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arXiv:1712.08701 · Journal of Physics Communications

Interacting superradiance samples: modified intensities and timescales, and frequency shifts

Martin Houde, Fereshteh Rajabi

Published Jul 12, 2018• 2 citations
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Abstract

We consider the interaction between distinct superradiance (SR) systems and use the dressed state formalism to solve the case of two interacting two-atom SR samples at resonance. We show that the ensuing entanglement modifies the transition rates and intensities of radiation, as well as introduces a potentially measurable frequency chirp in the SR cascade, the magnitude of which being a function of the separation between the samples. For the dominant SR cascade we find a significant reduction in the duration and an increase of the intensity of the SR pulse relative to the case of a single two-atom SR sample.

DOI
10.1088/2399-6528/aad300

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Interacting superradiance samples: modified intensities and timescales, and spectral broadening

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We consider the interaction between distinct superradiance (SR) samples and use the dressed state formalism to solve the case of two interacting two-atom SR samples at resonance. We show that the ensuing entanglement modifies the transition rates and intensities of radiation, as well as introduces a frequency chirp in the SR cascade that results in a potentially significant spectral broadening. For the dominant SR cascade we find a significant reduction in the duration and an increase of the intensity of the SR pulse relative to the case of a single two-atom SR sample.

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We consider the interaction between distinct superradiance (SR) systems and use the dressed state formalism to solve the case of two interacting two-atom SR samples at resonance. We show that the ensuing entanglement modifies the transition rates and intensities of radiation, as well as introduces a potentially measurable frequency chirp in the SR cascade, the magnitude of which being a function of the separation between the samples. For the dominant SR cascade we find a significant reduction in the duration and an increase of the intensity of the SR pulse relative to the case of a single two-atom SR sample.
We consider the interaction between distinct superradiance (SR) samples and use the dressed state formalism to solve the case of two interacting two-atom SR samples at resonance. We show that the ensuing entanglement modifies the transition rates and intensities of radiation, as well as introduces a frequency chirp in the SR cascade that results in a potentially significant spectral broadening. For the dominant SR cascade we find a significant reduction in the duration and an increase of the intensity of the SR pulse relative to the case of a single two-atom SR sample.
Fully-excited two-level atoms separated by less than the transition wavelength cooperatively emit light in a short burst, a phenomenon called superradiance by R. Dicke in 1954. The burst is characterized by a maximum intensity scaling with the square of the number of atoms NNN and a temporal width reduced by NNN compared to the single atom spontaneous decay time. Both effects are usually attributed to a synchronization of the electric dipole moments of the atoms occurring during the process of light emission. Contrary to this explanation, it was recently shown by use of a quantum path description that the peak intensity results from the quantum correlations among the atoms when occupying symmetric Dicke states. Here we investigate from this perspective the temporal evolution of the ensemble, starting in the small sample limit, i.e., when the atoms have mutual separations much smaller than the transition wavelength λλλ and pass down the ladder of symmetric Dicke states. In addition, we explore the temporal evolution for the case of non-interacting atoms with mutual separations much larger than λλλ. We show that in this case a similar superradiant burst of the emitted radiation is observed if the quantum correlations of the atoms are generated by conditional photon measurements retaining the atomic ensemble within or close to the symmetric subspace.
The superradiance (SR) phenomenon is considered for the case of a medium consisting of two resonant components. It is shown that the dynamics of emission in this case differs essentially from that for a monocomponent medium. The use of a two-component medium results in a substantial weakness in the requirements for duration of the pumping pulse. The peak pulse intensity of superradiance for the case of a two-component medium can exceed that for each of the components separately. By varying the active medium length and concentration of components we can control the spatiotemporal dynamics of emission. This enables us to transform the broadened pumping pulse of a lower intensity into the ultrashort high intensity pulse of SR.
Using the formalism developed earlier, we treat spontaneous emission from a pair of identical two-level atoms A1{A}_{1}A1​, A2{A}_{2}A2​, whose separation r21{r}_{21}r21​ can be comparable to the wavelength $\ensuremath{\lambda}$. We obtain expressions for time-dependent intensities and damping rates with the initial conditions (a) both atoms inverted, (b) prior excitation by a short $\frac{1}{2}\ensuremath{\pi}$ pulse, and (c) only A1{A}_{1}A1​ inverted. The results in (a) are compared with those obtained for a model consisting of two initially excited harmonic oscillators O1{O}_{1}O1​, O2{O}_{2}O2​. The atoms exhibit superradiant behavior, whereas O1{O}_{1}O1​, O2{O}_{2}O2​ tend to trap radiation. In (a), the intensity pattern $\mathcal{R}(\ensuremath{\theta},t)$ develops lobes in different directions at different times, so that the spatial distribution of photons at time $t\ensuremath{\rightarrow}\ensuremath{\infty}$ is the same as in the independent-atom case ${r}_{21}\ensuremath{\gg}\ensuremath{\lambda}$. For the oscillators, the lobes of $\mathcal{R}(\ensuremath{\theta},t)$ do not change direction, but only become more pronounced as time increases. In (b) and (c), the lobes oscillate back and forth at frequency $2{\ensuremath{\Omega}}_{12}$ corresponding to the shifts $\ifmmode\pm\else\textpm\fi{}{\ensuremath{\Omega}}_{12}$ of the triplet and singlet states due to the ${A}_{1}\ensuremath{-}{A}_{2}$ interaction. The intensity can therefore have a sinusoidal component. Field correlation functions calculated for (a) and (c) show that A2{A}_{2}A2​ and A2{A}_{2}A2​ radiate simultaneously around the frequencies $\ensuremath{\epsilon}\ifmmode\pm\else\textpm\fi{}{\ensuremath{\Omega}}_{12}$, where $\ensuremath{\epsilon}$ is the single-atom resonant frequency. The spectrum is calculated for case (c), and shows the effects of coherent linewidth enhancement in addition to the frequency shifts.
This thesis studies superradiance and subradiance in the normal modes of excitation of systems of resonant nuclei. The nuclei are treated as classical electric dipole oscillators interacting through their radiation fields. This coupling radically alters the radiative decay of the system relative to the decay of an isolated nucleus, and leads to both superradiant and subradiant states with strongly enhanced or suppressed radiative decay rates, and with normal mode frequencies which can be strongly shifted from the natural resonance frequency. This issue is of considerable current interest because it is now possible to create spatially coherent single exciton nuclear states by illuminating crystals containing resonant Mossbauer nuclei with synchrotron radiation pulses. The purpose of this thesis is to solve for the radiative eigenmodes in a system of nuclei and to investigate superradiance and subradiance both in the eigenmode solutions and in the synchrotron radiation produced nuclear exciton state.
The problem of the evolution in time of a system of two-level atoms that are coupled through their electromagnetic fields, is studied and solved in the framework of semiclassical radiation theory. The atoms may be in any initial states and the radiation reaction is fully taken into account. Both superradiance and time-dependent frequency shift or chirping effects are found. The assumption that all the atoms see the same field is shown to place severe constraints on the evolution of the system, in the form of constants of the motion. These constraints are most easily pictured in terms of the Bloch-vector representation of the atomic system, and they lead to explicit solutions for the time development of each atom. It is shown that the evolution of the complex system is describable by means of a collective super Bloch vector, whose behavior is similar to the behavior of the Bloch vector for a single isolated atom. The constraints on the motion also imply that the system cannot radiate all its energy coherently; some of it remains trapped, to be dissipated ultimately by incoherent processes. Some curves are presented to illustrate the behavior of the system in special cases.