Quantum computers can solve some problems exponentially faster than classical computers. Unfortunately, the computational power of quantum computers is currently limited by the number of working qubits. It is difficult to scale up these systems, because qubits are easily affected by noise in their environment. This noise leads to decoherence: loss of the qubit’s encoded information. A possible solution to diminish decoherence is using Majorana box qubits, as these qubits are predicted to be insensitive to local noise. However, this promising type of qubit does not exist yet. With the research described in this thesis, we aim to contribute to the development of Majorana box qubits (MBQs). In these qubits, Majorana zero modes, the basic elements of MBQs, are contained within a superconducting island to suppress Majorana parity fluctuations caused by quasiparticle poisoning. To enable parity readout of the MBQ, these modes are coupled to quantum dots within a nanowire network. To help realize MBQs, we need a better understanding of quasiparticles in superconducting islands, parity-readout techniques, and ways to fabricate nanowire networks. These three aspects are the focus of the experiments presented in this thesis. To study superconducting islands and readout techniques, we used InAs semiconductor nanowires with an epitaxially grown Al shell. Majorana signatures have already been observed in such nanowires. We addressed quasiparticle dynamics in superconducting islands by measuring the gate-charge modulation of the switching current. We found a consistent 2e-periodic modulation at zero magnetic field, and an exponential decrease of parity lifetime with increasing magnetic field. We explored MBQ readout, using a quantum dot level as a proxy for a Majorana zero mode, and measured its charge hybridization with another dot using gate-based readout. We showed that we can rapidly discriminate between two settings with different tunnel couplings, demonstrating the potential of gate-based readout to measure MBQs. And, using gate-based readout, we could study charge-transfer processes occurring in hybrid structures of superconducting islands coupled to quantum dots. Finally, to find a good material platform for nanowire networks, we characterized two two-dimensional systems. We realized quantum point contacts in InSb, which we used to measure the $g$-factor anisotropy, and effective electron mass in this system. And, we studied the spin-orbit interaction in InAs/GaSb by extracting the difference in density between electrons with different spin orientations. This thesis finishes with a proposal for a series experiments to realize MBQs. These experiments make use of superconducting islands and the reflectometry setup we developed for gate-based readout.
Quantum computers can solve some problems exponentially faster than classical computers. Unfortunately, the computational power of quantum computers is currently limited by the number of working qubits. It is difficult to scale up these systems, because qubits are easily affected by noise in their environment. This noise leads to decoherence: loss of the qubit’s encoded information. A possible solution to diminish decoherence is using Majorana box qubits, as these qubits are predicted to be insensitive to local noise. However, this promising type of qubit does not exist yet. With the research described in this thesis, we aim to contribute to the development of Majorana box qubits (MBQs). In these qubits, Majorana zero modes, the basic elements of MBQs, are contained within a superconducting island to suppress Majorana parity fluctuations caused by quasiparticle poisoning. To enable parity readout of the MBQ, these modes are coupled to quantum dots within a nanowire network. To help realize MBQs, we need a better understanding of quasiparticles in superconducting islands, parity-readout techniques, and ways to fabricate nanowire networks. These three aspects are the focus of the experiments presented in this thesis. To study superconducting islands and readout techniques, we used InAs semiconductor nanowires with an epitaxially grown Al shell. Majorana signatures have already been observed in such nanowires. We addressed quasiparticle dynamics in superconducting islands by measuring the gate-charge modulation of the switching current. We found a consistent 2e-periodic modulation at zero magnetic field, and an exponential decrease of parity lifetime with increasing magnetic field. We explored MBQ readout, using a quantum dot level as a proxy for a Majorana zero mode, and measured its charge hybridization with another dot using gate-based readout. We showed that we can rapidly discriminate between two settings with different tunnel couplings, demonstrating the potential of gate-based readout to measure MBQs. And, using gate-based readout, we could study charge-transfer processes occurring in hybrid structures of superconducting islands coupled to quantum dots. Finally, to find a good material platform for nanowire networks, we characterized two two-dimensional systems. We realized quantum point contacts in InSb, which we used to measure the g-factor anisotropy, and effective electron mass in this system. And, we studied the spin-orbit interaction in InAs/GaSb by extracting the difference in density between electrons with different spin orientations. This thesis finishes with a proposal for a series experiments to realize MBQs. These experiments make use of superconducting islands and the reflectometry setup we developed for gate-based readout.
