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arXiv:1804.08405 · Nature Communications

Parity transitions in the superconducting ground state of hybrid InSb–Al Coulomb islands

Jie Shen, Sebastian Heedt, Francesco Borsoi, Bernard van Heck, Saša Gazibegović, Roy L. M. Op het Veld, Diana Car, John A. Logan, Mihir Pendharkar, Senja J. J. Ramakers, Guanzhong Wang, Di Xu, Daniël Bouman, Attila Geresdi, Chris J. Palmstrøm, Erik P. A. M. Bakkers, Leo P. Kouwenhoven

Published Nov 9, 2018• 69 citations
arXivHTMLPDF

Abstract

The number of electrons in small metallic or semiconducting islands is quantised. When tunnelling is enabled via opaque barriers this number can change by an integer. In superconductors the addition is in units of two electron charges (2e), reflecting that the Cooper pair condensate must have an even parity. This ground state (GS) is foundational for all superconducting qubit devices. Here, we study a hybrid superconducting-semiconducting island and find three typical GS evolutions in a parallel magnetic field: a robust 2e-periodic even-parity GS, a transition to a 2e-periodic odd-parity GS, and a transition from a 2e- to a 1e-periodic GS. The 2e-periodic odd-parity GS persistent in gate-voltage occurs when a spin-resolved subgap state crosses zero energy. For our 1e-periodic GSs we explicitly show the origin being a single zero-energy state gapped from the continuum, i.e., compatible with an Andreev bound states stabilized at zero energy or the presence of Majorana zero modes.

