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arXiv:1712.07100 · Physical Review A

Dynamics of tunneling ionization using Bohmian mechanics

Nicolas Douguet, Klaus Bartschat

Published Jan 8, 2018• 46 citations
arXivHTMLPDF

Abstract

Recent attoclock experiments and theoretical studies regarding the strong-field ionization of atoms by few-cycle infrared pulses revealed features that have attracted much attention. Here we investigate tunneling ionization and the dynamics of the electron probability using Bohmian mechanics. We consider a one-dimensional problem to illustrate the underlying mechanisms of the ionization process. It is revealed that in the major part of the below-the-barrier ionization regime, in an intense and short infrared pulse, the electron does not tunnel through the entire barrier, but rather starts already from the classically forbidden region. Moreover, we highlight the correspondence between the probability of locating the electron at a particular initial position and its asymptotic momentum. Bohmian mechanics also provides a natural definition of mean tunneling time and exit position, taking account of the time dependence of the barrier. Finally, we find that the electron can exit the barrier with significant kinetic energy, thereby corroborating the results of a recent study [N. Camus et al., Phys. Rev. Lett. 119, 023201 (2017)].

DOI
10.1103/physreva.97.013402

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Recent attoclock experiments and theoretical studies regarding the strong-field ionization of atoms by few-cycle infrared pulses revealed features that have attracted much attention. Here we investigate tunneling ionization and the dynamics of the electron probability using Bohmian mechanics. We consider a one-dimensional problem to illustrate the underlying mechanisms of the ionization process. It is revealed that in the major part of the below-the-barrier ionization regime, in an intense and short infrared pulse, the electron does not tunnel through the entire barrier, but rather starts already from the classically forbidden region. Moreover, we highlight the correspondence between the probability of locating the electron at a particular initial position and its asymptotic momentum. Bohmian mechanics also provides a natural definition of mean tunneling time and exit position, taking account of the time dependence of the barrier. Finally, we find that the electron can exit the barrier with significant kinetic energy, thereby corroborating the results of a recent study [N. Camus et al., Phys. Rev. Lett. 119, 023201 (2017)].
Abstract In recent experiments of single-cycle field ionization of excited Na( nd ) atoms with principal quantum number n ∈ [ 6 , 15 ] (Li and Jones 2014 Phys. Rev. Lett. 112 143006 ) it was shown that the maximum field intensity necessary to ionize 10% of the atoms decreases with increasing n according to an n − 3 power law dependence. This scaling property at the same ionization probability was confirmed in classical trajectory Monte Carlo calculations. In this work we note that the scaling relation in the experiment is much more general, it is in fact valid for all ionization probabilities. When applied to the emitted electron energies it places a very wide distribution of electron momenta from different initial states onto a narrow range. These aspects are investigated in a one-dimensional model with a 3D hydrogen-like spectrum. Calculations confirm the general n − 3 scaling relation for the ionization probability and that this particular scaling of the kinetic emission spectrum puts the ejected electron momenta on a narrow common scale. The ionization mechanism itself is identified as quantum mechanical tunneling and the nature of the tunneling process is the direct origin of the scaling law.
Tunnel-ionization is investigated in the framework of relativistic quantum mechanics. \nFor an arbitrary constant electromagnetic field a gauge invariant energy \noperator is introduced in order to identify the classically forbidden region for \ntunnel-ionization. Furthermore, relativistic features of tunnel-ionization are explored. \nA one-dimensional intuitive picture predicts that the ionized electron wave \npacket in the relativistic regime experiences a momentum shift along the laser’s \npropagation direction. This is shown to be consistent with the well-known strong \nfield approximation. Furthermore, spin dynamics in tunnel-ionization process \nis discussed in the standard as well as in the dressed strong field approximation. \nNext, the tunneling time delay is investigated for tunnel-ionization by extending \nthe definition of the Wigner time delay. Later, this concept is redefined in terms of \nthe phase of the fixed energy propagator. The developed formalism is applied to \nthe deep-tunneling and the near-threshold-tunneling regimes. It is shown that in \nthe latter case signatures of the tunneling time delay can be measurable at remote \ndistance. Finally, the path-dependent formulation of gauge theory is discussed. It \nis demonstrated that this equivalent formulation of gauge theory leads to a canonical \ngauge fixing, in which the Feynman path integral becomes more intuitive and \nthe calculation of the quasiclassical propagator is considerably simplified
