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arXiv:1306.4787 · Physical Review A

Route from spontaneous decay to complex multimode dynamics in cavity QED

Dmitry O. Krimer, Matthias Liertzer, Stefan Rotter, Hakan E. Türeci

Published Mar 11, 2014• 51 citations
arXivHTMLPDF

Abstract

We study the non-Markovian quantum dynamics of an emitter inside an open multimode cavity, focusing on the case where the emitter is resonant with high-frequency cavity modes. Based on a Green's-function technique suited for open photonic structures, we study the crossovers between three distinct regimes as the coupling strength is gradually increased: (i) overdamped decay with a time scale given by the Purcell modified decay rate, (ii) underdamped oscillations with a time scale given by the effective vacuum Rabi frequency, and (iii) pulsed revivals. The final multimode strong-coupling regime (iii) gives rise to quantum revivals of the atomic inversion on a time scale associated with the cavity round-trip time. We show that the crucial parameter to capture the crossovers between these regimes is the nonlinear Lamb shift, accounted for exactly in our formalism.

DOI
10.1103/physreva.89.033820

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We study the non-Markovian quantum dynamics of an emitter inside an open multimode cavity, focusing on the case where the emitter is resonant with high-frequency cavity modes. Based on a Green's-function technique suited for open photonic structures, we study the crossovers between three distinct regimes as the coupling strength is gradually increased: (i) overdamped decay with a time scale given by the Purcell modified decay rate, (ii) underdamped oscillations with a time scale given by the effective vacuum Rabi frequency, and (iii) pulsed revivals. The final multimode strong-coupling regime (iii) gives rise to quantum revivals of the atomic inversion on a time scale associated with the cavity round-trip time. We show that the crucial parameter to capture the crossovers between these regimes is the nonlinear Lamb shift, accounted for exactly in our formalism.
We present a Heisenberg-Langevin formalism to study the effective dynamics of a superconducting qubit coupled to an open multimode resonator, without resorting to the rotating wave, two level, Born or Markov approximations. Our effective equations are derived by eliminating resonator degrees of freedom while encoding their effect in the Green's function of the electromagnetic background. We account for the openness of the resonator exactly by employing a spectral representation for the Green's function in terms of a set of non-Hermitian modes. A well-behaved time domain perturbation theory is derived to systematically account for the nonlinearity of weakly nonlinear qubits like transmon. We apply this method to the problem of spontaneous emission, capturing accurately the non-Markovian features of the qubit dynamics, valid for any qubit-resonator coupling strength. Any discrete-level quantum system coupled to the electromagnetic continuum is subject to radiative decay and renormalization of its energy levels. When inside a cavity, these quantities can be strongly modified with respect to vacuum. Generally, this modification can be captured by including only the closest resonant cavity mode. In circuit-QED architecture, with substantial coupling strengths, it is however found that such rates are strongly influenced by far off-resonant modes. A multimode calculation over the infinite set of cavity modes leads to divergences unless an artificial cutoff is imposed. Previous studies have not pointed out what the source of this divergence is. We show that unless the effect of A2A^2A2 is accounted for up to all orders exactly, any multimode calculations of circuit-QED quantities is bound to diverge. Subsequently, we present the calculation of finite radiative corrections to qubit properties that is free of an artificially introduced high frequency cut-off.
We study the radiative properties---the Lamb shift, Purcell decay rate, and spontaneous emission dynamics---of an artificial atom coupled to a long, multimode cavity formed by an array of Josephson junctions. Introducing a tunable coupling element between the atom and the array, we demonstrate that such a system can exhibit a crossover from a perturbative to a nonperturbative regime of light-matter interaction as one strengthens the coupling between the atom and the Josephson-junction array. As a consequence, the concept of spontaneous emission as the occupation of the local atomic site being governed by a single complex-valued exponent breaks down. This breakdown, we show, can be interpreted in terms of formation of hybrid atom-resonator modes with radiative losses that are nontrivially related to the effective coupling between individual modes. We develop a singular function expansion approach for the description of the open quantum system dynamics in such a multimode nonperturbative regime. This modal framework generalizes the normal-mode description of quantum fields in a finite volume, incorporating exact radiative losses and incident quantum noise at the delimiting surface. Our results are pertinent to recent experiments with Josephson atoms coupled to high-impedance Josephson-junction arrays.