DOI
10.1038/s41467-018-07279-7

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The number of electrons in small metallic or semiconducting islands is quantised. When tunnelling is enabled via opaque barriers this number can change by an integer. In superconductors the addition is in units of two electron charges (2e), reflecting that the Cooper pair condensate must have an even parity. This ground state (GS) is foundational for all superconducting qubit devices. Here, we study a hybrid superconducting-semiconducting island and find three typical GS evolutions in a parallel magnetic field: a robust 2e-periodic even-parity GS, a transition to a 2e-periodic odd-parity GS, and a transition from a 2e- to a 1e-periodic GS. The 2e-periodic odd-parity GS persistent in gate-voltage occurs when a spin-resolved subgap state crosses zero energy. For our 1e-periodic GSs we explicitly show the origin being a single zero-energy state gapped from the continuum, i.e., compatible with an Andreev bound states stabilized at zero energy or the presence of Majorana zero modes.
Quantum computers can solve some problems exponentially faster than classical computers. Unfortunately, the computational power of quantum computers is currently limited by the number of working qubits. It is difficult to scale up these systems, because qubits are easily affected by noise in their environment. This noise leads to decoherence: loss of the qubit’s encoded information. A possible solution to diminish decoherence is using Majorana box qubits, as these qubits are predicted to be insensitive to local noise. However, this promising type of qubit does not exist yet. With the research described in this thesis, we aim to contribute to the development of Majorana box qubits (MBQs). In these qubits, Majorana zero modes, the basic elements of MBQs, are contained within a superconducting island to suppress Majorana parity fluctuations caused by quasiparticle poisoning. To enable parity readout of the MBQ, these modes are coupled to quantum dots within a nanowire network. To help realize MBQs, we need a better understanding of quasiparticles in superconducting islands, parity-readout techniques, and ways to fabricate nanowire networks. These three aspects are the focus of the experiments presented in this thesis. To study superconducting islands and readout techniques, we used InAs semiconductor nanowires with an epitaxially grown Al shell. Majorana signatures have already been observed in such nanowires. We addressed quasiparticle dynamics in superconducting islands by measuring the gate-charge modulation of the switching current. We found a consistent 2e-periodic modulation at zero magnetic field, and an exponential decrease of parity lifetime with increasing magnetic field. We explored MBQ readout, using a quantum dot level as a proxy for a Majorana zero mode, and measured its charge hybridization with another dot using gate-based readout. We showed that we can rapidly discriminate between two settings with different tunnel couplings, demonstrating the potential of gate-based readout to measure MBQs. And, using gate-based readout, we could study charge-transfer processes occurring in hybrid structures of superconducting islands coupled to quantum dots. Finally, to find a good material platform for nanowire networks, we characterized two two-dimensional systems. We realized quantum point contacts in InSb, which we used to measure the ggg-factor anisotropy, and effective electron mass in this system. And, we studied the spin-orbit interaction in InAs/GaSb by extracting the difference in density between electrons with different spin orientations. This thesis finishes with a proposal for a series experiments to realize MBQs. These experiments make use of superconducting islands and the reflectometry setup we developed for gate-based readout.
Small superconducting islands can exhibit charge quantization, where Coulomb interactions compete with Cooper pairing. Using scanning tunneling spectroscopy, we probe this interplay by measuring the charging energy (E_{C}) and the pairing energy (Δ) of individual Pb nanoislands. Below a critical island size, where E_{C}>Δ, we observe a crossover between even and odd parity ground states. By applying controlled voltage pulses, we continuously tune the island's electrostatic potential and map the full charge-parity landscape. These results demonstrate tunable superconducting ground states, offering a potential platform for qubit design and control.
A practical quantum computer demands a physical quantum bit (qubit) that is scalable, has a well-defined initial state, and brings together coherence with reliable control and read-out. A compelling idea is to put together a locally protected Majorana qubit with a superconducting qubit. The superconducting qubit is used to read out the Majorana states while the Majorana qubit may act as a quantum memory. This thesis presents a series of studies on quantum transport in semiconducting nanowires coupled to superconductors to investigate various platforms for realizing Majorana. These studies are followed by microwave measurements on superconducting circuits compatible with semiconducting-superconducting heterostructures. We first evaluate the potential of Ge/Si core/shell nanowires by achieving induced superconductivity as well as estimating spin-orbit coupling. Next we explore the transport mediated by Andreev bound states formed in InSb nanowire quantum. A subgap negative differential conductance is investigated together with the coalescing Andreev resonances at zero bias relevant for the correct interpretation of Majorana experiments done on the same structures. We conclude our studies of semiconducting nanowires by exploring tunnel junctions in Sn-InSb nanowires that are prepared by in-situ shadowing using nearby nanowires and flakes. Tin shells are found to induce a hard superconducting gap persisting up to high magnetic fields. We observe the two-electron charging effect from a small superconducting island of Sn-InSb. This effect is attributed to charge parity stability, which makes this nanowire system an intriguing candidate for superconducting and topological quantum circuits. These Sn-InSb junctions are then used as the nonlinear element in a transmon qubit design where we observe a dispersive coupling between this nanowire Josephson junction and a superconducting resonator. We also present our progress towards building a magnetic field resilient superconducting circuit that allows integration with semiconducting and topological structures. In the last chapter, InSb semiconducting nanowires are utilized as shadow masks prior to superconductor deposition on an InAs quantum well. We study Josephson current properties in Josephson junctions made from these nanowire shadows. Our results point to highly transparent junctions that can be developed further for hybrid superconductor-semiconductor qubit systems.
We study the interplay between Coulomb blockade and superconductivity in a tunable superconductor-superconductor-normal-metal single-electron transistor. The device is realized by connecting the superconducting island via an oxide barrier to the normal-metal lead and with a break junction to the superconducting lead. The latter enables Cooper pair transport and (multiple) Andreev reflection. We show that these processes are relevant also far above the superconducting gap and that signatures of Coulomb blockade may reoccur at high bias while they are absent for small bias in the strong-coupling regime. Our experimental findings agree with simulations using a rate equation approach in combination with the full counting statistics of multiple Andreev reflection.
We investigate the superconducting Anderson impurity model for interacting quantum dot Josephson junctions with spin-orbit coupling and a term accounting for tunnelling through higher-energy orbitals. These elements establish the conditions required for spin polarization in the absence of external magnetic field at finite superconducting phase bias. This Hamiltonian has been previously used to model the Andreev spin qubit, where quantum information is encoded in spinful odd-parity subgap states. Here we instead analyse the even-parity sector, i.e., the Andreev pair qubit based on Andreev bound states (ABS). The model is solved using the zero-bandwidth approximation and the numerical renormalization group, with further insight from variational calculations. Electron-electron interaction admixes single-occupancy Yu-Shiba-Rusinov (YSR) components into the ABS states, thereby strongly enhancing spin transitions in the presence of spin-orbit coupling. The ABS states can thus become sensitive to local magnetic field fluctuations, which has implications for decoherence in Andreev pair qubits. For strong interaction U U , especially in the cross-over region between the ABS and YSR regimes for U \sim 2\Delta U ∼ 2 Δ , charge, spin, and inductive transitions can all become strong, offering avenues for spin control and quantum transduction.