A practical quantum computer demands a physical quantum bit (qubit) that is scalable, has a well-defined initial state, and brings together coherence with reliable control and read-out. A compelling idea is to put together a locally protected Majorana qubit with a superconducting qubit. The superconducting qubit is used to read out the Majorana states while the Majorana qubit may act as a quantum memory. This thesis presents a series of studies on quantum transport in semiconducting nanowires coupled to superconductors to investigate various platforms for realizing Majorana. These studies are followed by microwave measurements on superconducting circuits compatible with semiconducting-superconducting heterostructures. We first evaluate the potential of Ge/Si core/shell nanowires by achieving induced superconductivity as well as estimating spin-orbit coupling. Next we explore the transport mediated by Andreev bound states formed in InSb nanowire quantum. A subgap negative differential conductance is investigated together with the coalescing Andreev resonances at zero bias relevant for the correct interpretation of Majorana experiments done on the same structures. We conclude our studies of semiconducting nanowires by exploring tunnel junctions in Sn-InSb nanowires that are prepared by in-situ shadowing using nearby nanowires and flakes. Tin shells are found to induce a hard superconducting gap persisting up to high magnetic fields. We observe the two-electron charging effect from a small superconducting island of Sn-InSb. This effect is attributed to charge parity stability, which makes this nanowire system an intriguing candidate for superconducting and topological quantum circuits. These Sn-InSb junctions are then used as the nonlinear element in a transmon qubit design where we observe a dispersive coupling between this nanowire Josephson junction and a superconducting resonator. We also present our progress towards building a magnetic field resilient superconducting circuit that allows integration with semiconducting and topological structures. In the last chapter, InSb semiconducting nanowires are utilized as shadow masks prior to superconductor deposition on an InAs quantum well. We study Josephson current properties in Josephson junctions made from these nanowire shadows. Our results point to highly transparent junctions that can be developed further for hybrid superconductor-semiconductor qubit systems.
One of the essential limitations for a physical realisation of topological-qubit based quantum computing is the problem of uncontrolled quasiparticle poisoning of the superconducting charge island. These quasiparticles have been previously reported as a known limiting factor in most of the superconducting architectures. To this end, we consider the importance of equilibrium quasiparticle poisoning in hybrid semiconducting-superconducting systems believed to be able to host Majoranas. We employed gate-based dispersive sensing by investigating a reflected radiofrequency (RF) signal from a resonator, which is capacitively coupled to one of the gate electrodes of the hybrid double dot realised in an InAs nanowire. This way, the quantum capacitance of the system can be probed, which in turn reveals charge tunnelling processes, and can be used as an indicator of single-electron tunnelling events. By operating the device in a so-called floating regime, where a double dot system is entirely decoupled from the leads, external non-equilibrium quasiparticle poisoning events can be exponentially suppressed. By appropriately tuning the chemical potentials on the quantum dot and the superconducting island, we attempt to scrutinise the dynamics of the quasiparticles innate to the superconductor. We investigated the dependence of quasiparticle tunnelling rates on the temperature of the system, as well as the applied RF power, as both are predicted to increase the average number of quasiparticles on the island. In both cases, we could find no observational proof of quasiparticle tunnelling events through the use of our measurement technique. We report an observation of a two-level resonator response, which we explain using a two-level fluctuator. Analysing telegraph measurements, we demonstrate the viability of the analysis tool, which allows us to determine the average occupation times of each state. In principle, for processes occurring at rates slower than the measurement frequency, this technique can be used to convert a\nrelatively faint difference between the “poisoned and unpoisoned state”, to the signal of the gate being on coulomb resonance versus on Coulomb blockade, which is a much clearer signal to distinguish. Both, the technique, as well as the expected rates of the physical processes within the island, are evaluated in the context of the experiment.
