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arXiv:1805.05441 · Journal of Experimental and Theoretical Physics Letters

3D Uniform Manipulation of NV Centers in Diamond Using a Dielectric Resonator Antenna

Polina V. Kapitanova, Vladimir V. Soshenko, Vadim Vorobyov, Dmitry A. Dobrykh, Stepan V. Bolshedvorskii, Vadim N. Sorokin, Alexey V. Akimov

Published Oct 30, 2018• 23 citations
arXivHTMLPDF

Abstract

Ensembles of nitrogen-vacancy color centers in diamond hold promise for ultra-precise magnetometry, competing with superconducting quantum interference device detectors. By utilizing the advantages of dielectric materials, such as very low losses for electromagnetic field, with the potential for creating high Q -factor resonators with strong concentration of the field within it, we implemented a dielectric resonator antenna for coherent manipulation of a large ensemble of nitrogen-vacancy centers in diamond. We reached average Rabi frequency of 10 MHz in a volume of 7 mm 3 with a standard deviation of less than 1% at a moderate pump power. The obtained result enables use of large volume low nitrogen-vacancy concentration diamond plates in modern nitrogen-vacancy magnetometers thus improving sensitivity via larger coherence time and higher optical detected magnetic resonance contrast.

DOI
10.1134/s0021364018210014

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Ensembles of nitrogen-vacancy color centers in diamond hold promise for ultra-precise magnetometry, competing with superconducting quantum interference device detectors. By utilizing the advantages of dielectric materials, such as very low losses for electromagnetic field, with the potential for creating high Q -factor resonators with strong concentration of the field within it, we implemented a dielectric resonator antenna for coherent manipulation of a large ensemble of nitrogen-vacancy centers in diamond. We reached average Rabi frequency of 10 MHz in a volume of 7 mm 3 with a standard deviation of less than 1% at a moderate pump power. The obtained result enables use of large volume low nitrogen-vacancy concentration diamond plates in modern nitrogen-vacancy magnetometers thus improving sensitivity via larger coherence time and higher optical detected magnetic resonance contrast.
Ensembles of nitrogen-vacancy (NV) color centers in diamond hold promise of ultraprecise magnetometery competing with SQUID detectors.By utilizing advantages of dielectric materials such as very low losses for electromagnetic field and therefore possibility to create high quality factor resonators with strong concentration of the field in it we implemented a dielectric resonator antenna for coherent manipulation of large ensemble of NV centers in diamond.We reached average Rabi frequency of 10 MHz in the volume of 7 cubic millimeters with standard deviation less than 1% at moderate pump power.This result passes the way to improve sensitivity of cutting edge NV based magnetometers by two orders of magnitude practically reaching SQUID level of sensitivity.
Dielectric resonator antenna with circular polarization of microwave magnetic field for efficient, coherent and uniform spin manipulation at nitrogen-vacancy centers in diamond is discussed. The results of numerical simulations of the microwave magnetic field generated by the antenna are reported and analyzed. The uniform magnetic field with circular polarization is obtained inside the antenna. Using the simulated amplitude of the magnetic field inside the antenna the Rabi frequency is estimated. The Rabi frequency of 41 MHz with inhomogeneity less then 1 % for the diamond volume of 3 mm 3 is demonstrated under 10 W of input microwave power.
