Laser light can exhibit nonlinear behaviour when interacting with dense atomic vapours.\nThis can give rise to a variety of interesting phenomena such as slow light and optically induced transparency. Recently A.~J. van Lange measured nonlinear transmission of light through a Rubidium vapour and developed a physical model to describe these measurements. Van Lange also investigated the formation of different beam profiles, in a dense Rubidium vapour and from Gaussian input beams, as a function of intensity and optical frequency.\n\nHere we expand on van Lange's measurements by measuring over a large frequency range which includes multiple atomic transition lines and by employing off-axis holography which allows for simultaneous measurement of the intensity and phase. Analysis of beam profiles based on the structural similarity index (SSIM) uncovered beam profiles whose path through intensity-detuning space could be described with van Lange's generalised detuning curve. Off-axis holography measurements are in agreement with regular intensity measurements but exhibits a greater amount of noise.
Laser light can exhibit nonlinear behaviour when interacting with dense atomic vapours.\nThis can give rise to a variety of interesting phenomena such as slow light and optically induced transparency. Recently A.~J. van Lange measured nonlinear transmission of light through a Rubidium vapour and developed a physical model to describe these measurements. Van Lange also investigated the formation of different beam profiles, in a dense Rubidium vapour and from Gaussian input beams, as a function of intensity and optical frequency.\n\nHere we expand on van Lange's measurements by measuring over a large frequency range which includes multiple atomic transition lines and by employing off-axis holography which allows for simultaneous measurement of the intensity and phase. Analysis of beam profiles based on the structural similarity index (SSIM) uncovered beam profiles whose path through intensity-detuning space could be described with van Lange's generalised detuning curve. Off-axis holography measurements are in agreement with regular intensity measurements but exhibits a greater amount of noise.
Dense atomic vapors have strong non-linear optical properties for near-resonant light. As a result, an initially Gaussian beam profile is strongly distorted due to propagation through such a dense vapor, leading to various distinct beam profiles. In our experiment, we track the detuning from resonance at which these beam profiles occur as a function of intensity. We establish a detuning curve as a function of intensity for each shape at two different cell temperatures. After proper scaling, the detuning curves all collapse onto one universal detuning curve, which suggests that the shapes are manifestations of the same underlying phenomenon.
Abstract We study non-linear absorption of intense monochromatic light through a dense natural rubidium (Rb) vapour. We measure transmission through a 10 cm long heated vapour cell for atom densities up to 3 × 1019 m−3 and saturation parameters up to 104, for linear and circular polarisation, close to resonance on the 87Rb D2 F = 1 → F′ = 0, 1, 2 transition. The strong absorption at low intensity is frustrated by an interplay of optical non-linearities (saturation and optical pumping) and non-linear effects due to the high atom density (collisional broadening and collisional depumping). To understand the results of the transmission measurements, we developed a model that incorporates these non-linear effects into the optical absorption. The model takes into account the absolute line strengths of all transitions from both hyperfine levels of the ground state of both isotopes of naturally abundant Rb. Doppler and collisional broadening are included in the Voigt profiles for the resonances. We show the effect of each of the non-linear processes on the calculation results of the model, and from comparison with experiment we conclude that all non-linear effects are necessary for a quantitative agreement.
The quantum fluctuations of optical beams are highly correlated in electromagnetically induced transparency (EIT). The intensity fluctuations are enhanced by conversion of phase noise to intensity noise in atomic vapour. We have studied spectra of intensity fluctuations in dense rubidium vapour for different laser beam powers. Observed excess noise spectrum is broader than EIT window at the same optical power. Both spectral widths are proportional to the laser beam intensity. By using signal subtraction scheme we can reduce amplitude of the fluctuations to close the photonic short noise level. This result confirms the high degrees of intensity correlations and can be used to improve quality of optical atomic clocks.