Spin and topological-qubit based quantum computers require an easily scalable and highly sensitive method for readout and manipulation, for which Dispersive Gate Sensing (DGS) is a promising candidate [1, 2]. DGS enables sensing of single electron tunneling events in a mesoscopic system by measuring a reflected Radio Frequency (RF) signal from a resonator capacitively coupled to one of the system’s gate electrodes. From the resonator’s perspective, the system is modeled as an effective ‘parametric capacitance’ [3]. Motivated by its viability for qubit readout and control, we measure transport characteristics of a semiconducting-superconducting hybrid charge island system using this method. Doing so, we observe a spin degeneracy modulation of interdot tunnel couplings resulting from hybridization of a dot orbital with a subgap state of the superconductor, measured entirely within Coulomb blockade. Without DC measurement, we also track a subgap state’s energy via voltage intervals between island charge states as a function of field. Subsequently, we attempt to correlate changes in the resonator’s internal dissipation with coherence of tunneling into the superconducting island. In particular, we collapse a superconducting island’s lowest energy state to the Fermi level by applying a magnetic field. Contrary to expectations, internal dissipation in the resonator did not change dramatically with field, in fact decreasing at charge degeneracy points at all field strengths. We corroborate measurements with existing theory, augmented by simple analytical and numerical models demonstrating that coherence factors of superconducting quasiparticle states and the degeneracy of dot orbitals modulate parametric capacitance. A master equation model of finite temperature interdot tunneling is solved, agreeing with experimental evidence that Sisyphus dissipation is negligible when a dot orbital is hybridized with multiple independent quasiparticle states. To be employed in quantum computers, a full understanding of all phenomena contributing to a DGS signal in these hybrid systems is critical. Hence, these results mark a step towards unambiguous readout of Majorana parity in topological qubits [4].
Building a fault-tolerant quantum computer requires physical qubits with exceptionally low error rates. An exciting proposal for achieving this goal is to employ Majorana-based qubits, which may have error rates that are exponentially suppressed in macroscopic system parameters. Specifically, for Majorana qubits based on topological superconducting nanowires, errors are expected to be exponentially suppressed in the nanowire length, superconducting gap, and decreasing temperature. This thesis investigates errors in Majorana-based qubits from excited quasiparticles due to changes in chemical potentials and 1/f charge noise, and shows that such errors are not exponentially suppressed and can be quite substantial. In the first study of this thesis, we show that small temporal variations of the chemical potential can cause errors that grow linearly with the length of the nanowire. These errors stem from leakage into excited bulk quasiparticle states, which poison Majorana modes at opposite ends of the nanowire. We further demonstrate that the dynamics of this leakage are captured by the half Landau-Zener effect, which dictates its dependence on key parameters such as the superconducting gap, chemical potential variations, and dynamic changes in the spatial profile of Majorana modes. In the second study we investigate quasiparticle excitations due to high-frequency components of 1/f charge noise, which is ubiquitous in the materials surrounding the nanowire. We model 1/f noise as arising from two level fluctuators which cause chemical potential fluctuations following random telegraph noise. We demonstrate that 1/f noise causes error rates which grow linearly with the system size and are not exponentially suppressed in the superconducting gap. For existing tetron qubit designs, we estimate decoherence times to be an order of magnitude shorter than the target 1μs measurement time. This thesis also develops an algorithmic framework for applying the covariance matrix method to the time-dependent Kitaev chain model. This extends upon existing approaches, providing a key numerical tool used throughout this thesis. This work motivates engineering strategies to reduce coupling to two level systems in Majorana qubits, such as increasing the nanowire capacitance. Beyond Majoranas, a promising avenue is to investigate the impact of this quasiparticle excitation mechanism on superconducting circuits, such as superconducting qubits, resonators, and single-photon detectors.