Quantum sensors based on nitrogen-vacancy (NV) centers in diamond are expected to demonstrate a wide variety of applications. For high-sensitivity quantum sensors with NV center ensembles, uniform manipulation of the electron spins of the NV centers in large volumes is required. In addition, a broad microwave frequency bandwidth for manipulating the NV centers' electron spin is necessary for vector magnetometry and measurement under a finite static magnetic field. Here, we demonstrate a broadband microwave antenna for uniform manipulation of millimeter-scale volumes of diamond quantum sensors. The simulation shows that the current is distributed at both edges of the loop coil of a single copper plate due to the skin effect. The loop coil acts like a Helmholtz coil, which realizes uniformity in the z-direction of the microwave magnetic field (B1). The plate structure has a higher mechanical stability, durability, and a larger heat capacity than the Helmholtz coil, due to its large volume. The antenna achieves a higher performance than previously reported antennae, with a maximal B1 of 4.5 G, a broad bandwidth of 287 ± 6 MHz, and a peak-to-peak variation of 9.2% over a 3.1 mm3 cylinder volume. These performances show that the presented antenna is suitable for manipulating solid-state spin ensembles for high-sensitivity quantum sensors.
Individual nitrogen vacancy (NV) color centers in diamond are versatile, spin-based quantum sensors. Coherently controlling the spin of NV centers using microwaves in a typical frequency range between 2.5 and 3.5 GHz is necessary for sensing applications. In this work, we present a stripline-based, planar, Ω-shaped microwave antenna that enables one to reliably manipulate NV spins. We found an optimal antenna design using finite integral simulations. We fabricated our antennas on low-cost, transparent glass substrate. We created highly uniform microwave fields in areas of roughly 400 × 400 μm2 while realizing high Rabi frequencies of up to 10 MHz in an ensemble of NV centers.
Microwave delivery to samples in a cryogenic environment can pose experimental challenges such as restricting optical access, space constraints, and heat generation. Moreover, existing solutions that overcome various experimental restrictions do not necessarily provide a large homogeneous oscillating magnetic field over macroscopic length scales, which is required for control of spin ensembles or fast gate operations in scaled-up quantum computing implementations. Here, we show fast and coherent control of a negatively charged nitrogen-vacancy spin ensemble by taking advantage of the high permittivity of a KTaO3{\mathrm{K}\mathrm{Ta}\mathrm{O}}_{3}KTaO3​ dielectric resonator at cryogenic temperatures. We achieve Rabi frequencies of up to 48 MHz, with a total power-to-field conversion factor CP=9.66mT/W{C}_{\mathrm{P}}=\phantom{\rule{0.2em}{0ex}}9.66\phantom{\rule{0.2em}{0ex}}\mathrm{mT}/\sqrt{\mathrm{W}}CP​=9.66mT/W​ (approximately 191MHzRabi/W191\phantom{\rule{0.2em}{0ex}}{\mathrm{MHz}}_{\mathrm{Rabi}}/\sqrt{\mathrm{W}}191MHzRabi​/W​). We use the nitrogen-vacancy-center spin ensemble to probe the quality factor, the coherent enhancement, and the spatial distribution of the magnetic field inside the diamond sample. The key advantages of the dielectric resonator utilized in this work are ease of assembly, in situ tunability, a high magnetic field conversion efficiency, a low-volume footprint, and optical transparency. This makes KTaO3{\mathrm{K}\mathrm{Ta}\mathrm{O}}_{3}KTaO3​ dielectric resonators a promising platform for the delivery of microwave fields for the control of spins in various materials at cryogenic temperatures.
For quantum sensing based on nitrogen-vacancies (NV) ensembles, microwave antennas can couple the microwave field to the NV center, which leads it to becoming the core of spin manipulation and can directly affect the sensitivity of quantum sensing. The double split-ring resonator is a widely used microwave device for NV ensembles due to the advantages of high radiation efficiency and uniform magnetic field in millimeter-scale areas. But the bandwidth (30 MHz) is quite narrow which limits the application in quantum sensing with NV ensembles. Here, we experimentally achieve continuous tuning of the resonant frequency of the double split-ring resonator by changing the copper sheet position on the edge of the outer ring. The frequency tuning range can reach 80 MHz, up to 2-3 times the bandwidth, which can cover the transition of the electron spin under different magnetic field conditions. The performance of the tunable antenna in the quantum operation of NV centers is verified by optically detected magnetic resonance and Rabi oscillation. This tunable antenna is promising in the fabrication of integrated and arrayed quantum sensors based on NV ensembles.