In recent years great progress was made in the spatial control of light with dynamic phase and amplitude modulators such as spatial light modulators and digital micromirror devices. In this work we describe the theory and practice of light shaping with such devices, detailing the spatial control of amplitude, phase and polarisation of coherent laser beams. We use our expertise in generating and measuring light fields with spatially dependent polarisation structures to characterise the correlations between spatial modes and polarisation in such light fields. We do this by adapting concurrence, a quantum measure of entanglement, to these classical correlations. One of the most promising application of coherent laser light is in the control of atomic media via atom-light interactions. In this work we describe the construction of simple external cavity diode lasers designed for the generation of resonant light for atomic physics applications. We exploit these lasers and spatial light modulators to create and measure three-dimensional atomic population structures in a warm rubidium vapour. We also implement a magneto-optic and a dynamic dark spontaneous-force optical trap for rubidium. These traps produce dense (~ 10^11 cm^-3) and cold (~100 uK) clouds of rubidium atoms. We develop the theory of spatially dependent electromagnetically induced transparency in such traps using rate equations. We find that the absorption of linearly polarised light depends on the relative direction of a magnetic field and the light polarisation. We use the cold atom clouds to measure the direction of magnetic fields by using this dependence and laser beams with structured polarisation.
In this work, we present an experimental study on the spatial profile of coherent light generated in a forward four-wave mixing (FWM) process. We are interested in investigating how the transverse structure of the incident beams, more specifically of the Hermite-Gauss (HG) modes, is transferred to the generated signal in this nonlinear process. For the experiment, we used a continuous wave diode laser to excite a sample of Rubidium atoms, on the ⁸⁵Rb D2 line, tuned to the frequency of the 5²S_(1/2) ( = 3) → 5²P_(3/2) transition. With a Spatial Light Modulator, we were able to split the laser beam in two and structure them in the desired modes. These two beams, A and B, with wave vectors kA and kB, and linear orthogonal polarizations, with quasi-copropagated configuration, were used to induce two FWM signals in the directions 2kA-kB and 2kB-kA. The spatial profile of incident beams and the two nonlinear signals were captured by a CMOS camera, and the regimes of a thin or extensive medium were investigated. We were able to obtain results for a combination of gaussian-HG beams, as well as HG-HG beams. The profiles obtained by computer simulation were compared with the experimental measurements. Our theoretical model relies on solving the paraxial equation of the generated field. It leads to the overlap integrals of the incident beams, which unfold into some interesting selection rules in the transversal plane, for the thin and extensive medium regimes, and in the longitudinal axis, only for the long medium regime. Although the extensive medium regime presents some additional selection rules, the experimental requirements are difficult to achieve in our system, among them, we highlight the Gouy phase matching. On the other hand, a good agreement between theory and experiment was observed in the thin medium regime.
This thesis presents theoretical models and results of numerical simulations describing the propagation of optical pulses through dense, thermal atomic vapours. In particular we investigate the nonlinear effects of optical solitons due to self-induced transparency (SIT) in two-level systems, optical simultons in V-type three-level systems and electromagnetically induced transparency (EIT) in Λ-type systems, including the storage and retrieval of dark-state polaritons. An investigation is made into two-photon excitation of the 5D states of rubidium in a high-intensity beam including the hyperfine structure of the relevant atomic levels. Decay from these states to the 6P manifolds is ruled out as a cause of experimentally observed fluorescence due to the amount of power broadening associated with intensities necessary to provide any significant level of population in these highly excited states. We combine the nonlinear effects of optical solitons and EIT to explain experimentally observed steepened pulses in a V-type system in a micron-length cell. We explain the behaviour as the early formation of a simulton pulse drawn from a CW probe field by a strong coupling pulse, due to coherent population trapping. We predict that in a longer cell it may be possible to facilitate propagation of matched pulses, even when the transitions in the system have different propagation coefficients, as long as decoherence from collision broadening can be controlled. The fact that weak pulses can propagate with this scheme suggests an approach to achieving transparent propagation of single or few photon pulses distinct from, but related to, both SIT and EIT.