In the multimode regime of cavity quantum electrodynamics (cQED), light-matter coupling can be strong enough such as to allows a quantum emitter to couple with multiple resonant field modes. This regime leaves distinctive signatures in the behavior of both the field and the emitter, which are already accessible by modern experimental techniques. To model such effects in lossy cavities, effective discrete-mode approaches have been widely employed, despite their accuracy beyond two modes remaining rarely benchmarked. In this work, we demonstrate the necessity of employing multiple modes to describe the multimode signatures by analyzing the dynamics of an atom in a one-dimensional lossy resonator. The atom's dynamics is simulated using the formalism developed in Weitzel et al. (2026) (arXiv:2512.18478), where a resonance quantization prescription is provided. We investigate its dependency with respect to two different parameters: the light-matter coupling strength and the atom's position. In the former case, we find that the minimal number of modes necessary to capture the essential features of the atom's dynamics increases with the coupling strength. In the latter, we further observe that the multimode regime leads to a strong position-dependency of the atom's dynamics. In all cases, we discuss the physical interpretation of our results and further discuss about how the employed formalism can be used to recover physically relevant quantities.
We analyze the non-Markovian spontaneous-emission dynamics of a two-level test atom placed in a cavity formed by two atomic arrays in a waveguide quantum electrodynamics (QED) setup. We demonstrate a crossover from single-mode to multimode strong-coupling cavity QED as the cavity length $\ensuremath{\sim}d$ becomes comparable to the coherence length associated with collective spontaneous emission $\ensuremath{\sim}v/(N\ensuremath{\gamma})$. The resulting non-Markovian dynamics of the test atom and the emergent spectral density of the field are analyzed as a function of various tunable atomic array parameters: the number of atoms, length of the atomic cavity, and resonance frequency of the atoms forming the atomic mirrors. Our results show limitations to cooperatively enhanced light-matter coupling in the presence of time-delayed feedback. We further illustrate that the non-Markovian system dynamics can be efficiently approximated in terms of a few modes of the emergent spectral density of the field.
We study the dynamics of a transmon qubit that is capacitively coupled to an open multimode superconducting resonator. Our effective equations are derived by eliminating resonator degrees of freedom while encoding their effect in the Green's function of the electromagnetic background. We account for the dissipation of the resonator exactly by employing a spectral representation for the Green's function in terms of a set of non-Hermitian modes and show that it is possible to derive effective Heisenberg-Langevin equations without resorting to the rotating-wave, two-level, Born, or Markov approximations. A well-behaved time-domain perturbation theory is derived to systematically account for the nonlinearity of the transmon. We apply this method to the problem of spontaneous emission, capturing accurately the non-Markovian features of the qubit dynamics, valid for any qubit-resonator coupling strength.
We revisit the superstrong coupling regime of multi-mode cavity quantum electrodynamics (QED), defined to occur when the frequency of vacuum Rabi oscillations between the qubit and the nearest cavity mode exceeds the cavity's free spectral range. A novel prediction is made that the cavity's linear spectrum, measured in the vanishing power limit, can acquire an intricate fine structure associated with the qubit-induced cascades of coherent single-photon down-conversion processes. This many-body effect is hard to capture by a brute-force numerics and it is sensitive to the light-matter coupling parameters both in the infra-red and the ultra-violet limits. We focused at the example case of a superconducting fluxonium qubit coupled to a long transmission line section. The conversion rate in such a circuit QED setup can readily exceed a few MHz, which is plenty to overcome the usual decoherence processes. Analytical calculations were made possible by an unconventional gauge choice, in which the qubit circuit interacts with radiation via the flux/charge variable in the low-/high-frequency limits, respectively. Our prediction of the fine spectral structure lays the foundation for the "strong down-conversion" regime in quantum optics, in which a single photon excited in a non-linear medium spontaneously down-converts faster than it is absorbed.