Tunneling delays represent a hotly debated topic, with many conflicting definitions and little consensus on when and if such definitions accurately describe the physical observables. Here, we relate these different definitions to distinct experimental observables in strong field ionization, finding that two definitions, Larmor time and Bohmian time, are compatible with the attoclock observable and the resonance lifetime of a bound state, respectively. Both of these definitions are closely connected to the theory of weak measurement, with Larmor time being the weak measurement value of tunneling time and Bohmian trajectory corresponding to the average particle trajectory, which has been recently reconstructed using weak measurement in a two-slit experiment [S. Kocsis, B. Braverman, S. Ravets, M. J. Stevens, R. P. Mirin, L. K. Shalm, and A. M. Steinberg, Science 332, 1170 (2011)]. We demonstrate a big discrepancy in strong field ionization between the Bohmian and weak measurement values of tunneling time, and we suggest this arises because the tunneling time is calculated for a small probability postselected ensemble of electrons. Our results have important implications for the interpretation of experiments in attosecond science, suggesting that tunneling is unlikely to be an instantaneous process.
A clear consensus on how long it takes a particle to tunnel through a potential barrier has never been so urgently required, since the electron dynamics in strong-field ionization can be resolved on attosecond time-scale in experiment and the exact nature of the tunneling process is the key to trigger subsequent attosecond techniques. Here a general picture of tunneling time is suggested by introducing a quantum travel time, which is defined as the ratio of the travel distance to the expected value of the velocity operator under the barrier. Specially, if applied to rectangular barrier tunneling, it can retrieve the Büttiker-Landauer time τBLτ_{BL}τBL​ in the case of an opaque barrier, and has a clear physical meaning in the case of a very thin barrier wherein τBLτ_{BL}τBL​ can not be well defined. In the case of strong-field tunneling process, with the help of the newly defined time, the tunneling delay time measured by attoclock experiment can be interpreted as a travel time spent by the electron to tunnel from a point under the barrier to the tunnel exit. In addition, a peculiar oscillation structure in the wavelength dependence of tunneling delay time in deep tunneling regime is observed, which is beyond the scope of adiabatic tunneling picture. This oscillation structure can be attributed to the interference between the ground state tunneling channel and the excited states tunneling channels.
Tunneling ionization in static or slowly varying electric fields is a cornerstone of strong-field physics and provides the entry point for semiclassical descriptions of above-threshold ionization and high-harmonic generation. In conventional quantum mechanics, the Perelomov--Popov--Terent'ev (PPT) theory and its Ammosov--Delone--Krainov (ADK) form yield an ionization rate whose defining feature is an exponential dependence governed by an under-barrier (imaginary-time) action. Here we develop an analytical ADK-like tunneling model within \emph{space-fractional} quantum mechanics, where the quadratic kinetic energy is replaced by the Riesz fractional Laplacian of order 1<α≤21<α\le21<α≤2. Working in a static electric field in the length gauge, we derive a closed-form tunneling exponent for a triangular exit barrier. The fractional kinetic operator deforms the conventional Ip3/2I_p^{3/2}Ip3/2​ scaling to Ip1+1/αI_p^{1+1/α}Ip1+1/α​ and introduces a characteristic sin⁡(π/α)\sin(π/α)sin(π/α) factor encoding the complex-phase structure associated with nonlocal dispersion. We position this benchmark relative to prior tunneling studies in fractional quantum mechanics (primarily scattering through model barriers and fractal potentials) and provide a validation protocol for testing the exponent in time-dependent simulations of the fractional Schrödinger equation under a constant field. The result establishes a transparent reference for static-field ionization in nonlocal quantum dynamics and a baseline for strong-field approaches extensions.