We present a theoretical analysis of a Majorana-based qubit consisting of two topological superconducting islands connected via a Josephson junction. The qubit is operated by electrostatic gates which control the coupling of two of the four Majorana zero modes. At the end of the operation, readout is performed in the charge basis. Even though the operations are not topologically protected, the proposed experiment can potentially shed light on the coherence of the parity degree of freedom in Majorana devices and serve as a first step towards topological Majorana qubits. We discuss in detail the charge-stability diagram and its use for characterizing the parameters of the devices, including the overlap of the Majorana edge states. We describe the multilevel spectral properties of the system and present a detailed study of its controlled coherent oscillations, as well as decoherence resulting from coupling to a non-Markovian environment. In particular, we study a gate-controlled protocol where conversion between Coulomb-blockade and transmon regimes generates coherent oscillations of the qubit state due to the overlap of Majorana modes. We show that, in addition to fluctuations of the Majorana coupling, considerable measurement errors may be accumulated during the conversion intervals when electrostatic fluctuations in the superconducting islands are present. These results are also relevant for several proposed implementations of topological qubits which rely on readout based on charge detection.
The technology of quantum computing is believed to solve certain computational problems significantly faster than classical computers, enabling classically inaccessible problems. However, the technology is still in its infancy and it is still too early to conclude which physical system(s) will form the basis of tomorrow's quantum computer. Small-scale quantum processors, built on the superconducting transmon qubit, demonstrated already the anticipated quantum speed-up. Despite this tremendous milestone, scaling up to a full-fledged quantum computer is far from trivial: with these qubits, the flux-control causes crosstalk between qubits and heating, the room-temperature microwave control is hardly scalable and comes with high energetic radiation, and most importantly, the loss of quantum information in time leads to computational errors. Recent advances in various hybrid semiconductor materials enabled novel voltage-controlled transmons, gatemons, which are less susceptible to heating and crosstalk. Even more exciting, gatemons can be designed to host Majorana zero modes in a way that renders the qubit inherently protected against decoherence. In order to induce Majorana zero modes in such nanowire systems strong magnetic fields are required. Problematically, magnetic fields destroy the superconductivity that these microwave circuits rely on. In this thesis we integrate three types of hybrid Josephson junctions in magnetic field compatible microwave devices. Chapter 4 demonstrates the first graphene-based transmon. Due to the mono-atomic thickness of graphene in combination with magnetic field resilient coplanar waveguide resonators, we are able to operate the transmon circuit at an in-plane magnetic field of 1 Tesla. Chapter 5 embeds an InAs-Al semiconducting nanowire Josephson junction in a high quality factor superconducting transmission line resonator, demonstrating on-chip microwave generation. The gate-controllable semiconducting platform lends itself for fast pulse control, providing a perspective for the coherent on-chip manipulation of artificial two-level systems, in particular superconducting qubits such as transmons. Chapter 6 continues the development of InAs-Al nanowire transmons. The offset-charge-sensitive regime, additional plunger gates and magnetic field compatibility prepares the platform for the detection of coherent coupling between Majorana zero modes, a phenomena which unfortunately still remains unobserved. Additionally, we realise the first InSb-Al gatemon. The higher spin-orbit coupling makes InSb to be a preferred material in the search for Majorana signatures. Chapter 7 reports on the dynamics of quasiparticle tunneling events in real-time across the InAs-Al nanowire junction in a transmon architecture. The magnetic field compatibility of our device up to 1 Tesla together with in-situ voltage-controlled quasiparticle trap engineering, allows us to measure the survival of the charge-parity lifetime up to strong magnetic fields. A result which is extremely important in the research field of topological quantum computing, where the qubit space is defined in the charge-parity.