off-axis holography which allows for simultaneous measurement of the intensity and phase. Analysis of beam profiles based on the structural similarity index (SSIM) uncovered beam profiles whose path through intensity-detuning space could be described with van Lange's generalised detuning curve. Off-axis holography measurements are in agreement with regular intensity measurements but exhibits a greater amount of noise.
The resonant absorption, emission, and scattering of light are the fundamental optical processes that have been used both to probe matter and to manipulate light itself. In the last decade there has been essential progress in coherent control of both linear and nonlinear optical responses based on resonant excitation of atomic coherence in multilevel quantum systems. Some interesting and useful phenomena, resulting from coherent control of absorption and the group index, such as electromagnetically induced transparency, lasing without inversion, and ultra-slow group velocity of light have been widely studied. This work is focused on coherent control of refractive index and resonant fluorescence in multilevel medium. \n \nWe suggest two promising schemes for resonant enhancement of the refractive index with eliminated absorption and propose their implementation in transition element doped crystals with excited state absorption and in a cell of Rb atoms at natural abundance. We show how to use one of these schemes for spatial variation of the refractive index via its periodic resonant increase/decrease, remarkably keeping at the same time zero absorption/gain. It opens the way to production of transparent photonic structures (such as distributed Bragg reflectors, holey fibers, or photonic crystals) in a homogeneous resonant atomic media such as dielectrics with homogeneously distributed impurities, atomic, or molecular gases. These optically produced photonic structures could easily be controlled (including switching on/off, changing amplitude and period of modulation) and would be highly selective in frequency, naturally limited by the width of the optical resonance. \n \nWe also derive the optical fluorescence spectra of a three-level medium driven by two coherent fields at the adjacent transitions in a general case when all three transitions are allowed. We show that coherent driving can efficiently control the distribution of intensities between the fluorescent channels. In particular, the total intensity of fluorescence at the transition which is not driven by the optical fields may essentially exceed the fluorescence intensity at the driven transitions under the condition of two-photon resonance. This counter-intuitive effect is due to depletion of the intermediate state via atomic interference.