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arXiv:1801.01585 · Physical Review A

Spectral asymmetry of atoms in the van der Waals potential of an optical nanofiber

Burkley D. Patterson, Pablo Solano, Paul S. Julienne, Luis A. Orozco, S. L. Rolston

Published Mar 15, 2018• 12 citations
arXivHTMLPDF

Abstract

We measure the modification of the transmission spectra of cold $^{87}\mathrm{Rb}$ atoms in the proximity of an optical nanofiber (ONF). Van der Waals interactions between the atoms an the ONF surface decrease the resonance frequency of atoms closer to the surface. An asymmetric spectra of the atoms holds information of their spatial distribution around the ONF. We use a far-detuned laser beam coupled to the ONF to thermally excite atoms at the ONF surface. We study the change of transmission spectrum of these atoms as a function of heating laser power. A semiclassical phenomenological model for the thermal excitation of atoms in the atom-surface van der Waals bound states is in good agreement with the measurements. This result suggests that van der Waals potentials could be used to trap and probe atoms at few nanometers from a dielectric surface, a key tool for hybrid photonic-atomic quantum systems.

DOI
10.1103/physreva.97.032509

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We measure the modification of the transmission spectra of cold 87Rb^{87}\mathrm{Rb}87Rb atoms in the proximity of an optical nanofiber (ONF). Van der Waals interactions between the atoms an the ONF surface decrease the resonance frequency of atoms closer to the surface. An asymmetric spectra of the atoms holds information of their spatial distribution around the ONF. We use a far-detuned laser beam coupled to the ONF to thermally excite atoms at the ONF surface. We study the change of transmission spectrum of these atoms as a function of heating laser power. A semiclassical phenomenological model for the thermal excitation of atoms in the atom-surface van der Waals bound states is in good agreement with the measurements. This result suggests that van der Waals potentials could be used to trap and probe atoms at few nanometers from a dielectric surface, a key tool for hybrid photonic-atomic quantum systems.
We present measurements of the transmission spectra of 87Rb atoms at 780 nm in the vicinity of a nanofiber. A uniform distribution of fixed atoms around a nanofiber should produce a spectrum that is broadened towards the red due to shifts from the van der Waals potential. If the atoms are free, this also produces an attractive force that accelerates them until they collide with the fiber which depletes the steady-state density of near-surface atoms. It is for this reason that measurements of the van der Waals interaction are sparse. We confirm this by measuring the spectrum cold atoms from a magneto-optical trap around the fiber, revealing a symmetric line shape with nearly the natural linewidth of the transition. When we use an auxiliary 750 nm laser we are able to controllably desorb a steady flux of atoms from the fiber that reside near the surface (less than 50 nm) long enough to feel the van der Walls interaction and produce an asymmetric spectrum. We quantify the spectral asymmetry as a function of 750 nm laser power and find a maximum. Our model, which that takes into account the change in the density distribution, qualitatively explains the observations. In the future this can be used as a tool to more comprehensively study atom-surface interactions.
Surface-Induced Spectral Broadening during Efficient Two-Photon Excitation of Cold 133Cs^{133}\text{Cs}133Cs Atoms near an Optical Nanofiber
We report the experimental observation of the 133^{\text{133}}133Cs 6S1/2_{\text{1/2}}1/2​ to 6D5/2_{\text{5/2}}5/2​ single-frequency two-photon transition at low excitation power using an optical nanofiber embedded in a cold atom cloud. We investigate the 917 nm fluorescence spectra modified by the surface-induced interaction of the nanofiber, which exhibits a pronounced asymmetric broadening with a distinct red-shifted tail. We present a systematic theoretical description of the two-photon transition process of atoms near a nanofiber surface, considering atomic angular momentum coupling, guided-mode decay rate, and surface-induced van der Waals interactions. Owing to the tight spatial confinement provided by the guided evanescent field, efficient nonlinear excitation is realized at excitation powers down to tens of microwatts, corresponding to a reduction of approximately four orders of magnitude relative to typical free-space implementations. Our work reveals the interplay among waveguide-modified radiative dynamics, surface-induced interactions, and the spatial distribution of atoms around the nanofiber, and provides insights into further studies on nonlinear optical transitions and surface-mediated atomic dynamics in waveguide quantum electrodynamics systems.
We study the spontaneous emission of atoms near an optical nanofiber and analyze the coupling efficiency of the spontaneous emission into a nanofiber. We also investigate the influence of the van der Waals interaction of atoms with the surface of the optical nanofiber on the spectrum of coupled light. Using, as an example, 85 Rb atoms we show that the van der Waals interaction may considerably extend the red wing of the spontaneous emission line and, accordingly, produce a well-defined asymmetry of the spontaneous emission spectrum coupled into an optical nanofiber.
We analyse the lineshape of the fluorescence emitted by a cloud of optically excited cold atoms and coupled into an optical nanofibre. We examine the efficiency of the fluorescence coupling and describe the asymmetry of the lineshape caused by the redshifts arising from both the van der Waals and Casimir–Polder interaction of the atoms with the surface of the optical nanofibre. We compare the contributions of the van der Waals and Casimir–Polder redshifts and show that the lineshape of the fluorescence coupled into an optical nanofibre is, basically, influenced by the van der Waals redshift and is characterized by a long tail on the red side of the spectrum. We conclude that a measurement of the lineshape of the coupled fluorescence could be used to characterize the strength of the interaction of atoms with dielectric surfaces and for the detection of atoms using nanofibres.
In this thesis, a magneto-optical trap setup is used to laser cool and confine a cloud of 85Rb. The cloud typically contains 108 atoms in a 1 mm3 volume at a temperature in the region of the Doppler Limit (146 _K for 85Rb). To study the cold cloud, a subwavelength optical fibre - a nanofibre, or ONF - is positioned inside the cloud. The ONF can be used in two ways. Firstly, it is an efficient fluorescence collection tool for the cold atoms. Loading times, lifetimes and temperatures can be measured by coupling the atomic fluorescence to the evanescent region of the ONF. Secondly, the ONF is used as a probe beam delivery tool using the evanescent field properties of the device, allowing one to perform spectroscopy on few numbers of near-surface atoms. With improvements in optical density of the cloud, this system is an ideal candidate in which to generate electromagnetically induced transparency and slow light. A theoretical study of the van der Waals and Casimir-Polder interactions between an atom and a dielectric surface is also presented in this work in order to understand their effects in the spectroscopy of near-surface atoms.
We demonstrate how optical nanofibers can be used to manipulate and probe single-atom fluorescence. We show that fluorescence photons from a very small number of atoms, average atom number of less than 0.1, around the nanofiber can readily be observed through single-mode optical fiber under resonant laser irradiation. We show also that optical nanofibers enable us to probe the van der Waals interaction between atoms and surface with high precision by observing the fluorescence excitation spectrum.