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arXiv:1804.08684 · Optics Letters

Interplay between spontaneous decay rates and Lamb shifts in open photonic systems

Emmanuel Lassalle, Nicolas Bonod, Thomas Durt, Brian Stout

Published Apr 13, 2018• 21 citations
arXivHTMLPDF

Abstract

In this Letter, we describe the modified decay rate and photonic Lamb (frequency) shift of quantum emitters in terms of the resonant states of a neighboring photonic resonator. This description illustrates a fundamental distinction in the behaviors of closed (conservative) and open (dissipative) systems: the Lamb shift is bounded by the emission linewidth in closed systems while it overcomes this limit in open systems.

DOI
10.1364/ol.43.001950

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In this Letter, we describe the modified decay rate and photonic Lamb (frequency) shift of quantum emitters in terms of the resonant states of a neighboring photonic resonator. This description illustrates a fundamental distinction in the behaviors of closed (conservative) and open (dissipative) systems: the Lamb shift is bounded by the emission linewidth in closed systems while it overcomes this limit in open systems.
We study the non-Markovian quantum dynamics of an emitter inside an open multimode cavity, focusing on the case where the emitter is resonant with high-frequency cavity modes. Based on a Green's-function technique suited for open photonic structures, we study the crossovers between three distinct regimes as the coupling strength is gradually increased: (i) overdamped decay with a time scale given by the Purcell modified decay rate, (ii) underdamped oscillations with a time scale given by the effective vacuum Rabi frequency, and (iii) pulsed revivals. The final multimode strong-coupling regime (iii) gives rise to quantum revivals of the atomic inversion on a time scale associated with the cavity round-trip time. We show that the crucial parameter to capture the crossovers between these regimes is the nonlinear Lamb shift, accounted for exactly in our formalism.
We present an universal description for Lamb shift of a lossy two-level-emitter (TLE) inside a leaky cavity by combining the quantum dissipation theory and the perturbative treatment developed in cavity QED. The total spectrum function of bath associated with the TLE is deduced by the standard method developed for a quantum dissipation model, from which the total spontaneous emission rate and Lamb shift are calculated. The developed calculation scheme is able to reproduce the known Purcell enhancement factor and is shown to be in agreement with the analysis made for a confocal resonator. It is found that the Lamb shift due to a leaky cavity mode has a sharp drop when sweeping across the resonance point. The physics behind this unusual behavior and the related experimental observations made on both atom-cavity and quantum-dot cavity systems are also analyzed.
Any quantum-confined electronic system coupled to the electromagnetic continuum is subject to radiative decay and renormalization of its energy levels. When coupled to a cavity, these quantities can be strongly modified with respect to their values in vacuum. Generally, this modification can be accurately captured by including only the closest resonant mode of the cavity. In the circuit quantum electrodynamics architecture, it is, however, found that the radiative decay rates are strongly influenced by far off-resonant modes. A multimode calculation accounting for the infinite set of cavity modes leads to divergences unless a cutoff is imposed. It has so far not been identified what the source of divergence is. We show here that unless gauge invariance is respected, any attempt at the calculation of circuit QED quantities is bound to diverge. We then present a theoretical approach to the calculation of a finite spontaneous emission rate and the Lamb shift that is free of cutoff.
A landmark in the development of quantum electrodynamics was the discovery that emission–reabsorption of virtual photons modifies the value of energy levels in an atom from those computed by using Dirac’s equation (Lamb shift). An early result of statistical quantum electrodynamics was that the exchange of virtual photons in an ensemble of identical atoms leads as well to a change in the frequency of the radiation emitted from this system (cooperative Lamb shift). Dicke’s discovery that coherence effects lead to the shortening of the emission lifetime from a small sample by a factor equal to the number of atoms in the ensemble (superradiance or cooperative decay rate) was an early landmark in quantum optics. Both cooperative decay rate and cooperative Lamb shift were shown to have the same physical origin—the exchange of virtual photons, a process described by the Lienard–Wiechert dipole–dipole interaction. This effective potential is the kernel of the integral equation describing the dynamics of the system. This complex long-range kernel gives, for both cooperative quantities, strong dependence on the geometry of the atomic cloud. I summarize the known expressions for the initial cooperative decay rate and the cooperative Lamb shift in different geometries. The results for both the scalar photon and the vector photon (electrodynamics) theories for experimentally realizable systems of either uniform or phased polarization are given.
Motivated by the significant controversy between the two dispersion models and Weisskopf-Wigner approximation (WWA), for the first time to our knowledge, we introduce the position-dependent photon-atom interaction into the Green function method of the evolution operator and develop a universal theoretical treatment on spontaneous emission of atoms in photonic crystals (PCs). A position-sensitive generalized Lorentzian formulism (non-Lorentzian shape) for the decay of an excited atom in PCs is derived, an exact numerical method for calculating the local coupling strength, proportional to the photonic local density of state (LDOS), is presented. For weak interaction PCs with pseudo gaps, the generalized Lorentzian formulism may be reduced to the famous Lorentzian spectrum. In this case, we introduced a lifetime distribution function for an assembly of atoms and found that the lifetime distribution strongly depend on the spread configuration of these atoms in space, which clarifies successfully the tremendous discrepancy between different experiments. For the PCs with large full gaps, we found that the atomic position can fundamentally change the decay behavior of an excited atom: in strong interaction positions, the atomic decay is non-classical or exhibits an envelope-damped Rabi oscillation, while in weak interaction positions the WWA is valid. Recently, we also predicted giant Lamb shifts for hydrogen atoms in PCs, and revealed that in inhomogeneous electromagnetic environment, the dominant contribution to the Lamb shift comes from real photon emission, while the contribution from emission and reabsorption of virtual photon is negligible, in vast contrast with the case of free space where the virtual photon processes play a key role.
It is now well established that radiative decay of quantum emitters can be strongly modified by their environment. In this paper, we present an exact—within the weak-coupling approximation—multipole expression to compute the Lamb (frequency) shift induced by an arbitrary set of resonant scatterers on a nearby quantum emitter, using multiscattering theory. We also adopt a quasi-normal mode description to account for the line shape of the Lamb shift spectrum in the near field of a plasmonic nanosphere. It is then shown that the Lamb shift resonance can be blueshifted as the size of the nanoparticle increases, suggesting that nanoparticles may be used to tune this resonant interaction. Finally, a realistic calculation of the Lamb shift is made for a dimer configuration.